Charge ordered kagome lattices have been demonstrated to be intriguing platforms for studying the intertwining of topology, correlation, and magnetism. The recently discovered charge ordered kagome material ScV 6 Sn 6 does not feature a magnetic groundstate or excitations, thus it is often regarded as a conventional paramagnet. Here, using advanced muon-spin rotation spectroscopy, we uncover an unexpected hidden magnetism of the charge order. We observe an enhancement of the internal field width sensed by the muon ensemble, which takes place within the charge ordered state. More importantly, the muon spin relaxation rate below the charge ordering temperature is substantially enhanced by applying an external magnetic field. Taken together with the hidden magnetism found in A V 3 Sb 5 ( A = K, Rb, Cs) and FeGe kagome systems, our results suggest ubiqitous time-reversal symmetry-breaking in charge ordered kagome lattices.
We study the temperature evolution of quasiparticles in the correlated metal Sr$_2$RuO$_4$. Our angle resolved photoemission data show that quasiparticles persist up to temperatures above 200~K, far beyond the Fermi liquid regime. Extracting the quasiparticle self-energy we demonstrate that the quasiparticle residue $Z$ increases with increasing temperature. Quasiparticles eventually disappear on approaching the bad metal state of Sr$_2$RuO$_4$ not by losing weight but via excessive broadening from super-Planckian scattering. We further show that the Fermi surface of Sr$_2$RuO$_4$ - defined as the loci where the spectral function peaks - deflates with increasing temperature. These findings are in semi-quantitative agreement with dynamical mean field theory calculations.
We study the temperature evolution of quasiparticles in the correlated metal Sr_{2}RuO_{4}. Our angle resolved photoemission data show that quasiparticles persist up to temperatures above 200 K, far beyond the Fermi liquid regime. Extracting the quasiparticle self-energy, we demonstrate that the quasiparticle residue Z increases with increasing temperature. Quasiparticles eventually disappear on approaching the bad metal state of Sr_{2}RuO_{4} not by losing weight but via excessive broadening from super-Planckian scattering. We further show that the Fermi surface of Sr_{2}RuO_{4}-defined as the loci where the spectral function peaks-deflates with increasing temperature. These findings are in semiquantitative agreement with dynamical mean field theory calculations.
The band structure in a kagome lattice can naturally exhibit flat band, Dirac cones, and van Hove singularity, enabling rich interplays between correlation and topology. However, the flat band is rarely detected just at the Fermi level in kagome materials, which would be crucial to realize emergent flat band physics. Here, combining angle-resolved photoemission spectroscopy, transport measurements and first-principles calculation, we observe a striking Fermi-level flat band in paramagnetic YCr6Ge6 as a typical signature of electronic kagome lattice. We explicitly unveil that orbital character plays an essential role to realize electronic kagome lattice in crystals with transition-metal kagome layers. We further engineer this material with magnetic rare earth elements to break the time-reversal symmetry of the Fermi-level kagome flat band. Our work establishes a Fermi-level flat band in a kagome magnet as an exciting quantum platform.
Weyl nodes can be classified into zero-dimensional (0D) Weyl points (WPs), 1D Weyl nodal lines (WNL) and 2D Weyl nodal surfaces (WNS), which possess finite Chern numbers. Up to date, the largest Chern number of WPs identified in Weyl semimetals is 4, which is thought to be a maximal value for linearly crossing points in solids. On the other hand, whether the Chern numbers of nonzero-dimensional linear crossing Weyl nodal objects have one upper limit is still an open question. In this work, combining angle-resolved photoemission spectroscopy with density functional theory calculations, we show that the chiral crystal AlPt hosts a cube-shaped charged Weyl nodal surface which is formed by the linear crossings of two singly-degenerate bands. Different to conventional Weyl nodes, the cube-shaped nodal surface in AlPt is enforced by nonsymmorphic chiral symmetries and time reversal symmetry rather than accidental band crossings, and it possesses a giant Chern number |C| = 26. Moreover, our results and analysis prove that there is no upper limit for the Chern numbers of such kind 2D Weyl nodal object.
X. Y. Zhu,1, ∗ H. Zhang,1, ∗ D. J. Gawryluk,2 Z. X. Zhen,1 B. C. Yu,1 S. L. Ju,3 W. Xie,4 D. M. Jiang,1 W. J. Cheng,1 Y. Xu,1 M. Shi,3 E. Pomjakushina,2 Q. F. Zhan,1 T. Shiroka,5, 6, † and T. Shang1, ‡ 1Key Laboratory of Polar Materials and Devices (MOE), School of Physics and Electronic Science, East China Normal University, Shanghai 200241, China 2Laboratory for Multiscale Materials Experiments, Paul Scherrer Institut, Villigen CH-5232, Switzerland 3Swiss Light Source, Paul Scherrer Institut, Villigen CH-5232, Switzerland 4DESY, Notkestraβe 85, D-22607 Hamburg, Germany 5Laboratory for Muon-Spin Spectroscopy, Paul Scherrer Institut, Villigen PSI, Switzerland 6Laboratorium für Festkörperphysik, ETH Zürich, CH-8093 Zürich, Switzerland (Dated: January 10, 2022)
Topological superconductivity is an exotic phase of matter in which the fully gapped superconducting bulk hosts gapless Majorana surface states protected by topology. Intercalation of copper, strontium or niobium between the quintuple layers of the topological insulator Bi$_2$Se$_3$ increases the carrier density and leads to superconductivity that is suggested to be topological. Here we study the electronic structure of strontium-intercalated Bi$_2$Se$_3$ using angle resolved photoemission spectroscopy (ARPES) and Shubnikov-de Haas (SdH) oscillations. Despite the apparent low Hall number of $\sim2 \times 10 ^{19}$cm$^{-3}$, we show that the Fermi surface is shaped as an open cylinder with a larger carrier density of $\sim 10 ^{20}$cm$^{-3}$. We suggest that superconductivity in intercalated Bi$_2$Se$_3$ emerges with the appearance of a quasi-2D open Fermi surface.
We report on systematic temperature- and magnetic field-dependent studies of the EuGa$_4$ binary compound, which crystallizes in a centrosymmetric tetragonal BaAl$_4$-type structure with space group $I4/mmm$. The electronic properties of EuGa$_4$ single crystals, with an antiferromagnetic (AFM) transition at $T_\mathrm{N} \sim 16.4$ K, were characterized via electrical resistivity and magnetization measurements. A giant nonsaturating magnetoresistance was observed at low temperatures, reaching $\sim 7 \times 10^4$ % at 2 K in a magnetic field of 9 T. In the AFM state, EuGa$_4$ undergoes a series of metamagnetic transitions in an applied magnetic field, clearly manifested in its field-dependent electrical resistivity. Below $T_\mathrm{N}$, in the $\sim$4-7 T field range, we observe also a clear hump-like anomaly in the Hall resistivity which is part of the anomalous Hall resistivity. We attribute such a hump-like feature to the topological Hall effect, usually occurring in noncentrosymmetric materials known to host topological spin textures (as e.g., magnetic skyrmions). Therefore, the family of materials with a tetragonal BaAl$_4$-type structure, to which EuGa$_4$ and EuAl$_4$ belong, seems to comprise suitable candidates on which one can study the interplay among correlated-electron phenomena (such as charge-density wave or exotic magnetism) with topological spin textures and topologically nontrivial bands.
As exemplified by the growing interest in the quantum anomalous Hall effect, the research on topology as an organizing principle of quantum matter is greatly enriched from the interplay with magnetism. In this vein, we present a combined electrical and thermoelectrical transport study on the magnetic Weyl semimetal EuCd_{2}As_{2}. Unconventional contribution to the anomalous Hall and anomalous Nernst effects were observed both above and below the magnetic transition temperature of EuCd_{2}As_{2}, indicating the existence of significant Berry curvature. EuCd_{2}As_{2} represents a rare case in which this unconventional transverse transport emerges both above and below the magnetic transition temperature in the same material. The transport properties evolve with temperature and field in the antiferromagnetic phase in a different manner than in the paramagnetic phase, suggesting different mechanisms to their origin. Our results indicate EuCd_{2}As_{2} is a fertile playground for investigating the interplay between magnetism and topology, and potentially a plethora of topologically nontrivial phases rooted in this interplay.
We report a comprehensive study of the centrosymmetric Re3B and noncentrosymmetric Re7B3 superconductors. At a macroscopic level, their bulk superconductivity (SC), with T-c = 5.1K (Re3B) and 3.3 K (Re7B3), was characterized via electrical-resistivity, magnetization, and heat-capacity measurements, while their microscopic superconducting properties were investigated by means of muon-spin rotation and relaxation (mu SR). In both Re3B and Re7B3 the low-T zero-field electronic specific heat and the superfluid density (determined via transverse-field mu SR) suggest a nodeless SC. Both compounds exhibit some features of multigap SC, as evidenced by the temperature-dependent upper critical fields Hc(2)(T), as well as by electronic band-structure calculations. The absence of spontaneous magnetic fields below the onset of SC, as determined from zero-field mu SR measurements, indicates a preserved time-reversal symmetry in the superconducting state of both Re3B and Re7B3. Our results suggest that a lack of inversion symmetry and the accompanying antisymmetric spin-orbit coupling effects are not essential for the occurrence of multigap SC in these rhenium-boron compounds.
Constrained by the Nielsen-Ninomiya no-go theorem, in all so-far experimentally determined Weyl semimetals (WSMs) the Weyl points (WPs) always appear in pairs in the momentum space with no exception. As a consequence, Fermi arcs occur on surfaces which connect the projections of the WPs with opposite chiral charges. However, this situation can be circumvented in the case of unpaired WP, without relevant surface Fermi arc connecting its surface projection, appearing singularly, while its Berry curvature field is absorbed by nontrivial charged nodal walls. Here, combining angle-resolved photoemission spectroscopy with density functional theory calculations, we show experimentally that a singular Weyl point emerges in PtGa at the center of the Brillouin zone (BZ), which is surrounded by closed Weyl nodal walls located at the BZ boundaries and there is no Fermi arc connecting its surface projection. Our results reveal that nontrivial band crossings of different dimensionalities can emerge concomitantly in condensed matter, while their coexistence ensures the net topological charge of different dimensional topological objects to be zero. Our observation extends the applicable range of the original Nielsen-Ninomiya no-go theorem which was derived from zero dimensional paired WPs with opposite chirality.
Based onee annihilation data samples collected with the BESIII detect or at the BEPCII collider at 13 center of mass energies from 4.008 to 4.600 GeV, measurements of the Bo rn cr ss section of ee → pp̄π are performed. No significant resonant structure is observed in the measure d en rgy-dependent cross section. The upper limit on the Born cross section of ee → Y (4260) → pp̄π at the 90% C.L. is determined to be 0.01 pb.
The second-order Fourier coefficients (v(2)) characterizing the azimuthal distributions of Y(1S) and Y(2S) mesons produced in PbPb collisions at root s(NN) = 5.02 TeV are studied. The Y mesons are reconstructed in their dimuon decay channel, as measured by the CMS detector. The collected data set corresponds to an integrated luminosity of 1.7 nb(-1). The scalar product method is used to extract the v2 coefficients of the azimuthal distributions. Results are reported for the rapidity range vertical bar y vertical bar < 2.4, in the transverse momentum interval 0 < pT < 50 GeV/c, and in three centrality ranges of 10-30%, 30-50% and 50-90%. In contrast to the J/psi mesons, the measured v(2) values for the Y mesons are found to be consistent with zero. (C) 2021 The Author(s). Published by Elsevier B.V.
Electronic band structures in solids stem from a periodic potential reflecting the structure of either the crystal lattice or electronic order. In the stoichiometric ruthenate Ca3Ru2O7, numerous Fermi surface-sensitive probes indicate a low-temperature electronic reconstruction. Yet, the causality and the reconstructed band structure remain unsolved. Here, we show by angle-resolved photoemission spectroscopy, how in Ca3Ru2O7 a C-2-symmetric massive Dirac semimetal is realized through a Brillouin-zone preserving electronic reconstruction. This Dirac semimetal emerges in a two-stage transition upon cooling. The Dirac point and band velocities are consistent with constraints set by quantum oscillation, thermodynamic, and transport experiments, suggesting that the complete Fermi surface is resolved. The reconstructed structure-incompatible with translational-symmetry-breaking density waves-serves as an important test for band structure calculations of correlated electron systems.
We report the observation of anomalous Hall resistivity in single crystals of EuAl4, a centrosymmetric tetragonal compound, which exhibits coexisting antiferromagnetic (AFM) and charge-density-wave (CDW) orders with onset at T-N similar to 15.6 K and T-CDW similar to 140 K, respectively. In the AFM state, when the magnetic field is applied along the c-axis direction, EuAl4 undergoes a series of metamagnetic transitions. Within this field range, we observe a clear humplike anomaly in the Hall resistivity, representing part of the anomalous Hall resistivity. By considering different scenarios, we conclude that such a humplike feature is most likely a manifestation of the topological Hall effect, normally occurring in noncentrosymmetric materials known to host nontrivial topological spin textures. In view of this, EuAl4 would represent a rare case where the topological Hall effect not only arises in a centrosymmetric structure, but it also coexists with CDW order.
Several decades after the discovery of superconductivity in bismuthates, the strength of their electron-phonon coupling and its evolution with doping remain puzzling. To clarify these issues, polycrystalline hole-doped Ba1-xKxBiO3 (0.1 <= x <= 0.6) samples were systematically synthesized and their bulk and microscopic superconducting properties were investigated by means of magnetic susceptibility and muon-spin rotation and relaxation (mu SR), respectively. The phase diagram of Ba1-xKxBiO3 was reliably extended up to x = 0.6, which is still found to be a bulk superconductor. The lattice parameter a increases linearly with K content, implying a homogeneous chemical doping. The low-temperature superfluid density, measured via transverse-field mu,SR, indicates an isotropic fully gapped superconducting state with zero-temperature gaps Delta(0)/k(B)T(c) = 2.15, 2.10, and 1.75, and magnetic penetration depths lambda(0), = 219, 184, and 279 nm for x = 0.3, 0.4, and 0.6, respectively. A change in the superconducting gap, from a nearly ideal BCS value (1.76k(B)T(c) in the weak-coupling case) in the overdoped x = 0.6 region, to much higher values in the optimally doped case, implies a gradual decrease in electron-phonon coupling with doping.
In the context of correlated insulators, where electron–electron interactions (U) drive the localization of charge carriers, the metal–insulator transition is described as either bandwidth- or filling-controlled1. Motivated by the challenge of the insulating phase in Sr2IrO4, a new class of correlated insulators has been proposed, in which spin–orbit coupling (SOC) is believed to renormalize the bandwidth of the half-filled jeff = 1/2 doublet, allowing a modest U to induce a charge-localized phase2,3. Although this framework has been tacitly assumed, a thorough characterization of the ground state has been elusive4,5. Furthermore, direct evidence for the role of SOC in stabilizing the insulating state has not been established, because previous attempts at revealing the role of SOC6,7 have been hindered by concurrently occurring changes to the filling8–10. We overcome this challenge by employing multiple substituents that introduce well-defined changes to the signatures of SOC and carrier concentration in the electronic structure, as well as a new methodology that allows us to monitor SOC directly. Specifically, we study Sr2Ir1−xTxO4 (T = Ru, Rh) by angle-resolved photoemission spectroscopy, combined with ab initio and supercell tight-binding calculations. This allows us to distinguish relativistic and filling effects, thereby establishing conclusively the central role of SOC in stabilizing the insulating state of Sr2IrO4. Most importantly, we estimate the critical value for SOC in this system to be λc = 0.42 ± 0.01 eV, and provide the first demonstration of a spin–orbit-controlled metal–insulator transition. A combined ARPES and DFT study of Ru- and Rh-substituted samples of Sr2IrO4 reveals a collapse of its correlated insulating phase that is controlled by spin–orbit coupling.
We report angle-resolved photoemission spectroscopy and first-principles numerical calculations for the band-structure evolution of the 3d heavy-fermion compound CaCu3Ru4O12. Below T similar to 200 K, we observed an emergent hybridization gap between the Cu 3d-electron-like band and the Ru 4d-hole-like band and the resulting flat band features near the Fermi level centered around the Brillouin-zone corner. Our results confirm the non-Kondo nature of the CaCu3Ru4O12, in which the Cu3d(xy) electrons are less correlated and not in the Kondo limit. Comparison between theory and experiment also suggests that other mechanisms may be needed to give a full quantitative explanation of the peculiar properties in this material.
A measurement is presented of electroweak (EW) production of a W boson in association with two jets in proton-proton collisions at s = 13 Te . The data sample was recorded by the CMS Collaboration at the LHC and corresponds to an integrated luminosity of 35.9 fb - 1 . The measurement is performed for the l ν jj final state (with l ν indicating a lepton-neutrino pair, and j representing the quarks produced in the hard interaction) in a kinematic region defined by invariant mass m jj \u003e 120 Ge and transverse momenta p T j \u003e 25 Ge . The cross section of the process is measured in the electron and muon channels yielding σ EW ( W jj ) = 6.23 ± 0.12 (stat) ± 0.61 (syst) pb per channel, in agreement with leading-order standard model predictions. The additional hadronic activity of events in a signal-enriched region is studied, and the measurements are compared with predictions. The final state is also used to perform a search for anomalous trilinear gauge couplings. Limits on anomalous trilinear gauge couplings associated with dimension-six operators are given in the framework of an effective field theory. The corresponding 95% confidence level intervals are - 2.3 c W W W / Λ 2 2.5 Te - 2 , - 8.8 c W / Λ 2 16 Te - 2 , and - 45 c B / Λ 2 46 Te - 2 . These results are combined with the CMS EW Zjj analysis, yielding the constraint on the c W W W coupling: - 1.8 c W W W / Λ 2 2.0 Te - 2 .