Easy-plane multi-𝐪 magnetic ground state of Na_3Co_2SbO_6
arxiv(2023)
Abstract
Na_3Co_2SbO_6 is a potential Kitaev magnet with a monoclinic layered
crystal structure. Recent investigations of the C_3-symmetric sister compound
Na_2Co_2TeO_6 have uncovered a unique triple-𝐪 magnetic ground
state, as opposed to a single-𝐪 (zigzag) one, prompting us to
examine the influence of the reduced structural symmetry of Na_3Co_2SbO_6
on its ground state. Neutron diffraction data obtained on a twin-free crystal
reveal that the ground state remains a multi-𝐪 state, despite the
system's strong in-plane anisotropy. This robustness of multi-𝐪
orders suggests that they are driven by a common mechanism in the honeycomb
cobaltates, such as higher-order magnetic interactions. Spin-polarized neutron
diffraction results show that the ordered moments are entirely in-plane, with
each staggered component orthogonal to the propagating wave vector. The
inferred ground state favors a so-called XXZ easy-plane anisotropic starting
point for the microscopic model over a Kitaev one, and features unequal ordered
moments reduced by strong quantum fluctuations.
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