Spin Supersolid Phase and Double Magnon-Roton Excitations in a Cobalt-based Triangular Lattice

Supersolid is an exotic quantum state of matter that hosts spontaneously the features of both solid and superfluidity, which breaks the lattice translational symmetry and U(1) gauge symmetry. Here we conduct inelastic neutron scattering (INS) measurements and tensor-network calculations on the triangular-lattice cobaltate Na_2BaCo(PO_4)_2, which is proposed in [Xiang et al., Nature 625, 270-275 (2024)] as a quantum magnetic analog of supersolid. We uncover characteristic dynamical signatures, which include distinct magnetic Bragg peaks indicating out-of-plane spin solidity and gapless Goldstone modes corresponding to the in-plane spin superfluidity, offering comprehensive spectroscopic evidence for spin supersolid in Na_2BaCo(PO_4)_2. We also compute spin dynamics of the easy-axis triangular-lattice model, and reveal magnon-roton excitations containing U(1) Goldstone and roton modes associated with the in-plane spin superfluidity, as well as pseudo-Goldstone and roton modes related to the out-of-plane spin solidity, rendering double magnon-roton dispersions in the spin supersolid. Akin to the role of phonon-roton dispersion in shaping the helium thermodynamics, the intriguing magnetic excitations also strongly influence the low-temperature thermodynamics of spin supersolid down to sub-Kelvin regime, explaining the recently observed giant magnetocaloric effect in Na_2BaCo(PO_4)_2.