Multiple and nonlocal cation redox in Ca–Ce–Ti–Mn oxide perovskites for solar thermochemical applications

Robert B. Wexler,Gopalakrishnan Sai Gautam,Robert T. Bell,Sarah Shulda,Nicholas A. Strange,Jamie A. Trindell,Joshua D. Sugar,Eli Nygren,Sami Sainio,Anthony H. McDaniel,David S. Ginley,Emily A. Carter,Ellen B. Stechel

Energy and Environmental Science（2023）

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摘要

Ca 2/3 Ce 1/3 Ti 1/3 Mn 2/3 O 3 demonstrates promising two-step thermochemical H 2 production potential. Quantum-based modeling highlights A-site Ce 4+ reduction as the key factor in its redox activity, providing insights for further performance optimization.

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关键词

ca–ce–ti–mn oxide perovskites,nonlocal cation redox,solar thermochemical applications

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