Magnetic hysteresis mechanism in Lu0.9Sr0.1Cr0.5Fe0.5O3 studied by Monte Carlo simulations.
Journal of physics. Condensed matter : an Institute of Physics journal(2024)
摘要
In this work we report magnetic properties of the orthorhombic perovskite
Lu0.9Sr0.1Cr0.5Fe0.5O3 synthesized by a wet chemical method. As in LuCr0.5Fe0.5O3 the compound
with Sr shows the magnetization reversal phenomenon, but the magnetic order and the compensation
temperature occur at higher temperatures. Interestingly, in M vs H curves a hysteresis loop is observed
when Cr4+ and Cr3+ ions coexist as a consequence of the aliovalent substitution of Lu3+ by Sr2+ in the
B sites of the perovskite. To explain this behavior, we performed numerical simulations with a
magnetic model for Lu1-xSrxCr0.5Fe0.5O3 perovskites with x=0 and x=0.1. We found that the
ferromagnetic coupling of Fe3+ and Cr4+ through superexchange interactions (according the empiric
Goodenough-Kanamori-Anderson rules, GKA) increases the magnetization at high fields and that the
presence of ferromagnetic clusters explains the hysteretic behavior found in simulations.
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