Synthesis of CC/BiPO<sub>4</sub>/Bi<sub>2</sub>WO<sub>6</sub> Composite Material and Its Photocatalytic Performance
Optics and Photonics Journal(2023)
摘要
Along with the popularity of environmental protection concepts, the environmental treatment of water pollution attracts widespread attention, among which, the research on Bi-based semiconductor photocatalytic degradation technology has made great progress. However, the development of such bismuth-based composites still remains a challenging task due to difficult recovery and low catalytic efficiency. Herein, a novel CC/BiPO4/Bi2WO6 composite was successfully synthesized through two-step hydrothermal method using activated flexible carbon cloth as a substrate. The results of the photocatalytic degradation experiments showed that the obtained CC/BiPO4/Bi2WO6 composites can degrade 92.1% RhB in 60 min under UV-visible light irradiation, which was much higher than that of unloaded BiPO4 (24.4%) and BiPO4/Bi2WO6 (52.9%), exhibiting a better adsorption-photocatalytic degradation performance than BiPO4 and BiPO4/Bi2WO6. Photoluminescence spectra indicated that the improved photocatalytic activity was due to the more effective inhibition of photogenerated carrier complexation. Furthermore, the radical capture experiments confirmed that h+, ·OH and O2- were the main active substances in the photocatalytic degradation process of RhB by the CC/BiPO4/Bi2WO6 composites. More importantly, the prepared CC/BiPO4/Bi2WO6 composite had a simple separation process and good recycling stability, and its photocatalytic degradation efficiency can still reach 53.3% after six cycles of RhB degradation.
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关键词
photocatalytic performance,synthesis,composite material,cc/bipo&,lt,sub&,gt,4&,lt,/sub&,gt,/bi&,lt,sub&,gt,2&,lt,/sub&,gt,wo&,lt,sub&,gt,6&,lt,/sub&,gt,,cc/bipo&,lt,sub&,gt,4&,lt,/sub&,gt,/bi&,lt,sub&,gt,2&,lt,/sub&,gt,wo&,lt,sub&,gt,6&,lt,/sub&,gt,
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