Continuous-Wave Lasing in Perovskite LEDs with an Integrated Distributed Feedback Resonator

Advanced materials (Deerfield Beach, Fla.)(2023)

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摘要
Realization of electrically pumped laser diodes based on solution-processed semiconductors is a long-standing challenge. Metal halide perovskites have shown great potential toward this goal due to their excellent optoelectronic properties. Continuous-wave (CW) optically pumped lasing in a real electroluminescent device represents a key step to current-injection laser diodes, but it has not yet been realized. This is mainly due to the challenge of incorporating a resonant cavity into an efficient light-emitting diode (LED) able to sustain intensive carrier injection. Here, CW lasing is reported in an efficient perovskite LED with an integrated distributed feedback resonator, which shows a low lasing threshold of 220 W cm-2 at 110 K. Importantly, the LED works well at a current density of 330 A cm-2, indicating the carrier injection rate already exceeds the threshold of optically pumping. The results suggest that electrically pumped perovskite laser diodes can be achieved once the Joule heating issue is overcome. Continuous-wave lasing in an efficient perovskite LED with an integrated distributed feedback resonator is achieved, showing a low threshold of 220 W cm-2 at 110 K. The LED can also work well at a current density of 330 A cm-2, indicating the carrier injection rate already exceeds the threshold of optically pumping. The results suggest that electrically pumped perovskite laser diodes can be achieved once the Joule heating issue is overcome.image
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continuous-wave,light-emitting diodes,metal halide perovskites,perovskite lasers
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