Microplastic (MP) pollution in the aquatic environment has become a problem of growing concern due to potential adverse effects on aquatic organisms and ecosystems. While MP transport and fate in marine systems has been researched to quite some extent relatively little is known about the transport mechanisms of MP particles in terrestrial surface waters and in saturated porous media like in groundwater or the hyporheic zone (HZ). We investigated the transport and fate of small (1, 3 and 10 μm diameter) polystyrene MP particles in a rippled, sandy stream bed (D50 = 1.04 mm) using CFD simulations calibrated to a set of flume experiments. A novel detection system for fluorescent MP particles (Boos et al. 2021) was used to track and quantify particle movement in the turbulent open water and in the hyporheic sediments in the laboratory flume following a pulse injection of MP particles into the surface water compartment. A new, integrated CFD simulation scheme within the OpenFOAM suite of CFD solvers was implemented for the flume system for a seamless simulation of water flow and particle transport in the open water and in the hyporheic sediments (Dichgans et al. 2023). Additionally we simulated the transport and fate of a range of “virtual” particles in the open water for different channel geometries using a Lagrangian approach. Simulations show that 1 μm MP particles are transported through the HZ like a solute, following the typical hyporheic flow cells below the bedforms. Transport and particle progression through the HZ could be adequately described with an advection-dispersion equation. Larger 10 µm MP particles instead showed retarded transport through the HZ, while retardation increased with travel distance in the sediments. Our results indicate that advective pumping across the streambed interface can transport very small MP particles through the HZ, while larger particles are increasingly retained. Distinct flow structures in the open water are found to be decisive for the fate of MP particles in the river channel. References: Dichgans, F., Boos, J.P., Ahmadi, P., Frei, S., Fleckenstein, J.H. (2023), Integrated numerical modeling to quantify transport and fate of microplastics in the hyporheic zone, Water Research, 243, https://doi.org/10.1016/j.watres.2023.120349 Boos, J.-P., Gilfedder, B. S., & Frei, S. (2021), Tracking microplastics across the streambed interface: Using laserinduced-fluorescence to quantitatively analyze microplastic transport in an experimental flume. Water Resources Research, 57, e2021WR031064.https://doi.org/10.1029/2021WR031064 Boos, J.-P., Dichgans, F., Fleckenstein, J.H., Gilfedder, B. S., Frei, S. (2024) Assessing the Behavior of Microplastics in Fluvial Systems: Infiltration and Retention Dynamics in Streambed Sediments. Water Resources Research, accepted

Microplastics (MPs) have been detected ubiquitously in fluvial systems and advective transfer has been proposed as a potential mechanism for the transport of (sub-) pore-scale MPs from surface waters into streambed sediments. However, the influence of particle and sediment properties, as well as the hydrodynamic flow regime, on the infiltration behavior and mobility of MPs in streambed sediments remains unclear. In this study, we conducted a series of flume experiments to investigate the effect of particle size (1-10 mu m), sediment type (fine and coarse sand), and flow regime (high/low flow) on particle infiltration dynamics in a rippled streambed. Quantification of particles in the flume compartments (surface flow, streambed interface, and in the streambed) was achieved using continuous fluorescence techniques. Results indicated that the maximum infiltration depth into the streambed decreased with increasing particle size (11, 10, and 7 cm for 1, 3, and 10 mu m). The highest particle retardation was observed in the fine sediment experiment, where 22% of the particles were still in the streambed at the end of the experiment. Particle residence times were shortest under high flow conditions, suggesting that periods of increased discharge can effectively flush MPs from streambed sediments. This study provides novel insights into the complex dynamics of MP infiltration and retention in streambed sediments and contributes to a better understanding of MPs fate in fluvial ecosystems. Quantitative data from this study can improve existing modeling frameworks for MPs transport and assist in assessing the exposure risk of MPs ingestion by benthic organisms. Microplastics (MPs) (small plastic particles) are present in river systems worldwide. The processes that lead to their transport and retention in rivers are not fully understood. Scientists have proposed that the infiltration of surface water into the streambed can carry MPs with it. In this study, we conducted experiments in a controlled environment that resembles a stream and its streambed. We investigated how different sizes of plastic particles (1, 3, and 10 mu m), the types of sediment (fine and coarse sand), and water flow rates (low and high) affect how far particles travel in a streambed. We found that the size of MPs played a significant role in their depth of infiltration. Larger particles did not infiltrate as deeply as smaller particles, and were also retained in the streambed. Fine sand trapped particles for a longer time than coarse sand, and 22% of the particles remained in the streambed until the end of the experiment. Faster flowing water quickly removed MPs from the streambed. Our research helps understand how MPs spread in river systems and how long they remain in the streambed. The data can be used to improve transport models and assess the risk MPs pose to aquatic organisms. (Sub-) Pore-scale microplastics were advectively transferred from the surface water into the streambed sediments in flume experiments Infiltration patterns depend on microplastic size, streambed sediment type and surface flow velocities Microplastic retention was observed for 10 mu m beads, 1 mu m beads were considerably retarded in fine sediments

Background The dataset contains data on Microplastic transport experiments run in an experimental flume of the University of Bayreuth. It was analysed in the paper by J.P. Boos, F. Dichgans, J.H. Fleckenstein, B.S. Gilfedder and S. Frei, "Assessing the Behavior of Microplastics in Fluvial Systems: Infiltration and Retention Dynamics in Streambed Sediments", currently under review in Water Resources Research Description of the dataset This dataset contains data used for individual particle detection, and is a companion of the main dataset (10.5281/zenodo.10083568). The files need to be downloaded and merged into the given folder structure. Put the folder "1Pix" along with the folder "10Pix" to the folder in "210812/Data-FIS/matlab/2_Experiment/exp/". Disclaimer The data and code are provided as is without any warranty. Funding Funded by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) -– Project Number 391977956 –- SFB 1357.

Despite the significance of rivers and streams as pathways for microplastics (MP) entering the marine environment, limited research has been conducted on the behavior of MP within fluvial systems. Specifically, there is a lack of understanding regarding the infiltration and transport dynamics of MP across the streambed interface and within the hyporheic sediments. In this study, transport and retention of MP are investigated using a new numerical modeling approach. The model is built as a digital twin of accompanying flume experiments, which are used to validate the simulation results. The model accurately represents particle transport in turbulent water flow and within the hyporheic zone (HZ). Simulations for transport and infiltration of 1 µm MP particles into a sandy streambed demonstrate that the advection-dispersion equation can be used to adequately represent particle transport for pore-scale sized MP within the HZ. To assess the applicability of the modeling framework for larger MP, the experiment was repeated using 10 µm particles. The larger particles exhibited delayed infiltration and transport behavior, and while the model successfully represented the spatial extent of particle transport through the HZ, it was unable to fully replicate hyporheic transit times. This study is the first to combine explicit validation against experimental data, encompassing qualitative observations of MP concentration patterns and quantification of fluxes. By that, it significantly contributes to our understanding of MP transport processes in fluvial systems. The study also highlights the advantages and limitations of employing a fully integrated modeling approach to investigate the transport and retention behavior of MP in rivers and streams.

The majority of microplastics (MPs) in marine environments originate from terrestrial sources and are transported by rivers and streams. In fluvial systems, interactions between particles, biota and sediments influence particle mobility and retention. It has been shown that the transport behaviour of MPs differs from the one of natural sediments. However, specific transport mechanisms for MPs are not yet fully understood, mainly because of the limited availability of reliable experimental data. As part of this study, transport mechanisms for MPs in fluvial systems (surface flow and hyporheic sediments) were investigated using an experimental flume environment. Realistic flow conditions were represented by varying sediment characteristics (e.g. glass beads or sand) and bedform structures (e.g. riffle-pool sequences, ripples and dunes). To track MPs in i) surface flow, ii) at the streambed interface and iii) within hyporheic sediments, we developed a quantitative method for fluorescent MP particles (1-10 mu m) based on state-of-the-art fluorometric techniques. Particle velocities in surface flow were measured by Particle-Image Velocimetry and LaserDoppler-Velocimetry. With this setup, for the first time it was possible to quantitatively track advective MP transfer from surface flow into the streambed sediments. Empirical results obtained from this study can be used in a next step to establish and validate transport models for MPs.

Although rivers and streams are major transport vectors of microplastics into the marine environment, little research has been conducted to understand the transport behavior of microplastic particles in fluvial systems. This work contributes to the understanding of these transport processes, specifically focusing on the interface of the surface water flow and the hyporheic zone. Transport of microplastic particles in fluvial systems is currently modeled mainly at larger, river- or basin-wide scales using existing hydrodynamic and sediment transport models. To investigate the transport behavior of microplastic particles along the interface between the hyporheic zone and the open water flow domain, smaller-scale models are required so that the complex processes in this region can be adequately represented and analyzed. To this end, a novel modeling technique will be presented based on the open source CFD toolbox OpenFOAM. It combines a new coupling approach for the hydrodynamic processes in the surface water and hyporheic zone with transport modeling of microplastics. The methodology considers the latest findings regarding deposition and resuspension of microplastic particles as well as the hyporheic exchange in a fully coupled model. The model is validated by accompanying flume experiments and relevant transport processes are identified from the presented scenario simulations.

Rivers and streams are a primary transport vector for microplastics (MPs), connecting terrestrial sources to marine environments. While previous studies indicated that pore-scale MPs can accumulate in streambed sediments, the specific MPs transport and retention mechanisms in fluvial systems remain poorly understood. We present a novel method for a quantitative analysis of the spatiotemporal transport and retention of pore-scale MPs in an experimental flume. A continuous mass balance for MPs in surface water was achieved using two online fluorometers, while a laser-induced Fluorescence-Imaging-System was developed to track and quantify the spatial migration of MPs through the streambed sediments. The detection limit was <1 μg/L for 1 μm polystyrene microbeads with the fluorometers and 3 μg/L for the Fluorescence-Imaging-System. The system was able to quantitatively track the advective transfer of MPs into the streambed sediments: a process that has yet not been observed experimentally. Results showed that MPs infiltrated into the streambed sediments up to a depth twice the bedform amplitude. This work provides a novel experimental method to quantitatively monitor MP transport through porous media and advective exchange of MP across the streambed interface.

The files contain datasets that were generated during laboratory-based real-time valvometry, and laser doppler anemometry measurements. The article was published in Journal of Hazardous Materials (accepted June 8, 2022).

Rivers and streams are a primary transport vector for microplastics (MPs), connecting terrestrial sources to marine environments. While previous studies indicated that pore‐scale MPs can accumulate in streambed sediments, the specific MPs transport and retention mechanisms in fluvial systems remain poorly understood. As part of this technical note, we present a novel method for a quantitative analysis of the spatiotemporal transport and retention of pore‐scale MPs in an experimental flume. A continuous mass balance for MPs in surface water was achieved using two online fluorometers, while a laser‐induced Fluorescence‐Imaging‐System was developed to track and quantify the spatial migration of MPs through the streambed sediments. The detection limit was <1 μg/L for 1 μm polystyrene microbeads with the fluorometers and 3 μg/L for the Fluorescence‐Imaging‐System. The system was able to quantitatively track the advective transfer of MPs into the streambed sediments: a process that has yet not been observed experimentally. Results showed that MPs infiltrated into the streambed sediments up to a depth twice the bedform amplitude. This work provides a novel experimental method to quantitatively monitor MP transport through porous media and advective exchange of MP across the streambed interface.

Rivers and streams are the dominant transport vectors for microplastic (MP) input into marine environments. During transport, complex physicochemical interactions between particles, water and river sediments influence particle mobility and retention. The specific transport mechanisms of MP in fluvial systems are not yet fully understood, and the main reason lies in the limitation in reliable data derived from experimental analysis.In our subproject of the ‘CRC 1357 Microplastics’, we investigate the hydrodynamic mechanisms that control the transport and retention behavior of MP in open channel flows and streambed sediments. In an experimental flume environment, we create realistic hydrodynamic and hyporheic flow conditions by using various porous media (e.g. glass beads or sand) and bedform structures (e.g. riffle-pool sequences, ripples and dunes), modelled from real stream systems.The method developed here can quantitatively analyze the transport of pore-scale particles (1-40 µm) based on fluorometric techniques. Particle velocity distributions and particle transport are measured using Particle-Image-Velocimetry and Laser-Doppler-Velocimetry. With our setup, we can quantitatively investigate time-resolved MP transport and retention through the aqueous and solid phase in a flume scale experiment.

&lt;p&gt;Although a major part of marine microplastic (MP) pollution originates from rivers and streams, the mechanistic behavior of MP in fluvial systems is only poorly understood. MP enter fluvial systems from e.g. waste water treatment plant (WWTP) effluents, sewer overflows during heavy rain events, agricultural runoff, aerial input/atmospheric fallout, road runoff or via fragmentation of plastic litter. As part of this project we want to investigate the hydrodynamic transport mechanisms that control the behavior and re-distribution of MP in open channel flow and the streambed sediments. Hydrodynamic conditions in open channel flow are represented in an experimental flume environment.&amp;#160; Different porous media materials (e.g. aqua beads, glass beads and sand) are used in the flume experiments to shape typical bed form structures such as riffle-pool sequences, ripples and dunes. The aim of this experimental setup is to create hydrodynamic flow conditions such as hydraulic jumps, low and high flow velocity environments for which the transport and sedimentation behavior of MP can be investigated under realistic conditions. Hydrodynamic flow conditions in the flume are characterized using a Laser-Doppler-Anemometry (LDA) and Particle Image Velocimetry (PIV). Detection and tracking of fluorescent MP-particles in open channel flow and in porous media will be achieved with a fluorescence-camera-system.&lt;/p&gt;

Microplastics (MPs) have been found ubiquitously in oceanic and terrestrial environments. As the production and consumption of plastic polymers increases the amount of plastic evading accepted disposal pathways and entering natural systems is also expected to increase. To date the focus of plastic and MP research in particular has been on the ocean, there has recently been a rapid increase in interest in MP levels and distribution in terrestrial systems. However, the focus of existing studies has mostly been on the quantification and distribution of MP contamination in the sediment or on the water column of rivers and lakes. The aim of this project is to investigate the fundamental physical and biological influences on the transport of microplastics (MPs) in lake systems. In particular, we will focus on an understanding of the migration and distribution of MPs, and a systematic investigation on transport and sedimentation of MP in the lake water column. Lab and field experiments are planned to investigate the behavior of different MPs polymers, shapes and sizes under different conditions and determine how this influence the MP transport. The settling velocity of MPs in stationary water was measured in the laboratory using particle image velocimetry (PIV) which was then compared to manual timing of the sinking velocity. The trajectories of the settling MPs have also been tracked during weak turbulences. In addition, the results were compared with theoretical calculations. To investigate microbial colonization and biofilm formation on the surface of MPs, samples were exposed on a natural lake environment for varying time periods. The colonization of MP surfaces by microorganisms and their excretion of extracellular polymeric substances (EPS) were examined by laser microscopic techniques and subsequently the effect of the microbiological colonization of settling velocity was determined. In this work we show that the transport of MP is complex, as it is influenced by plastic type, shape, and biological colonization as well as the hydrodynamic conditions in the lake water column.