A universal technique is developed for the detection of high harmonics generated by relativistic and subrelativistic laser pulses irradiating a solid target. Features in the spectra of harmonics generated by a parametric mid-IR laser system and near-IR laser system based on chirped pulse amplification were analyzed. Experimental spectra of harmonics in the range up to 35 nm were recorded. They can be used as a source of coherent radiation in the extreme UV region.

Terahertz pulse generation from multiterawatt laser surface plasma near thick solid targets and thin foils has been studied. Pulses with energies up to 7 μJ were detected in the spectral region <3 THz in the direction of specular reflection from the surface of the CaF 2 target. The dependence of the terahertz pulse energy $${{W}_{{{\text{THz}}}}}$$ on the laser pulse intensity $$I_{L}^{\alpha }$$ can be approximated by the power function $${{W}_{{{\text{THz}}}}} \sim I_{L}^{\alpha }$$ . For a fixed laser pulse duration and variable energy the power index lies in the range $$\alpha \approx 1.5{-} 2.8$$ , while for a fixed energy and variable duration $$\alpha \approx 1$$ .

We obtained the spectra of high optical harmonics produced by subrelativistic femtosecond pulses on the surface of polystyrene, CaF 2 , BK7, and Al solid targets. High harmonics of up to the 51st order of radiation with central 3.85 µm wavelength were observed. The highest order harmonics were generated from the polystyrene target surface. The harmonics energy versus their numbers is shown to fit well a decaying power law with the exponent ranging from 4 to 8/3.

We obtained the spectra of high optical harmonics produced by subrelativistic femtosecond pulses on the surface of polystyrene, CaF2, BK7, and Al solid targets. High harmonics of up to the 51st order of radiation with central 3.85 µm wavelength were observed. The highest order harmonics were generated from the polystyrene target surface. The harmonics energy versus their numbers is shown to fit well a decaying power law with the exponent ranging from 4 to 8/3.

Combined optical nonlinearity of bound and free electrons in a fast-ionizing medium driven by ultrashort, mid-infrared (mid-IR) pulses gives rise to a vast variety of ultrafast nonlinear-optical scenarios, producing bright, broadband radiation in spectral ranges as different as ultraviolet (UV) and terahertz (THz). Given its enormous bandwidth, a quantitative experimental analysis of this type of nonlinear response is anything but simple. Here, we confront this challenge by ultrabroadband spectral measurements performed across the spectral range from the UV to the millimeter-wave (MMW) band jointly with beam profile analysis in the THz-to-MMW band and direct time-domain field waveform characterization. As one of the most striking results, the nonlinear response of a fast-ionizing gas driven by a two-color field, consisting of a high-peak-power sub-100-fs mid-IR pulse and its second harmonic, is shown to provide a source of a bright multiband supercontinuum (SC) radiation, whose spectrum spans over about 14 octaves, stretching from below 300 nm all the way beyond 4.3 mm. The MMW-to-THz part of this SC is emitted, as direct measurements show, in the form of half-cycle field waveforms that can be focused to yield a field strength of≈5MV/cm. At least 1.5% of the MMW–THz supercontinuum energy is emitted in the MMW range, giving rise to MMW field strengths up to 100 kV/cm in the beam waist region.

We identify and experimentally demonstrate a physical scenario whereby high-peak-power mid-infrared (mid-IR) pulses can be compressed as a part of their free-beam spatiotemporal evolution within the regions of anomalous dispersion in air to yield few-cycle subterawatt field waveforms. Unlike filamentation-assisted pulse compression, the pulse-compression scenario identified in this work does not involve any noticeable ionization of air, enabling a whole-beam self-compression of mid-IR laser pulses without ionization-induced loss. Ultrashort high-peak-power 3.9 ae m laser pulses are shown to exhibit such self-compression dynamics when exposed to the dispersion anomaly of air induced by the asymmetric-stretch rovibrational band of carbon dioxide. Even though the group-velocity dispersion cannot be even defined as a single constant for the entire bandwidth of mid-IR laser pulses used in experiments, with all soliton transients shattered by high-order dispersion, 100 -200 GW, 100 fs, 3.9 ae m laser pulses can be compressed in this regime to 35 fs subterawatt field waveforms. (C) 2017 Optical Society of America

Recent breakthroughs in ultrafast photonics in the mid-IR help understand complex interactions of high-intensity mid-IR field waveforms with matter, offer new approaches for x-ray generation, enable mid-IR laser filamentation in the atmosphere, facilitate lasing in filaments, give rise to unique regimes of laser-matter interactions, and reveal unexpected properties of materials in the mid-IR range.

We present experimental studies of long-distance transmission of ultrashort mid-infrared laser pulses through atmospheric air, probing air dispersion in the 3.6–4.2-μm wavelength range. Atmospheric air is still highly transparent to electromagnetic radiation in this spectral region, making it interesting for long-distance signal transmission. However, unlike most of the high-transmission regions in gas media, the group-velocity dispersion, as we show in this work, is anomalous at these wavelengths due to the nearby asymmetric-stretch rovibrational band of atmospheric carbon dioxide. The spectrograms of ultrashort mid-infrared laser pulses transmitted over a distance of 60 m in our experiments provide a map of air dispersion in this wavelength range, revealing clear signatures of anomalous dispersion, with anomalous group delays as long as 1.8 ps detected across the bandwidth covered by 80-fs laser pulses.

Angle-resolved spectral analysis of a multioctave high-energy supercontinuum output of mid-infrared laser filaments is shown to provide a powerful tool for understanding intricate physical scenarios behind laser-induced filamentation in the mid-infrared. The ellipticity of the mid-infrared driver beam breaks the axial symmetry of filamentation dynamics, offering a probe for a truly (3+1)-dimensional spatiotemporal evolution of mid-IR pulses in the filamentation regime. With optical harmonics up to the 15th order contributing to supercontinuum generation in such filaments alongside Kerr-type and ionization-induced nonlinearities, the output supercontinuum spectra span over five octaves from the mid-ultraviolet deep into the mid-infrared. Full (3+1)-dimensional field evolution analysis is needed for an adequate understanding of this regime of laser filamentation. Supercomputer simulations implementing such analysis articulate the critical importance of angle-resolved measurements for both descriptive and predictive power of filamentation modeling. Strong enhancement of ionization-induced blueshift is shown to offer new approaches in filamentation-assisted pulse compression, enabling the generation of high-power few- and single-cycle pulses in the mid-infrared.