Nonreciprocal quantum devices with low loss are indispensable in quantum information processing but challenging to be realized. Here we report an experiment to realize the nonreciprocal phase shift larger than rr with low loss in a cavity-free and magnetic-free cold atomic ensemble based on electromagneti-cally induced transparency. Furthermore, a four-port all-optical circulator is demonstrated with an average isolation ratio of 22.25 dB and transmission of 0.94 for each channel. At its optimal working point, the circulator's total isolation ratio reaches 63.47 dB, transmission reaches 0.86, and fidelity at about 0.99. Our work can advance further investigation of nonreciprocity with cold atoms in quantum information processing applications.

Quantum interference between identical single particles reveals the intrinsic quantum statistic nature of particles, which could not be interpreted through classical physics. Here, we demonstrate quantum interference between non-identical bosons using a generalized beam splitter based on a quantum memory. The Hong-Ou-Mandel type interference between single photons and single magnons with high visibility is demonstrated, and the crossover from the bosonic to fermionic quantum statistics is observed by tuning the beam splitter to be non-Hermitian. Moreover, multi-particle interference that simulates the behavior of three fermions by three input photons is realized. Our work extends the understanding of the quantum interference effects and demonstrates a versatile experimental platform for studying and engineering quantum statistics of particles.

Time synchronization and phase shaping of single photons both play fundamental roles in quantum information applications that rely on multi-photon quantum interference. Phase shaping typically requires separate modulators with extra insertion losses. Here, we develop an all-optical built-in phase modulator for single photons using a quantum memory. The fast phase modulation of a single photon in both step and linear manner are verified by observing the efficient quantum-memory-assisted Hong-Ou-Mandel interference between two single photons, where the anti-coalescence effect of bosonic photon pairs is demonstrated. The developed phase modulator may push forward the practical quantum information applications.

We report the generation of heralded single photons with Gaussian-shape temporal waveforms through the spatial light modulation technique in an atomic ensemble. Both the full width at half maximum and the peak position of the Gaussian waveform can be controlled while the single photon nature holds well. We also analyze the bandwidth of the generated single photons in frequency domain and show how the sidebands of the frequency spectrum are modified by the shape of the temporal waveform. The generated single photons are especially suited for the realization of high efficiency quantum storage based on electromagnetically induced transparency.

A quantum memory, for storing and retrieving flying photonic quantum states, is a key interface for realizing long-distance quantum communication and large-scale quantum computation. While many experimental schemes demonstrating high storage and retrieval efficiency have been performed with weak coherent light pulses, all quantum memories for true single photons achieved so far have efficiencies far below 50%, a threshold value for practical applications. Here, we report the demonstration of a quantum memory for single-photon polarization qubits with an efficiency of >85% and a fidelity of >99%, based on balanced two-channel electromagnetically induced transparency in laser-cooled rubidium atoms. For the single-channel quantum memory, the optimized efficiency for storing and retrieving single-photon temporal waveforms can be as high as 90.6%. This result pushes the photonic quantum memory closer to practical applications in quantum information processing.