Solvent modulation strategy for Sb-based anode to achieve stable potassium storage

Ningning Chen,Nailu Shen,Xiaoping Yi,Yinshuang Pang,Zhi Liu,Hong Chen,Jing Zheng,Qingxue Lai,Yanyu Liang

CHEMICAL ENGINEERING JOURNAL（2023）

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摘要

•A novel ether-ester mixed electrolyte is applied to the Sb@NC alloy electrode.•Ethylene carbonate can change the solvation environment of K+.•Molecular dynamics simulations reveal electron transfer pathways.•Electrolyte exchange experiments further demonstrate the dynamics of SEI.

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关键词

Solvation structure,Solid electrolyte interphase (SEI),Potassium-ion batteries,Sb-based alloy type anode

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