Lightning the Spin: Harnessing the Potential of 2D Magnets in Opto-Spintronics

Since the emergence of 2D magnets in 2017, the diversity of these materials has greatly expanded. Their 2D nature (atomic-scale thickness) endows these magnets with strong magnetic anisotropy, layer-dependent and switchable magnetic order, and quantum-confined quasiparticles, which distinguish them from conventional 3D magnetic materials. Moreover, the 2D geometry facilitates light incidence for opto-spintronic applications and potential on-chip integration. In analogy to optoelectronics based on optical-electronic interactions, opto-spintronics use light-spin interactions to process spin information stored in the solid state. In this review, opto-spintronics is divided into three types with respect to the wavelengths of radiation interacting with 2D magnets: 1) GHz (microwave) to THz (mid-infrared), 2) visible, and 3) UV to X-rays. It is focused on the recent research advancements on the newly discovered mechanisms of light-spin interactions in 2D magnets and introduces the potential design of novel opto-spintronic applications based on these interactions. 2D magnets provide diverse magnetic orders for spins to be aligned, including intralayer ferromagnetism, antiferromagnetism, and interlayer (A-type) antiferromagnetism, which allow the spins to precess in a wide range of frequency from GHz to X-ray. By interacting with the given wavelength of light/electromagnetic wave, the spins can be excited (written) and detected (read), realizing different types of opto-spintronic devices and functions.image