Boron-coated straw detector technology as an alternative to helium-3 and boron trifluoride based proportional counters for ground level neutron monitoring: a design study.

Michael Aspinall, Cory Binnersley, Steve Bradnam,Stephen Croft,Malcolm Joyce,Lee Packer, Jim Wild

crossref(2022)

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摘要
<p>The global network of neutron monitors comprises predominantly of the monitor standardised by Carmichael in 1964, the NM-64.&#160; The design of these existing monitors and their instrumentation have changed very little over the last sixty years. &#160;For example, their neutron detectors rely on gas filled proportional counters that are either filled with highly toxic boron trifluoride (BF<sub>3</sub>) or helium-3 (<sup>3</sup>He).&#160; Almost the entire global supply of <sup>3</sup>He is derived from a waste product of nuclear weapons programmes and, with the termination of such programmes and reducing nuclear weapons stockpile, the supply of <sup>3</sup>He has become limited.&#160; Consequently, <sup>3</sup>He supply became strictly controlled in 2008 and its price has fluctuated since.&#160; In some cases, new neutron monitors have reverted to BF<sub>3</sub> filled counter tubes when the price of <sup>3</sup>He has been at a premium.&#160; Helium-3 filled proportional counters are also used extensively in radiation portal monitors deployed for homeland security and non-proliferation; objectives which have increased significantly over the last two decades.&#160; The reduced production and increased demand for <sup>3</sup>He has led to concerns over its supply and provided the research motivation for alternative neutron detection methods which are viable in terms of sensitivity, stability and gamma-rejection for certain applications.&#160; One of these alternative technologies is based on boron-coated straws (BCS) manufactured and supplied by Proportional Technologies, Inc (PTI). &#160;The technology is built on a patented low-cost technology that enables long copper tubes, known as &#8216;straws&#8217;, to be coated on the inside with a thin layer of <sup>10</sup>B-enriched boron carbide (<sup>10</sup>B<sub>4</sub>C).&#160; Thermal neutrons captured in the <sup>10</sup>B are converted into secondary particles, through the <sup>10</sup>B(n, &#945;) reaction.&#160; The straws can be of various diameter (circa 4 mm to 15 mm), length (up to 2 m) and shape (round, star or pie) to increase the surface area of <sup>10</sup>B.&#160; Multiple straws can be packed inside a 1&#8221; diameter aluminium tube acting as a single drop-in replacement for traditional <sup>3</sup>He detectors or individually distributed directly throughout the moderating medium, thus increasing efficiency by detecting the thermal neutrons at the point that they are created.&#160; BCS-based detectors are widely used in systems for homeland security, safeguards and neutron imaging in direct exchange for <sup>3</sup>He tubes.&#160; This study aims to design a neutron monitor utilising BCS technology that is cheaper, more compact and produces comparable results to the existing network of NM-64 monitors.&#160; Monte Carlo simulations using the MCNP radiation transport code to model several BCS-based solutions and an NM-64 computational benchmark are reported.&#160; These models are validated experimentally using a standard PTI portal monitor (PTI-110-NDME) to determine its efficiency, dieaway, deadtime and gamma rejection using a combination of bare <sup>252</sup>Cf, AmLi and <sup>137</sup>Cs sources.&#160; The PTI-110-NDME consists of a 12&#8221; x 5&#8221; x 1 m high density polyethylene (HDPE) slab with thirty ~15-mm diameter straws, 93 cm active length, embedded uniformly throughout the moderator. &#160;Funded by UK Research & Innovation (UKRI), this research is part of the Space Weather Instrumentation, Measurement, Modelling and Risk (SWIMMR) programme.</p>
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