In gases adsorbed on smooth surfaces, the binding energy E 1 of the lowest quantum state (first layer) is usually much lower than that of the excited state (second layer), E 2 . The typical energy difference for helium on graphite amounts to about 50 K which gives a vanishingly small Boltzmann factor e -(E 2 -E 1 )/k B T at temperatures below 1 K, and no atom should be present on the excited level (second layer), according to statistical physics. However, in our investigations on sub-monolayer of 3 He adsorbed on a carbon nanotube, we have detected helium atoms traveling freely along the tube. Free particles were shown to be responsible for quantized satellite peaks appearing in mechanical oscillation spectra next to the main resonance. We demonstrate that side peaks reflect transitions between different longitudinal quantum states of free helium atoms on the oscillating tube. Radial quantum fluctuations in AC electric field have been considered in the framework of Rabi oscillations and shown to lift some amount of particles above the dense first layer. Besides, zero-point pressure at moderate densities promotes radial fluctuations significantly.
Low-noise amplifiers are of great significance in the field of quantum technologies. We study a thermally driven parametric amplifier based on a superconductor-insulator-graphene-insulator-superconductor (S-I-G-I-S) junction coupled to a superconducting microwave cavity. The strong nonlinearity in the temperature dependence of our device leads to thermal self-modulation that produces impedance oscillations at frequencies around twice the angular cavity resonance frequency omega r. In particular, reactance modulation of the effective capacitance yields a gain of 18.6 dB over a frequency span of 125 kHz with a minimum noise temperature of TN = 1.4 K. Our theoretical modeling gives insight into the exact mixing processes, confirmation of the electron-phonon coupling parameter and possible improvements of the studied system.
From the background of microwave-optomechanical experiments involving carbon nanotubes, the optimization of superconducting coplanar waveguide resonator devices is discussed. Two devices, one with unmodified geometry compared to previous work and one integrating several improvements, are lithographically built up step-by-step. After each step, the low-temperature GHz transmission properties are retested. This allows to identify the impact of the fabrication and the geometry modification on the device properties. In addition, simplified circuit geometries are modeled numerically, confirming the experimental results and providing further insights for optimization.
Low dimensional fermionic quantum systems are exceptionally interesting because they reveal distinctive physical phenomena, including among others, topologically protected excitations, edge states, frustration, and fractionalization. Our aim was to confine 3 He on a suspended carbon nanotube to form 2-dimensional Fermi-system. Here we report our measurements of the mechanical resonance of the nanotube with adsorbed sub-monolayer down to 10 mK. At intermediate coverages we have observed the famous 1/3 commensurate solid. However, at larger monolayer densities we have observed a quantum phase transition from 1/3 solid to an unknown, soft, and mobile solid phase. We interpret this mobile solid phase as a bosonic commensurate crystal consisting of helium dimers with topologically-induced zero-point vacancies which are delocalized at low temperatures. We thus demonstrate that 3 He on a nanotube merges both fermionic and bosonic phenomena, with a quantum phase transition between fermionic solid 1/3 phase and the observed bosonic dimer solid.
Nonlinear phenomena in superconducting resonator circuits are of great significance in the field of quantum technology. We observe thermal self-oscillations in a monolayer graphene flake coupled to Molybdenum-Rhenium superconducting resonator. The graphene flake forms a SINIS junction coupled to the resonator with strong temperature dependent resistance. In certain conditions of pump power and frequency, this nonlinearity leads to thermal self-oscillations appearing as sidebands in cavity transmission measurements with strong temperature dependence and gate tunability. The experimental observations fit well with theoretical model based on thermal instability. The modelling of the oscillation sidebands provides a method to evaluate electron phonon coupling in disordered graphene sample at low energies.
Entangled microwave photons form a fundamental resource for quantum information processing and sensing with continuous variables. We use a low-loss Josephson metamaterial comprising superconducting, non-linear, asymmetric inductive elements to generate frequency-entangled photons from vacuum fluctuations at a rate of 2 giga entangled bits per second spanning over 4 GHz bandwidth. The device is operated as a traveling wave parametric amplifier under Kerr-relieving biasing conditions. Furthermore, we realize the first successfully demonstration of single-mode squeezing in such devices -- $3.1\pm0.7$\,dB below the zero-point level at half of modulation frequency.
Experimental dataset for article “Electrical Low-Frequency 1/fγ Noise Due to Surface Diffusion of Scatterers on an Ultra-low-Noise Graphene Platform”, Nano letters, 21(18), 7637-7643 (2021), doi: 10.1021/acs.nanolett.1c02325
Low-frequency 1/f γ noise is ubiquitous, even in high-end electronic devices. Recently, it was found that adsorbed O2 molecules provide the dominant contribution to flux noise in superconducting quantum interference devices. To clarify the basic principles of such adsorbate noise, we have investigated low-frequency noise, while the mobility of surface adsorbates is varied by temperature. We measured low-frequency current noise in suspended monolayer graphene Corbino samples under the influence of adsorbed Ne atoms. Owing to the extremely small intrinsic noise of suspended graphene, we could resolve a combination of 1/f γ and Lorentzian noise induced by the presence of Ne. We find that the 1/f γ noise is caused by surface diffusion of Ne atoms and by temporary formation of few-Ne-atom clusters. Our results support the idea that clustering dynamics of defects is relevant for understanding of 1/f noise in metallic systems.
Abstract We have studied 1/f noise in critical current $$I_c$$ I c in h-BN encapsulated monolayer graphene contacted by NbTiN electrodes. The sample is close to diffusive limit and the switching supercurrent with hysteresis at Dirac point amounts to $$\simeq 5$$ ≃ 5 nA. The low frequency noise in the superconducting state is measured by tracking the variation in magnitude and phase of a reflection carrier signal $$v_{rf}$$ v rf at 600–650 MHz. We find 1/f critical current fluctuations on the order of $$\delta I_c/I_c \simeq 10^{-3}$$ δ I c / I c ≃ 10 - 3 per unit band at 1 Hz. The noise power spectrum of critical current fluctuations $$S_{I_c}$$ S I c measured near the Dirac point at large, sub-critical rf-carrier amplitudes obeys the law $$S_{I_c}/{I{_c}}^2 = a/f^{\beta }$$ S I c / I c 2 = a / f β where $$a\simeq 4\times 10^{-6}$$ a ≃ 4 × 10 - 6 and $$\beta \simeq 1$$ β ≃ 1 at $$f > 0.1$$ f > 0.1 Hz. Our results point towards significant fluctuations in $$I_c$$ I c originating from variation of the proximity induced gap in the graphene junction.
M. R. Perelshtein, K. V. Petrovnin, V. Vesterinen, S. Hamedani Raja, I. Lilja, M. Will, A. Savin, S. Simbierowicz, ∗ R. N. Jabdaraghi, J. S. Lehtinen, L. Grönberg, J. Hassel, † M. P. Prunnila, J. Govenius, G. S. Paraoanu, and P. J. Hakonen ‡ QTF Centre of Excellence, Department of Applied Physics, Aalto University, P.O. Box 15100, FI-00076 AALTO, Finland QTF Centre of Excellence, VTT Technical Research Centre of Finland Ltd, P.O. Box 1000, FI-02044 VTT, Finland
Low dimensional fermionic quantum systems are exceptionally interesting because they reveal distinctive physical phenomena, including among others, topologically protected excitations, edge states, frustration, and fractionalization. Two-dimensional ^3He has indeed shown a remarkable variety of phases including the unusual quantum spin liquid. Our aim was to lower the dimension of the ^3He system even more by confining it on a suspended carbon nanotube. In our measurements the mechanical resonance of the nanotube with adsorbed sub-monolayer of ^3He was measured as a function of coverage and temperature down to 10 mK. At lowest temperatures and low coverages we have observed a liquid-gas coexistence which transforms to the famous 1/3 commensurate solid phase at intermediate densities. However, at larger monolayer densities we have observed a quantum phase transition from 1/3 solid to a completely new, soft and mobile solid phase. We interpret this mobile solid phase as a bosonic commensurate crystal consisting of helium dimers with topologically protected zero-point vacancies which are delocalized at low temperatures. We thus demonstrate that ^3He on a nanotube merges both fermionic and bosonic phenomena, with a quantum phase transition between fermionic solid 1/3 phase and a newly observed bosonic dimer solid. The mobility and softness of the bosonic dimer solid are conditioned by topology-induced vacancies which become delocalized at low temperatures owing to a large zero-point motion.
Ultralight mechanical resonators based on low-dimensional materials are well suited as exceptional transducers of minuscule forces or mass changes. However, the low dimensionality also provides a challenge to minimize resistive losses and heating. Here, we report on a novel approach that aims to combine different two-dimensional (2D) materials to tackle this challenge. We fabricated a heterostructure mechanical resonator consisting of few layers of niobium diselenide (NbSe2) encapsulated by two graphene sheets. The hybrid membrane shows high quality factors up to 245,000 at low temperatures, comparable to the best few-layer graphene mechanical resonators. In contrast to few-layer graphene resonators, the device shows reduced electrical losses attributed to the lower resistivity of the NbSe2 layer. The peculiar low-temperature dependence of the intrinsic quality factor points to dissipation over two-level systems which in turn relax over the electronic system. Our high sensitivity readout is enabled by coupling the membrane to a superconducting cavity which allows for the integration of the hybrid mechanical resonator as a sensitive and low loss transducer in future quantum circuits.