Topology of Bi_2Se_3 nanosheets
arXiv (Cornell University)(2023)
摘要
Recently, the quantum spin-Hall edge channels of two-dimensional colloidal
nanocrystals of the topological insulator Bi_2Se_3 were observed directly.
Motivated by this development, we reconsider the four-band effective model
which has been traditionally employed in the past to describe thin nanosheets
of this material. Derived from a three-dimensional k·p model, it physically describes the top and
bottom electronic surface states that become gapped due to the material's small
thickness. However, we find that the four-band model for the surface states
alone, as derived directly from the three-dimensional theory, is inadequate for
the description of thin films of a few quintuple layers and even yields an
incorrect topological invariant within a significant range of thicknesses. To
address this limitation we propose an eight-band model which, in addition to
the surface states, also incorporates the set of bulk bands closest to the
Fermi level. We find that the eight-band model not only captures most of the
experimental observations, but also agrees with previous first-principles
calculations of the ℤ_2 invariant in thin films of varying
thickness. Moreover, we demonstrate that the topological properties of thin
Bi_2Se_3 nanosheets emerge as a result of an intricate interplay between
the surface and bulk states. In particular, the surface bands of the eight-band
model differ drastically from their counterparts in their four-band model, with
the missing topology of the latter restored by the newly added bulk bands.
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关键词
nanosheets,topology
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