Creating an Ethane Trap in a Ketone-Decorated MOF for One-Step Ethylene Separation from C2 Hydrocarbons

Mingxing Zhang, Meng Chen,Junyang Jiang, Xingge He, Haitian Zhao,Yu Wang,Penghui Liu,Rui Dang,Su Wang,Miao Wang,Tongming Sun,Guoping Qin,Yanfeng Tang,Huihui Cui

INORGANIC CHEMISTRY（2023）

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摘要

One-step C2H4 purification from a mixture of C2H2/C2H4/C2H6 by physical adsorption separation was realized via creating an ethane trap in MOF NTUniv-63 by the utilization of a ketone-decorated semirigid ligand, which has further been verified by the breakthrough experiment, isosteric heats of adsorption (Q(st)), and Grand Canonical Monte Carlo (GCMC) modeling.

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