This article contains my personal account on how I got interested in spin transport phenomena, which ultimately resulted in investigating multiple facets of spin-orbit torques, as well as magnetization dynamics. Originally this research focused on questions that seemed rather academic with little relevance to applications. But over time it developed into one of the key research areas for modern spintronic devices. This journey started off with investigating spin polarized charge currents, later focused on pure spin currents, and ultimately explored spin waves (magnons) as the potential carriers of spin information. Most of this work was performed in the Magnetic Films group of the Argonne National Laboratory, which for more than three decades used to be one of the world-leading places for magnetism research.
Hybrid magnonic systems have recently attracted significant attention due to their intriguing physics and potential applications in coherent information processing. In this regard, we have investigated magnonmagnon coupling in the all-oxide insulator garnet Y3Fe5O12 (YIG)/Tm3Fe5O12 (TmIG) heterostructure. The presence of an avoided mode crossing region between the ferromagnetic resonance modes of YIG and TmIG indicates interfacial exchange coupling. This all-insulator system enables interfacial coupling via magnon-magnon interactions. The mode crossing occurs at fc = 6.88 GHz, corresponding to the minimal resonance separation between the two hybrid modes. The coupling strength is determined to be 78 MHz (or 2.8 mT), providing clear evidence of magnon-magnon coupling between the two Kittel modes in the YIG/TmIG insulator system at 200 K. These findings pave the way for engineering magnonic band structures, tunable coherent magnonic interactions, and nonreciprocal spin transport, which are crucial for advancing ultralow-power magnonic devices.
The orbital angular momentum of electrons presents exciting opportunities for developing energy-efficient, low-power magnetic devices. Typically, the generation of orbital currents is driven by the transfer of orbital angular momentum from 3d transition metal magnets, either through the application of an electric field using the orbital Hall effect or through magnetization dynamics. Chiral phonons are quantized lattice vibrations that carry non-zero angular momentum due to the circular motion of atoms. An interplay of chiral phonon dynamics and electrons would enable the direct generation of orbital angular momentum, even without the need for magnetic elements. Here we experimentally demonstrate the generation of orbital currents from chiral phonons activated in the chiral insulator α-quartz under an applied magnetic field and a temperature gradient. We refer to this phenomenon as the orbital Seebeck effect. The generated orbital current is selectively detected in tungsten and titanium films deposited on quartz through the inverse orbital Hall effect. Our findings hold promise for orbitronics based on chiral phonons in non-magnetic insulators and shed light on the fundamental understanding of chiral phonons and their interaction with electron orbitals. Generation of orbital currents in a non-magnetic material can be useful to build efficient orbitronic devices. Now, the interplay of chiral phonons and electrons is shown to produce orbital currents in α-quartz.
Spin waves (magnons) in two-dimensional (2D) materials have received increasing interest due to their unique states and potential for tunability. However, many interesting features of these systems, including Dirac points and topological states, occur at high frequencies, where experimental probes are limited. Here, we study a crystal formed by patterning a hexagonal array of holes in a perpendicularly magnetized thin film. Through simulation, we find that the magnonic band structure imitates that of graphene, but additionally has some kagomelike character and includes a few flat bands. Surprisingly, its nature can be understood using a nine-band tight-binding Hamiltonian. This clear analogy to 2D materials enables band-gap engineering in 2D, topological magnons along 1D phase boundaries, and spectrally isolated modes at 0D point defects. Interestingly, the 1D phase boundaries allow access to the valley degree of freedom through a magnonic analog of the quantum valley Hall insulator. These approaches can be extended to other magnonic systems, but are potentially more general due to the simplicity of the model, which resembles existing results from electron, phonon, photon, and cold-atom systems. This finding brings the physics of spin waves in 2D materials to more experimentally accessible scales, augments it, and outlines a few principles for controlling magnonic states.
Due to the presence of robust spin-sublattices, which have a low susceptibility to external magnetic field, spin current induced torques play a key role in antiferromagnetic-spintronic device implementations. Since the torque-efficiency is highly dependent on the angle between the spin polarization and the local moments, the noncollinear antiferromagnet IrMn3 with its well-defined local moment orientations dictated by the kagome lattice presents a unique prototypical materials system for such studies in antiferromagnets. In this work, we have investigated the optimum substrate choice and deposition conditions of (001) oriented IrMn3 in addition to spin-orbit torque effects due to a spin current from a positive (or negative) spin Hall angle neighboring Pt (or W) layer. Comparison with the collinear Ir20Mn80/Pt bilayers clarifies the contribution to the current induced resistance change from the triangular spin structure of IrMn3. Our study enables the assessment of the effectiveness of the spin-orbit torque induced manipulation of the Neel vector in noncollinear antiferromagnetic systems.
Spontaneous dynamic systems have attracted significant attention for their rich underlying physics such as phase-locking and synchronization. In this work, we report a new mechanism of generating magnetic spontaneous oscillation via parametric pumping. By applying a pump tone to excite propagating spin waves in a yttrium iron garnet delay line, four-wave mixing converts the pump mode into two phase-autonomous propagating magnon modes, i.e. a spontaneous mode with nearly twice the wavenumber of the pump mode and an idler mode with nearly zero wavenumber. This allows us to reliably generate ultrasharp spin wave dynamics with broad frequency tunability from the pump and magnetic field. We show that the spontaneous mode can be phase-locked to a probe tone, similar to an auto-oscillator. Furthermore, the spontaneous dynamics can be used to implement a high-gain magnonic parametric amplifier with a gain up to 40 dB. Our results open a new avenue for studying nonlinear magnonics and synchronization physics in propagating magnon geometry and for developing new magnonic devices.
Cluster magnetic multipoles are order parameters that characterize the symmetry of spin arrangements in magnetic materials. In particular, high-order multipoles play a pivotal role in altermagnets and non-collinear antiferromagnets where they govern electrical and optical phenomena. While spatially non-uniform multipole textures have been observed on the micrometer scale, their behavior at mesoscopic lengths remains largely unexplored. Here, we introduce a comprehensive micromagnetic framework for vector-like cluster magnetic multipoles, enabling quantitative, spatially resolved analysis of non-uniform multipole systems. As a demonstration, we apply the framework to magnetic-octupole domain-wall motion in the non-collinear antiferromagnet Mn_3Sn. Our simulations capture key features of domain-wall dynamics, including profile deformation and the emergence of an effective inertial mass. This work provides a unified approach for investigating the mesoscopic dynamics of high-order cluster multipoles, and opens new avenues for understanding and engineering the physical properties of functional magnetic materials, such as altermagnets and non-collinear antiferromagnets, for advanced spintronic technologies.
Magnetic skyrmions and related topological spin textures have emerged as a central topic in condensed-matter physics, combining fundamental significance with potential for transformative applications in spintronics, magnonics, and beyond. Over the past decade, advances in material platforms, imaging techniques, theoretical modeling, and device concepts have established skyrmionics as a rapidly expanding field. At the same time, challenges remain in stabilizing, controlling, and integrating such textures into functional architectures, while novel phenomena such as antiskyrmions, higher-order skyrmions, hopfions, and antiferromagnetic textures arise. The 2026 Skyrmionics Roadmap represents a collective effort of many authors, providing a comprehensive perspective on the current state-of-the-art and the outlook for the coming years. In 33 focused sections, each co-authored by two researchers, we chart progress in theory and modeling, material systems, skyrmion dynamics, and skyrmion technologies. By offering a consolidated vision, this Roadmap aims to guide both fundamental research and application-driven efforts, accelerating the transition of skyrmionics from conceptual breakthroughs toward practical technologies.
Materials with broken fundamental symmetries, such as chiral crystals, provide a rich playground for exploring unconventional spin-dependent transport phenomena. The interplay between a material's chirality, strong spin-orbit coupling, and charge currents can lead to complex non-reciprocal effects, where electrical resistance depends on the direction of current and magnetic fields. In this study, we systematically investigate the angular dependencies of magnetoresistance in single-crystalline chiral tellurium (Te). We observe distinct non-reciprocal magnetoresistances for magnetic fields applied along three orthogonal directions: parallel to the current along the chiral axis (z), in the sample plane but perpendicular to the current (y), and out of the sample plane (x). Through the detailed analysis of the chirality- and thickness dependence of the signals, we successfully disentangle multiple coexisting mechanisms. We conclude that the Edelstein effect, arising from the chiral structure's radial spin texture, is responsible for the non-reciprocity along the z axis. In contrast, the chirality-independent signal along the y axis is attributed to the Nernst effect, and the non-reciprocity along the x axis may originate from the orbital magnetization. These findings elucidate the complex interplay of spin, orbital, and thermal effects in Te, providing a complete picture of its non-reciprocal transport properties.
We demonstrate strong coupling between propagating spin wave modes and microwave photons in superconducting resonator-magnetic thin film hybrid circuits. By fabricating the resonator directly on yttrium iron garnet thin films grown on rare-earth-free Y_3Sc_2Ga_3O_12 substrates, we achieve strong coupling of both Damon-Eshbach and backward-volume spin wave modes to the resonator, with coupling strengths exceeding both the magnon and photon damping rates. Furthermore, we observe nonreciprocal spin wave radiation of the hybrid magnonic mode in the Damon-Eshbach configuration, highlighting the potential for incorporating intrinsic spin-wave nonreciprocity into hybrid magnonic systems. These results open new avenues for integrating spin-wave magnonics with cavity magnonics, and for harnessing spin waves for potential applications in quantum information science.
Spin-orbit torques have emerged as a powerful mechanism for manipulating magnetic moments in spintronic devices, offering a pathway to more efficient and scalable memory and logic technologies. While conventional spin-orbit torques generated in heavy metals and topological insulators have been extensively studied, recent advancements in unconventional spin-orbit torques demonstrated out-of-plane spin polarizations that could effectively switch perpendicular magnetizations without the need for additional external in-plane magnetic fields, promising significant implications for the development of energy-efficient and compact spintronic devices. Unconventional spin-orbit torques are usually found in materials with low symmetries, such as transition metal dichalcogenides, topological insulators, and 2-D materials. Here, we provide a brief overview of unconventional spin-orbit torques and present two example material systems: CrPt3 and MoTe2, both exhibiting strong spin-orbit coupling and phase-dependent spin-orbit torques, and focus on their unique origins and potential applications. We discuss the roles of magnetic and crystallographic orders in generating unconventional spin-orbit torques, highlighting how these factors contribute to the observed anisotropic and directional dependencies.
Magnons, the quanta of collective spin excitations in magnetic materials, may enable functionalities, such as nonreciprocity and transduction in hybrid quantum devices. To assess the potential of such applications, it is necessary to understand magnon dynamics beyond the simple harmonic oscillator regime, where theory predicts effects like population-dependent damping and quantum fluctuations in the form of magnon shot noise. Probing these phenomena requires sensors with high sensitivity and the ability to resolve magnon properties across different excitation regimes. Here, we demonstrate accurate and sensitive detection of magnon population and decay over a wide range of occupation numbers. We use a superconducting qubit to probe magnons in a ferrimagnet over approximately 2000 excitations. Using qubit control and parametrically induced qubit-magnon interactions, we demonstrate few-excitation sensitive detection of magnons with a dynamic range of approximately 30 dB, and are able to accurately resolve their decay with few-ns sensitivity. These capabilities offer a powerful and practical technique for probing magnon dynamics in or beyond the linear regime over a wide range of excitations.
Spin textures that are not readily available in the domain structures of continuous magnetic thin films can be stabilized when patterned to micro/nano scales due to the dominant effect of dipolar magnetic interactions. Fabrication of such devices enables a thorough study of their RF dynamics excited by highly concentrated spin-polarized/pure-spin currents. For this purpose, in this study, we have employed a truncated astroid geometry to achieve stable magnetic antivortex core nucleation/annihilation which was detectable using the anisotropic magnetoresistance (AMR) at various temperatures. Furthermore, by depositing a soft magnetic thin film (20 nm thick permalloy) capped with a heavy-metal 2nm Pt layer, we were able to probe the spin orbit torque induced excitations accompanied by self-torque due to half-antivortex cores reminiscent of an isolated-antivortex, yielding GHz frequency oscillations with high quality factors (~50000). The observed RF oscillations can be attributed to a non-uniform domain wall oscillation mode close to the stable-antivortex core nucleation site as seen in micromagnetic simulations. This fundamental study of antivortex core response to spin currents is crucial for the assessment of their potential applications in high frequency spintronic devices such as reservoir computers.
Magnetic thin films with strong magnetoelastic coupling and low Gilbert damping are key materials for many magnetoelectric devices. Here, we investigated the effects of boron doping concentration on magnetostriction and temperature dependent Gilbert damping in magnetron sputtered (Fe80Ga20)1-xBx films. A crystalline to amorphous structural transition was observed for a boron content near 8% and coincided with a decrease in coercivity from 76 Oe to 3 Oe. A 10% doping concentration is optimal for achieving both large magnetostriction of 48.8 ppm and low Gilbert damping of 6x10-3. The temperature dependence of the damping shows an increase at low temperatures with a peak around 40 K, and we associate the relative increase A alpha/alpha RT with magnetoelastic contributions to the damping, which has a maximum of 55.7% at 8% boron. An increase in the inhomogeneous linewidth broadening was observed in the structural transition regime at about 8% boron concentration. This study suggests that incorporation of glass forming elements, in this case boron, into Fe80Ga20 is a practical pathway for simultaneously achieving enhanced magnetoelastic coupling and reduced Gilbert damping.
Magnon interference is a hallmark of coherent magnon interactions. In this work, we demonstrate single-shot magnon interference using up to four magnon pulses in two remotely coupled yttrium iron garnet spheres mediated by a coplanar superconducting resonator. By exciting one YIG sphere with injected microwave pulses, we achieve coherent energy exchange between the two spheres, facilitating their interference processes, including Rabi-like oscillation with a single pulse, constructive and destructive interference with two pulses, and interference peak sharpening with up to four pulses—analogous to diffraction grating in optical interference. The resulting interference patterns can be precisely controlled by changing the frequency detuning and time delay of the magnon pulses. The demonstration of time-domain coherent control of remote magnon interference opens new pathways for advancing coherent information processing through multi-operation, circuit-integrated hybrid magnonic networks.
The advance of magnon spintronics requires understanding of time-domain magnon pulse transmission in order to develop high-speed information processing protocols. In this work, we demonstrate single-shot electrical detection of narrow-band magnon pulse transmission in a yttrium iron garnet thin-film delay line. The high signal-to-background ratio of magnon transmission band allows us to directly probe the magnon transmission electrically using a fast oscilloscope and to study its spectral evolution using Fast Fourier Transform (FFT) of the time-domain transmitted signal. At elevated input power, we show a magnon transmission reduction and a spectral distortion, which can be understood by the nonlinear magnon excitation in the transmission band defined by the antenna geometry. In addition, we also find that the higher- (lower-) frequency magnon spectral component exhibits a lower (higher) magnon group velocity, showing a dispersion agreeing with the Damon-Eshbach dependence. Our results provide important guidance of magnon pulse engineering for their applications in spin wave computing and coherent magnon information processing.
The scalable synthesis of materials with strong spin orbit coupling (SOC) is crucial for the development of spintronic and magnetic devices. Here, wafer-scale growth of 1T' MoTe2 using metal-organic chemical vapor deposition (MOCVD) at low temperatures (400 °C) is demonstrated. The synthesized films exhibit uniform coverage across the entire substrate, as well as accurate stoichiometry. This low-temperature synthesis is compatible with silicon back-end-of-line (BEOL) processes, enabling in-memory and in-sensor computing for data-intensive applications. Furthermore, it was found that the grown 1T' MoTe2 exhibits strong spin-orbit coupling, as revealed by the spin torque ferromagnetic resonance (ST-FMR) measurements conducted on a 1T' MoTe2/permalloy bilayer. These measurements indicate significant damping-like torques in the wafer-scale 1T' MoTe2 film and indicate high spin-charge conversion efficiency. The BEOL-compatible process and potent spin orbit torque demonstrate the promise of MOCVD-grown MoTe2 in advanced device applications.
The chiral induced spin selectivity (CISS) effect, in which the structural chirality of a material determines the preference for the transmission of electrons with one spin orientation over that of the other, is emerging as a design principle for creating next-generation spintronic devices. CISS implies that the spin preference of chiral structures persists upon injection of pure spin currents and can act as a spin analyzer without the need for a ferromagnet. Here, we report an anomalous spin current absorption in chiral metal oxides that manifests a colossal anisotropic nonlocal Gilbert damping with a maximum-to-minimum ratio of up to 1000%. A twofold symmetry of the damping is shown to result from differential spin transmission and backscattering that arise from chirality-induced spin splitting along the chiral axis. These studies reveal the rich interplay of chirality and spin dynamics and identify how chiral materials can be implemented to direct the transport of spin current.
We investigate the structural and electronic origin of antiferromagnetic (AFM) coupling in the yttrium iron garnet (YIG) and permalloy (Ni80Fe20, 80 Fe 20 , Py) bilayer system at the atomic level. Ferromagnetic resonance (FMR) spectra reveal unique hybrid modes in samples prepared with surface ion milling, indicative of antiferromagnetic exchange coupling at the YIG/Py interface. Using atomic resolution scanning transmission electron microscopy (STEM), we found that AFM coupling appears at the YIG/Py interface of the tetrahedral YIG surface formed with ion milling. The STEM measurements suggest that the interfacial AFM coupling is predominantly driven by an oxygen-mediated superexchange coupling mechanism, which is confirmed by the density-functional theory (DFT) calculations to be energetically favorable. Thus, the combined experimental and theoretical results reveal the critical role of interfacial atomic structure in determining the type of magnetic coupling in a YIG/ferromagnet heterostructure, and prove that the interfacial structure can be experimentally tuned by surface ion milling.
Spin-orbit torques have emerged as a powerful mechanism for manipulating magnetic moments in spintronic devices, offering a pathway to more efficient and scalable memory and logic technologies. While conventional spin-orbit torques generated in heavy metals and topological insulators have been extensively studied, recent advancements in unconventional spin-orbit torques demonstrated out-of-plane spin polarizations that could effectively switch perpendicular magnetizations without the need for additional external in-plane magnetic fields, promising significant implications for the development of energy-efficient and compact spintronic devices. Unconventional spin-orbit torques are usually found in materials with low symmetries, such as transition metal dichalcogenides, topological insulators, and two-dimensional (2D) materials. Here we provide a brief overview of unconventional spin-orbit torques and present two example material systems: CrPt3 and MoTe2, both exhibiting strong spin-orbit coupling and phase-dependent spin-orbit torques, and focus on their unique origins and potential applications. We discuss the roles of magnetic and crystallographic orders in generating unconventional spin-orbit torques, highlighting how these factors contribute to the observed anisotropic and directional dependencies.