Strongly Localized Moir Exciton in Twisted Homobilayers

SMALL(2024)

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摘要
Artificially molding exciton flux is the cornerstone for developing promising excitonic devices. In the emerging hetero/homobilayers, the spatial separated charges prolong exciton lifetimes and create out-plane dipoles, facilitating electrically control exciton flux on a large scale, and the nanoscale periodic moire potentials arising from twist-angle or/and lattice mismatch can substantially alter exciton dynamics, which are mainly proved in the heterostructures. However, the spatially indirect excitons dynamics in homobilayers without lattice mismatch remain elusive. Here the nonequilibrium dynamics of indirect exciton in homobilayers are systematically investigated. The homobilayers with slightly twist-angle can induce a deep moire potential (>50 meV) in the energy landscape of indirect excitons, resulting in a strongly localized moire excitons insulating the transport dynamics from phonons and disorder. These findings provide insights into the exciton dynamics and many-body physics in moire superlattices modulated energy landscape, with implications for designing excitonic devices operating at room temperature.
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关键词
exciton dynamics,homobilayers,localized excitons,moire superlattices
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