Giant domain wall anomalous Hall effect in an antiferromagnet

arxiv(2023)

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摘要
The Hall effect plays a crucial role in establishment of band theory of solids and discovery of emergent new phases of interacting electrons such as the topological phases of matter. Generally, the dissipationless Hall effect requires time-reversal symmetry breaking (TRSB), where TRSB induced by external magnetic field results in ordinary Hall effect, while TRSB caused by spontaneous magnetization gives rise to anomalous Hall effect (AHE) which scales with the net magnetization. The AHE is therefore not expected in antiferromagnets with vanishing small magnetization. However, large AHE was recently observed in certain antiferromagnets with noncolinear spin structure and nonvanishing Berry curvature, thus opening a new area for exploration of large AHE in antiferromagnets. Here, we report another origin of AHE in a layered antiferromagnet, namely the domain wall (DW) skew scattering with Weyl points near the Fermi level, in experiments for the first time. Interestingly, the DWs form a unique periodic stripe structure with controllable periodicity by external magnetic field, which decreases nearly monotonically from 975 nm at 0 T to 232 nm at 4 T. Electrons incident on DW with topological bound states experience strong asymmetric scattering, leading to giant extrinsic AHE, with the DW Hall conductivity (DWHC) at 2 K and 1.2 T even reaching a record value of about 1.51*104 S cm-1 among bulk systems, which is two orders of magnitude larger than the intrinsic anomalous Hall conductivity. The observation of giant DWHC and controllable stripe DW structure in an antiferromagnet not only sets a new paradigm for exploration of large extrinsic anomalous Hall effect, but also provides potential applications in spintronic devices.
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