Magnetic phase diagram of EuPdSn_2
arxiv(2024)
摘要
A magnetic phase diagram for EuPdSn_2 is constructed based on magnetization,
DC-susceptibility and specific heat as a function of applied field, and neutron
diffraction results at zero field. The contribution of the ferromagnetic FM and
antiferromagnetic AFM components to the measured magnetic susceptibility can be
separated and weighted as a function of the applied field B by taking the
temperature dependence of the neutron counts from the FM phase at B=0 as a
reference. In the magnetically ordered phase, the temperature dependence of the
specific heat does not follow the mean-field prediction for the Eu^2+ J=7/2
quantum number rather that for J=5/2. This deviation and the consequent
discrepancy for the entropy is discussed in the context of a non-Zeeman
distribution of the eight fold ground state. Comparing the respective
variations of magnetization M(T,B) and entropy S(T,B), the thermodynamic
relationship dM/dT=dS/dB=0 is observed for the ranges: 0更多
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