The neutron richness of the light charged particles emitted out of the fission plane in heavy ion reactions has been experimentally investigated via the production of A=3 mirror nuclei in ^86 Kr + ^nat Pb reactions at 25 MeV/u. The energy spectra and angular distributions of triton (t) and ^3 He in coincidence with two fission fragments are measured with the Compact Spectrometer for Heavy IoN Experiment (CSHINE). The energy spectrum of ^3 He is observed harder than that of triton in the fission events, in accordance with the phenomena reported as “ ^3 He-puzzle” in inclusive measurements. With a data-driven energy spectrum peak cut scenario, it is observed that the yield ratio R(t/^3He) increases with the angle to the fission plane, showing an enhancement of neutron-rich particle emission from out-of-fission-plane. A qualitative comparison with the transport model calculations suggests that this observation may serve as a new probe for the nuclear symmetry energy.
A rapidly converging 4-dimensional Fourier shape parametrization is used to model the fission process of heavy nuclei. Potential energy landscapes are computed within the macroscopic-microscopic approach, on top of which the multi-dimensional Langevin equation is solved to describe the fission dynamics. Charge equilibration at scission and de-excitation by neutron evaporation of the primary fragments after scission is investigated. The model describes various observables, including fission-fragment mass, charge, and kinetic energy yields, as well as post-scission neutron multiplicities and, most importantly, their correlations, which are crucial to unravel the complexity of the fission process. The parameters of the dynamical model were tuned to reproduce experimental data obtained from thermal neutron-induced fission of $^{235}$U, which allows us to discuss the transition from asymmetric to symmetric fission along the Fm isotopic chain.
The neutron rich neck zone created in heavy ion reaction is experimentally probed by the production of the $A=3$ isobars. The energy spectra and angular distributions of triton and $^3$He are measured with the CSHINE detector in $^{86}$Kr +$^{208}$Pb reactions at 25 MeV/u. While the energy spectrum of $^{3}$He is harder than that of triton, known as "$^{3}$He-puzzle", the yield ratio $R({\rm t/^3He})$ presents a robust rising trend with the polar angle in laboratory. Using the fission fragments to reconstruct the fission plane, the enhancement of out-plane $R({\rm t/^3He})$ is confirmed in comparison to the in-plane ratios. Transport model simulations reproduce qualitatively the experimental trends, but the quantitative agreement is not achieved. The results demonstrate that a neutron rich neck zone is formed in the reactions. Further studies are called for to understand the clustering and the isospin dynamics related to neck formation.
Two-body correlations of the isotope-resolved light and heavy clusters are measured in $^{86}$Kr+$^{\rm 208}$Pb reactions at 25 MeV/u. The yield and kinetic variables of the $A=3$ isobars, triton and $^3$He, are analyzed in coincidence with the heavy clusters of $7\le A \le 14$ emitted at the earlier chance. While the velocity spectra of both triton and $^3$He exhibit scaling behavior over the type of the heavy clusters, the yield ratios of ${\rm t/^3He}$ correlate reversely to the neutron-to-proton ratio $N/Z$ of the latter, showing the ping-pong modality of the $N/Z$ of emitted clusters. The commonality that the $N/Z$ of the residues keeps the initial system value is extended to the cluster emission in heavy ion reactions. The comparison of transport model calculations to the data is discussed.
Potential energy surfaces of even-even superheavy nuclei are evaluated within the macroscopic-microscopic approximation. A very rapidly converging analytical Fourier-type shape parametrization is used to describe nuclear shapes throughout the periodic table, including those of fissioning nuclei. The Lublin Strasbourg Drop and another effective liquid-drop type mass formula are used to determine the macroscopic part of nuclear energy. The Yukawa-folded single-particle potential, the Strutinsky shell-correction method, and the BCS approximation for including pairing correlations are used to obtain microscopic energy corrections. The evaluated nuclear binding energies, fission-barrier heights, and Q-alpha energies show a relatively good agreement with the experimental data. A simple one-dimensional WKB model a la Swiatecki is used to estimate spontaneous fission lifetimes, while alpha-decay probabilities are obtained within a Gamow-type model.
The calculations of the potential energy surface are essential in the theoretical description of the fission process. In the constrained self-consistent approach, the smooth evolution of nuclear shape is described from the ground state until a very elongated one with a narrow neck. In all microscopic calculations, the rupture of the neck at scission is associated with a substantial change of nuclear matter density distribution and rapid energy decrease. In this paper, we show that there is no discontinuity of the potential energy surface at scission when multi-constrained calculations are applied with the neck constraint. An early rupture of the neck at lower quadrupole and octupole moments is discussed as competitive with the conventional fission path. We discuss the neck properties in the scission configuration. We find that the neck radius in the asymmetric fission mode cannot decrease below 2 fm, and the nuclear matter density cannot decrease below the saturation density. In the compact fission mode, nuclear density may go down to half of the saturation density before the rupture of the neck.
Fission properties of the actinide nuclei are deduced from theoretical analysis. We investigate potential energy surfaces and fission barriers and predict the fission fragment mass yields of actinide isotopes. The results are compared with experimental data where available. The calculations were performed in the macroscopic-microscopic approximation with the Lublin-Strasbourg Drop (LSD) for the macroscopic part, and the microscopic energy corrections were evaluated in the Yukawa-folded potential. The Fourier nuclear shape parametrization is used to describe the nuclear shape, including the non-axial degree of freedom. The fission fragment mass yields of the nuclei considered are evaluated within a 3D collective model using the Born-Oppenheimer approximation.
The microscopic studies on nuclear fission require the evaluation of the potential energy surface as a function of the collective coordinates. A reasonable choice of constraints on multipole moments should be made to describe the topography of the surface completely within a reasonable amount of computing time. We present a detailed analysis of fission barriers in the self-consistent Hartree-Fock-Bogoliubov approach with the D1S parametrization of the Gogny nucleon-nucleon interaction. Two heavy isotopes representing different spontaneous fission modes - $^{252}$Cf (asymmetric) and $^{258}$No (bimodal) - have been chosen for the analysis. We have shown the existence of complicated structures on the energy surface that can not be fully described in two-dimensional calculations. We analyze apparent problems that can be encountered in this type of calculations: multiple solutions for given constraints and transitions between various potential energy surfaces. We present possible solutions on how to deal with these issues.
Potential energy surfaces and fission barriers of superheavy nuclei are analyzed in a macroscopic-microscopic model. The Lublin-Strasbourg Drop (LSD) model is used to obtain the macroscopic part of the energy, whereas the shell and pairing energy corrections are evaluated using the Yukawa-folded potential; a standard flooding technique is utilized to determine barrier heights. A Fourier shape parametrization containing only three deformation parameters is shown to effectively reproduce the nuclear shapes of nuclei approaching fission. In addition, a non-axial degree of freedom is taken into account to better describe the structure of nuclei around the ground state and in the saddle region. In addition to the symmetric fission valley, a new highly asymmetric fission mode is predicted in most superheavy nuclei. The fission fragment mass distributions of the considered nuclei are obtained by solving 3D Langevin equations.
An effective Fourier nuclear shape parametrization, which describes well the most relevant degrees of freedom on the way to fission is used to construct a three-dimensional collective model. The potential energy surface is evaluated within the macroscopic-microscopic approach based on the Lublin-Strasbourg drop macroscopic energy and Yukawa-folded single-particle potential. A phenomenological inertia parameter is used to describe the kinetic properties of the fissioning system. The fission fragment mass yields are obtained by using an approximate solution of the underlying Hamiltonian. The predicted mass fragmentations for even-even Pt to Ra isotopes are compared with available experimental data. Their main characteristics are well reproduced when the neck rupture probability dependent on the neck radius is introduced.
There has been much recent interest in nuclear fission, due in part to a new appreciation of its relevance to astrophysics, stability of superheavy elements, and fundamental theory of neutrino interactions. At the same time, there have been important developments on a conceptual and computational level for the theory. The promising new theoretical avenues were the subject of a workshop held at the University of York in October 2019; this report summarises its findings and recommendations.
Fragment mass distributions from fission of the excited compound nucleus 178Pt have been deduced from the measured fragment velocities. The 178Pt nucleus was created at the JAEA tandem facility in a complete fusion reaction 36Ar + 142Nd, at beam energies of 155, 170 and 180 MeV. The data are indicative of a mixture of the mass-asymmetric and mass-symmetric fission modes associated with higher and lower total kinetic energies of the fragments, respectively. The measured fragment yields are dominated by asymmetric mass splits, with the symmetric mode contributing at the level of ≈1/3. This constitutes the first observation of a multimodal fission in the sub-lead region. Most probable experimental fragment-mass split of the asymmetric mode, AL/AH≈79/99, is well reproduced by nuclear density functional theory using the UNEDF1-HFB and D1S potentials. The symmetric mode is associated by theory with very elongated fission fragments, which is consistent with the observed total kinetic energy/fragment mass correlation.
Cluster radioactivity is an exotic nuclear decay observed in actinides where a light nucleus is emitted while the remaining heavy mass residue is the doubly magic $^{208}$Pb or a nucleus in its neighborhood. We have investigated this type of decay in heavier nuclei up to Lv $(Z=116)$ within a microscopic theory. It has been found that super asymmetric fission with $^{208}$Pb as heavy fragment may be dominant decay channel in some super heavy nuclei. This reaction is closely related with cluster radioactivity.
A simple WKB model, able to describe the emission of protons, α-particles and nuclear clusters as well as the spontaneous fission process, is presented. Potential energy surfaces of fissioning nuclei are determined within the macroscopic-microscopic model, using a new Fourier-type shape parametrisation and fission-fragment mass distributions are calculated.
The time-dependent generator coordinate method with the gaussian overlap approximation (TDGCM+GOA) formalism is applied to describe the fission of $^{252}$Cf. We perform analysis of fission from the initial states laying in the energetic range from the ground state to the state located 4 MeV above the fission barrier. The fission fragment mass distributions, obtained for different parity, energy of levels and types of mixed states, are calculated and compared with experimental data. The impact of the total time of wave packet propagation on the final results is studied as well. The weak dependence of obtained mass yields on the initial conditions is shown.
Proton emission is described using a model which has previously given good results in the description of \(\alpha\) and cluster radioactivity. The simple phenomenological formalism, based on the Gamow theory for alpha decay, is now extended by including the centrifugal term. The model contains only one parameter: the effective nuclear radius constant. Its value was once found for alpha and cluster emitters. A good agreement with the experimental half-lives for proton radioactivity is achieved without any additional fitting procedures to the data for proton emission.
Fragment mass distribution is one of the major, measurable characteristics of fission. The shape of the observed yield allows to determine type of fission and-indirectly-to investigate structure of the mother nucleus. It has been proven, that basic properties of nascent fragments are preliminary determined by the configuration of pre-scission point. We assume, that the shape of a nucleus obtained in its prescission point provides information about the possible fragment mass asymmetry.
A simple phenomenological formula, based on the Swiatecki idea for the evaluation of the spontaneous fission half-lives, is proposed. The model contains only one adjustable parameter fixed to the data for even-even nuclei and an additional hindrance factor for odd nuclei, which gives the effect of an odd particle. A good agreement with the experimental data for isotopes with 90 <= Z <= 103 is achieved.