Tuning exciton emission via ferroelectric polarization at a heterogeneous interface between a monolayer transition metal dichalcogenide and a perovskite oxide membrane
arxiv(2024)
摘要
We demonstrate the integration of a thin BaTiO_3 (BTO) membrane with
monolayer MoSe_2 in a dual gate device that enables in-situ manipulation of
the BTO ferroelectric polarization with a voltage pulse. While two-dimensional
(2D) transition metal dichalcogenides (TMDs) offer remarkable adaptability,
their hybrid integration with other families of functional materials beyond the
realm of 2D materials has been challenging. Released functional oxide membranes
offer a solution for 2D/3D integration via stacking. 2D TMD excitons can serve
as a local probe of the ferroelectric polarization in BTO at a heterogeneous
interface. Using photoluminescence (PL) of MoSe_2 excitons to optically
readout the doping level, we find that the relative population of charge
carriers in MoSe_2 depends sensitively on the ferroelectric polarization.
This finding points to a promising avenue for future-generations versatile
sensing devices with high sensitivity, fast read-out, and diverse applicability
for advanced signal processing.
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