THz-induced carrier multiplication in TaAs Weyl semimetal

2023 48TH INTERNATIONAL CONFERENCE ON INFRARED, MILLIMETER, AND TERAHERTZ WAVES, IRMMW-THZ(2023)

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摘要
Topological Dirac and Weyl semimetals (D&W SM) have attracted a lot of attention due to their unusual electronic properties, which are strongly dependent on the symmetry of the system. By altering the symmetry of the lattice, using for example a pulse of light, one can expect to modify their topological nature and induce/suppress the related properties "on demand". High-field Terahertz (THz) radiation that interacts with vibrational states under near-resonant conditions is a promising pump candidate to induce structural changes in D& W SM compounds, possibly leading to topological transient or permanent changes. There are, however, some challenges to achieving such control. D&W SM have a specific band structure showing a 3D-linear dispersion around nodes, which makes them sensitive to THz-induced carrier multiplication. These carrier multiplication processes can compete with and ultimately screen the interaction of the THz light with vibrational modes. Here, we present recent results of 2D-THz spectroscopy of a bulk Weyl semimetal TaAs in reflection. We highlight THz-induced carrier multiplication effects and study the field and temperature dependence of the number of carriers induced by the THz field. We examine possible carrier multiplication mechanisms which could be involved.
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关键词
2D-terahertz spectroscopy,3D-linear dispersion,band structure,electronic properties,lattice symmetry,near-resonant conditions,TaAs/bin,terahertz radiation,terahertz-induced carrier multiplication,topological Dirac semimetals,vibrational modes,vibrational states,Weyl semimetal
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