Beneficial vs. inhibiting passivation by the native lithium solid electrolyte interphase revealed by electrochemical Li⁺ exchange

Gustavo M. Hobold,Kyeong‐Ho Kim,Betar M. Gallant

Energy and Environmental Science（2023）

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摘要

Electrolytes that achieve highest Li Coulombic efficiency display quantifiably higher rates of electrochemical Li + exchange. The effect is attributed to their improved SEI and better-percolated Li deposits that boost Li + exchange as the cell cycles.

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electrochemical lithium,solid electrolyte interphase,native lithium

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Beneficial vs. inhibiting passivation by the native lithium solid electrolyte interphase revealed by electrochemical Li+ exchange

Beneficial vs. inhibiting passivation by the native lithium solid electrolyte interphase revealed by electrochemical Li⁺ exchange