Enhanced bio-ethanol production from bamboo residues by alkali-aided Fenton reaction pretreatment and enzymatic saccharification
Industrial Crops and Products(2023)
摘要
Alkali extraction was used to assist the Fenton pretreatment for overcoming the recalcitrance of bamboo and producing more sugar-based chemicals and bioethanol. The alkali-aided Fenton pretreatment showed the delignification of 55.33% and xylan removal of 80.76%. The surface lignin coverage, hydrophobicity, specific surface area, and cellulose crystallinity index were obviously changed by the combined pretreatment, which made cellulose accessibility increased by about 2-folds than Fenton pretreatment alone. The cleavage of β-O-4 linkage, the decrease of condensed structure and syringyl unit were observed in the residual lignin from the NaOH-Fenton pretreated D. brandisii, all of which reduced the nonproductive adsorption between enzymes and lignin. When NaOH-Fenton pretreated four bamboo residues were performed enzymatic hydrolysis, glucose yields of 66–74% and ethanol concentration of 11–16 g/L were obtained. The sequential NaOH-Fenton pretreatment should be considered as an environmentally-friendly bamboo biorefinery technology in the future.
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关键词
Bamboo residues,Alkali extraction,Fenton pretreatment,Lignin modification,Nonproductive adsorption,Enzymatic saccharification
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