Experimental Demonstration of Robotic Active Matter Micellization

Active matter composed of self-propelled particles features a fascinating set of self-organization phenomena, spanning from motility-induced phase separation to phototaxis to topological excitations depending on the nature and parameters of the system. In the present Letter, we consider the formation of micelles from particles with a broken symmetry having a circular back and a sharpened nose and moving towards the cusp. As we demonstrate in experiments with robotic swarms, such particles can either remain in the isotropic phase or form micelles depending on the location of their center of inertia in accordance with a recent theoretical proposal [T. Kruglov, A. Borisov, Particles 2021 (2021)]. Crucially, the predicted micellization does not involve any charge asymmetry, in contrast to that observed in surfactants, and is governed by an interplay of activity and particle shape asymmetry. This renders the observed ordering reversible upon switching of the particles' activity and opens the route towards novel applications in tunable structuring of materials.