We address the challenge of certifying quantum behavior with single macroscopic massive particles, subject to decoherence and finite data. We propose a hypothesis-testing framework that distinguishes between classical and quantum mechanics based on position measurements. While interference pattern visibility in single-particle quantum superposition experiments has been commonly used as a sufficient criterion to falsify classical mechanics, we show that, from a hypothesis-testing perspective, it is neither necessary nor efficient. Focusing on recent proposals to prepare macroscopic superposition states of levitated nanoparticles, we show that the likelihood ratio test—which leverages differences across the entire probability distribution—provides an exponential reduction in measurements needed to reach a given confidence level. These results generalize to a broad class of quantum states, and offer a principled, efficient method to falsify classical mechanics in interference experiments, relaxing the experimental constraints faced by current efforts to test quantum mechanics at the macroscopic scale.

Levitated high-mass quantum systems provide access to unprecedented regimes in both fundamental science and technological applications. However, deterministic generation and manipulation of quantum non-Gaussian states, which are central to many continuous-variable quantum advantages, remain elusive in such platforms. In this work, we propose a theoretical protocol for preparing a continuous-variable degree of freedom of a levitated massive object in a variety of quantum states, including Fock and Schrödinger cat states, without coupling to auxiliary two-level systems. Our approach enhances otherwise weak nonharmonic effects by transient wave-function delocalization and combines this with optimal control of the potential. Specifically, time-dependent modulation of the linear component of the potential, in the presence of a static cubic nonharmonicity, provides a route to universal control of the mode. We analyze quantum state preparation under such control and estimate the required nonharmonicity, motional delocalization, and maximum tolerable decoherence for generating target non-Gaussian states. The proposed optimal-control scheme can also be readily extended beyond single-particle state preparation, for example, to unitary transformations and nonlinear measurements. As a concrete example, we demonstrate mechanical Bell-state preparation for two interacting particles using only local modulation of weakly nonharmonic potentials, while the interparticle interaction remains effectively linear. We emphasize that the protocols presented here apply to different mechanical degrees of freedom, such as center-of-mass motion and libration, and can also be implemented in other weakly nonharmonic systems with a leading cubic nonharmonicity.

While the wave packet of a massive particle grows linearly under free dynamics, it grows exponentially in an inverted harmonic potential, offering a pathway to rapidly increase quantum fluctuations to macroscopic dimensions. In this work, we experimentally demonstrate this principle by expanding the center-of-mass thermal state of a 125nm silica nanoparticle to a position uncertainty of 43.4nm within 260µs. This expansion, achieved using an inverted dark potential to minimize decoherence from photon recoil, represents a 952-fold increase, reaching a scale comparable to the nanoparticle's physical size. This work represents a key advancement toward preparing macroscopic quantum superpositions at unprecedented mass and length scales.

Subwavelength atomic arrays feature strong light-induced dipole-dipole interactions, resulting in subradiant collective resonances characterized by narrowed linewidths. In this work, we present a sideband cooling scheme for atoms trapped in subwavelength arrays that utilizes these narrow collective resonances. Working in the Lamb-Dicke regime, we derive an effective master equation for the atomic motion by adiabatically eliminating the internal degrees of freedom of the atoms, and validate its prediction with numerical simulations of the full system. Our results demonstrate that subradiant resonances enable the cooling of ensembles of atoms to temperatures lower than those achievable without dipole interactions, provided the atoms have different trap frequencies. Remarkably, narrow collective resonances can be sideband-resolved even when the individual atomic transition is not. In such scenarios, ground-state cooling becomes feasible solely due to light-induced dipole-dipole interactions. This approach could be utilized for future quantum technologies based on dense ensembles of emitters, and paves the way towards harnessing many-body cooperative decay for enhanced motional control.

Every massive particle behaves like a wave, according to quantum physics. Yet, this characteristic wave nature has only been observed in double-slit experiments with microscopic systems, such as atoms and molecules. The key aspect is that the wavefunction describing the motion of these systems extends coherently over a distance comparable to the slit separation, much larger than the size of the system itself. Preparing these states of more massive and complex objects remains an outstanding challenge. While the motion of solid-state oscillators can now be controlled at the level of single quanta, their coherence length remains comparable to the zero-point motion, limited to subatomic distances. Here, we prepare a delocalized state of a levitating solid-state nanosphere with coherence length exceeding the zero-point motion. We first cool its motion to the ground state. Then, by modulating the stiffness of the confinement potential, we achieve more than a threefold increment of the initial coherence length with minimal added noise. Optical levitation gives us the necessary control over the confinement that other mechanical platforms lack. Our work is a stepping stone towards the generation of delocalization scales comparable to the object size, a crucial regime for macroscopic quantum experiments, and towards quantum-enhanced force sensing with levitated particles.

The observation of quantum phenomena often necessitates sufficiently pure states, a requirement that can be challenging to achieve. In this study, our goal is to prepare a nonclassical state originating from a mixed state, using dynamics that preserve the initial low purity of the state. We generate a quantum superposition of displaced thermal states within a microwave cavity using only unitary interactions with a transmon qubit. We measure the Wigner functions of these “hot” Schrödinger cat states for an initial purity as low as 0.06. This corresponds to a cavity mode temperature of up to 1.8 kelvin, 60 times hotter than the cavity’s physical environment. Our realization of highly mixed quantum superposition states could be implemented with other continuous-variable systems, e.g., nanomechanical oscillators, for which ground-state cooling remains challenging.

Waveguide quantum electrodynamics—the study of atomic systems interacting with propagating electromagnetic fields—is a powerful platform for understanding the complex interplay between light and matter. Qubit control is an indispensable tool in this field, and most experiments thus far have used narrowband control pulses to interact with qubits at specific frequencies. Dynamics can change significantly with fast, broadband pulses, since waveguide properties such as dispersion affect the pulse evolution and its impact on the qubit. Here we use dispersion to achieve spatial addressing of superconducting qubits separated by a subwavelength distance within a microwave waveguide. This approach relies on a self-focusing effect to create a position-dependent interaction between a chirped pulse and an individual qubit. This method emphasizes the importance of dispersion in the design and analysis of quantum experiments, and offers avenues for the rapid control of quantum states.

Exploiting quantum effects in a mechanical oscillator, such as back-action-evading measurements or squeezing of the mechanical degrees of freedom, requires the oscillator to be prepared in a high-purity quantum state. The largest state purities in optomechanics to date have been achieved with costly cryogenic cooling combined with coupling to electromagnetic resonators driven with a coherent radiation field. Here we use coherent scattering into a Fabry-Pérot cavity to cool the megahertz-frequency librational mode of an optically levitated silica nanoparticle from room temperature to its quantum ground state. We use sideband thermometry to infer a phonon population of 0.04 quanta under optimal conditions, corresponding to a state purity of 92%. The purity reached by our room-temperature experiment exceeds the performance offered by mechanically clamped oscillators in a cryogenic environment, establishing a platform for high-purity quantum optomechanics at room temperature.

We present a theoretical proposal for preparing and manipulating a state of a single continuous-variable degree of freedom confined to a nonharmonic potential. By utilizing optimally controlled modulation of the potential's position and depth, we demonstrate the generation of non-Gaussian states, including Fock, Gottesman-Kitaev-Preskill, multi-legged-cat, and cubic-phase states, as well as the implementation of arbitrary unitaries within a selected two-level subspace. Additionally, we propose protocols for single-shot orthogonal state discrimination, algorithmic cooling, and correcting for nonlinear evolution. We analyze the robustness of this control scheme against noise. Since all the presented protocols rely solely on the precise modulation of the effective nonharmonic potential landscape, they are relevant to several experiments with continuous-variable systems, including the motion of a single particle in an optical tweezer or lattice, or current in circuit quantum electrodynamics.

The ability to engineer cavity-mediated interactions has emerged as a powerful tool for the generation of non-local correlations and the investigation of non-equilibrium phenomena in many-body systems. Levitated optomechanical systems have recently entered the multiparticle regime, which promises the use of arrays of strongly coupled massive oscillators to explore complex interacting systems and sensing. Here we demonstrate programmable cavity-mediated interactions between nanoparticles in vacuum by combining advances in multiparticle optical levitation and cavity-based quantum control. The interaction is mediated by photons scattered by spatially separated particles in a cavity, resulting in strong coupling that is long-range in nature. We investigate the scaling of the interaction strength with cavity detuning and interparticle separation and demonstrate the tunability of interactions between different mechanical modes. Our work will enable the exploration of many-body effects in nanoparticle arrays with programmable cavity-mediated interactions, generating entanglement of motion, and the use of interacting particle arrays for optomechanical sensing.

We introduce a numerical method to simulate nonlinear open quantum dynamics of a particle in situations where its state undergoes significant expansion in phase space while generating small quantum features at the phase-space Planck scale. Our approach involves simulating the Wigner function in a time-dependent frame that leverages information from the classical trajectory to efficiently represent the quantum state in phase space. To demonstrate the capabilities of our method, we examine the open quantum dynamics of a particle evolving in a one-dimensional weak quartic potential after initially being ground-state cooled in a tight harmonic potential. This numerical approach is particularly relevant to ongoing efforts to design, optimize, and understand experiments targeting the preparation of macroscopic quantum superposition states of massive particles through nonlinear quantum dynamics.

We introduce and theoretically analyze a scheme to prepare and detect non-Gaussian quantum states of an optically levitated particle via the interaction with light pulses that generate cubic and inverted potentials. We show that this approach allows to operate on sufficiently short time- and length scales to beat decoherence in a regime accessible in state-of-the-art experiments. Specifically, we predict the observation of single-particle interference of a nanoparticle with a mass above 108 atomic mass units delocalized by several nanometers, on timescales of milliseconds. The proposed experiment uses only optical and electrostatic control, and can be performed at about 10-10 mbar and at room temperature. We discuss the prospect of this method for coherently splitting the wavepacket of massive dielectric objects without using either projective measurements or an internal level structure.

Received 12 December 2023DOI:https://doi.org/10.1103/PhysRevA.109.019901©2024 American Physical SocietyPhysics Subject Headings (PhySH)Research AreasCooling & trappingDielectric propertiesMicroparticlesOptical forcesOptomechanicsQuantum opticsAtomic, Molecular & OpticalQuantum Information, Science & TechnologyCondensed Matter, Materials & Applied Physics

Levitated nanoparticles provide a controllable and isolated platform for probing fundamental quantum phenomena at the macroscopic scale. In this work, we introduce an optimization method to determine optimal static potentials for the generation of largely delocalized and non-Gaussian quantum states of levitated nanoparticles. Our optimization strategy accounts for position-dependent noise sources originating from the fluctuations of the potential. We provide key figures of merit that allow for fast computation and capture relevant features of the dynamics, mitigating the computational demands associated with the multiscale simulation of this system. Specifically, we introduce coherence length and coherent cubicity as signatures of large delocalization and quantum non-Gaussian states, respectively. We apply the optimization approach to a family of quartic potentials and show that the optimal configuration depends on the strength and nature of the noise in the system. Additionally, we benchmark our results with the full quantum dynamics simulations of the system for the optimal potentials.

We spatially expand and subsequently contract the motional thermal state of a levitated nanoparticle using a hybrid trapping scheme. The particle 's center-of-mass motion is initialized in a thermal state (temperature 155 mK) in an optical trap and then expanded by subsequent evolution in a much softer Paul trap in the absence of optical fields. We demonstrate expansion of the motional state 's standard deviation in position by a factor of 24. In our system, state expansion occurs devoid of backaction from photon recoil, making this approach suitable for coherent wave function expansion.

We derive an analytical expression of a Wigner function that approximately describes the time evolution of the one-dimensional motion of a particle in a nonharmonic potential. Our method involves two exact frame transformations, accounting for both the classical dynamics of the centroid of the initial state and the rotation and squeezing about that trajectory. Subsequently, we employ two crucial approximations, namely the constant-angle and linearized-decoherence approximations, upon which our results rely. These approximations are effective in the regime of wide potentials and small fluctuations, namely potentials that enable spatial expansions orders of magnitude larger than the one of the initial state but that remain smaller compared to the relevant dynamical length scale (e.g., the distance between turning points). Our analytical result elucidates the interplay between classical and quantum physics and the impact of decoherence during nonlinear dynamics. This analytical result is instrumental to designing, optimizing, and understanding proposals using nonlinear dynamics to generate macroscopic quantum states of massive particles.

The quantum ground state of a massive mechanical system is a steppingstone for investigating macroscopic quantum states and building high fidelity sensors. With the recent achievement of ground-state cooling of a single motional mode, levitated nanoparticles have entered the quantum domain. To overcome detrimental cross-coupling and decoherence effects, quantum control needs to be expanded to more system dimensions, but the effect of a decoupled dark mode has thus far hindered cavity-based ground state cooling of multiple mechanical modes. Here, we demonstrate two-dimensional (2D) ground-state cooling of an optically levitated nanoparticle. Utilising coherent scattering into an optical cavity mode, we reduce the occupation numbers of two separate centre-of-mass modes to 0.83 and 0.81, respectively. By controlling the frequency separation and the cavity coupling strengths of the nanoparticle's mechanical modes, we show the transition from 1D to 2D ground-state cooling while avoiding the effect of dark modes. Our results lay the foundations for generating quantum-limited high orbital angular momentum states with applications in rotation sensing. The demonstrated 2D control, combined with already shown capabilities of ground-state cooling along the third motional axis, opens the door for full 3D ground-state cooling of a massive object.

We analyze theoretically the motional quantum dynamics of a levitated dielectric sphere interacting with the quantum electromagnetic field beyond the point-dipole approximation. To this end, we derive a Hamiltonian describing the fundamental coupling between photons and center-of-mass phonons, including Stokes and anti-Stokes processes, and the coupling rates for a dielectric sphere of arbitrary refractive index and size. We then derive the laser recoil heating rates and the information radiation patterns (the angular distribution of the scattered light that carries information about the center-of-mass motion) and show how to evaluate them efficiently in the presence of a focused laser beam, in either a running- or a standing-wave configuration. This information is crucial to implement active feedback cooling of optically levitated dielectric spheres beyond the point-dipole approximation. Our results predict several experimentally feasible configurations and parameter regimes where optical detection and active feedback can simultaneously cool to the ground state the three-dimensional center-of-mass motion of dielectric spheres in the micrometer regime. Scaling up the mass of the dielectric particles that can be cooled to the center-of-mass ground state is relevant not only for testing quantum mechanics at large scales but also for current experimental efforts that search for new physics (e.g., dark matter) using optically levitated sensors.

We quantize the electromagnetic field in the presence of a nonmoving dielectric sphere in vacuum. The sphere is assumed to be lossless, dispersionless, isotropic, and homogeneous. The quantization is performed using normalized eigenmodes as well as plane-wave modes. We specify two useful alternative bases of normalized eigenmodes: spherical eigenmodes and scattering eigenmodes. A canonical transformation between plane-wave modes and normalized eigenmodes is derived. This formalism is employed to study the scattering of a single photon, coherent squeezed light, and two-photon states off a dielectric sphere. In the latter case we calculate the second-order correlation function of the scattered field, thereby unveiling the angular distribution of the Hong-Ou-Mandel interference for a dielectric sphere acting as a three-dimensional beam splitter. Our results are analytically derived for an arbitrary size of the dielectric sphere with a particular emphasis on the small-particle limit. This work sets the theoretical foundation for describing the quantum interaction between light and the motional, rotational and vibrational degrees of freedom of a dielectric sphere.

We propose to introduce additional control in levitated optomechanics by trapping a meta-atom, i.e., a subwavelength and high-permittivity dielectric particle supporting Mie resonances. In particular, we theoretically demonstrate that optical levitation and center-of-mass ground-state cooling of silicon nanoparticles in vacuum is not only experimentally feasible but it offers enhanced performance over widely used silica particles in terms of trap frequency, trap depth, and optomechanical coupling rates. Moreover, we show that, by adjusting the detuning of the trapping laser with respect to the particle's resonance, the sign of the polarizability becomes negative, enabling levitation in the minimum of laser intensity, e.g., at the nodes of a standing wave. The latter opens the door to trapping nanoparticles in the optical near-field combining red and blue-detuned frequencies, in analogy to two-level atoms, which is of interest for generating strong coupling to photonic nanostructures and short-distance force sensing.