Top-down vs. bottom-up synthesis of Ga–based supported catalytically active liquid metal solutions (SCALMS) for the dehydrogenation of isobutane

Narayanan Raman, Jakob Söllner,Nnamdi Madubuko,Sharanya Nair,Nicola Taccardi,Matthias Thommes,Marco Haumann,Peter Wasserscheid

Chemical Engineering Journal（2023）

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摘要

•Isobutane dehydrogenation catalyzed by supported liquid alloys (SCALMS).•Comparison between two synthesis protocols.•Distribution of alloy particles either inside or outside of support material.•Evidence for pore blocking from detailed sorption and intrusion studies.•Catalytic performance correlates with alloy distribution.

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关键词

catalytically,active liquid metal solutions,dehydrogenation,synthesis,top-down

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