We investigate spin transport through polarization-resolved spectroscopy by propagating polariton condensates in a quasi-one-dimensional microcavity ridge along macroscopic distances. Under circularly polarized, continuous-wave, nonresonant excitation, a sinusoidal precession of the spin in real space is observed whose phase depends on the emission energy. The experiments are compared with simulations of the spinor-polariton condensate dynamics based on a generalized Gross-Pitaevskii equation, modified to account for incoherent pumping, decay, and energy relaxation within the condensate.
Spin-selective spatial filtering of propagating polariton condensates, using a controllable spin-dependent gating barrier, in a one-dimensional semiconductor microcavity ridge waveguide is reported. A nonresonant laser beam provides the source of propagating polaritons, while a second circularly polarized weak beam imprints a spin dependent potential barrier, which gates the polariton flow and generates polariton spin currents. A complete spin-based control over the blocked and transmitted polaritons is obtained by varying the gate polarization.
We present a time-resolved photoluminescence (PL) study in real and momentum space of a polariton condensate switch in a quasi-one-dimensional semiconductor microcavity. The polariton flow across the ridge is gated by excitons inducing a barrier potential due to repulsive interactions. A study of the device operation dependence on the power of the pulsed gate beam obtains a satisfactory compromise for the on-off signal ratio and switching time of the order of 0.3 and similar to 50 ps, respectively. The opposite transition is governed by the long-lived gate excitons, consequently, the off-on switching time is similar to 200 ps, limiting the overall operation speed of the device to similar to 3 GHz. The experimental results are compared to numerical simulations based on a generalized Gross-Pitaevskii equation, taking into account incoherent pumping, decay, and energy relaxation within the condensate.
C.A. acknowledge financial support from a Spanish FPU scholarship. P.G.S. acknowledges Greek GSRT program “ARISTEIA” (1978) for financial support.The work was partially supported by the Spanish MEC MAT2011-22997, CAM (S-2009/ESP-1503), and FP7 ITN’s “Clermont4” (235114), “Spin-optronics” (237252), and “INDEX”(289968) projects
We introduce an electrically driven scheme to tune the polariton condensate energy in a high-finesse GaAs microcavity. In contrast to the conventional redshift observed in semiconductor quantumwells (QWs) under applied electrical bias arising from the quantum-confined Stark effect (QCSE), we report here the blueshift of a polariton condensate caused by controlled reduction of the Rabi splitting due to tunneling-induced charge buildup and fractional bleaching of QWs. At larger electrical bias, the QCSE becomes dominant, leading to a redshift in the linear regime, while in the nonlinear regime to the eventual quenching of the condensate emission. This ability to tune the polariton condensate energy brings within reach the realization of voltage-controlled polariton condensate devices and variable-wavelength sources of coherent light.
When pumped nonresonantly, semiconductor microcavity polaritons form Bose–Einstein condensates that can be manipulated optically. Using tightly-focused excitation spots, radially expanding condensates can be formed in close proximity. Using high time resolution streak camera measurements we study the time dependent properties of these macroscopic coherent states. By coupling this method with interferometry we observe directly the phase locking of two independent condensates in time, showing the effect of polariton–polariton interactions. We also directly observe fast spontaneous soliton-like oscillations of the polariton cloud trapped between the pump spots, which can be either dark or bright solitons. This transition from dark to bright is a consequence of the change of sign of the nonlinearity which we propose is due to the shape of the polariton dispersion leading to either positive or negative polariton effective mass.
We study the dynamics of polariton condensate wave trains that propagate along a quasi one-dimensional waveguide. Through the application of tuneable potential barriers the propagation can be reflected and multiple reflections used to confine and store a propagating state. Energy-relaxation processes allow the delayed relaxation into a long-living coherent ground state. Aside the potential routing of polariton condensate signals, the system forms an AND-type logic gate compatible with incoherent inputs.
We study the dynamics of polariton condensate wave trains that propagate along a quasi one-dimensional waveguide. Through the application of tuneable potential barriers the propagation can be reflected and multiple reflections used to confine and store a propagating state. Energy-relaxation processes allow the delayed relaxation into a long-living coherent ground state. Aside the potential routing of polariton condensate signals, the system forms an AND-type logic gate compatible with incoherent inputs.
Spin quantum beat spectroscopy is employed to investigate the in-plane anisotropy of the spin dynamics in (001) GaAs/AlGaAs quantum wells induced by an external electric field. This technique allows the anisotropy of the spin relaxation rate Gamma(s) and the electron Lande g factor g* to be measured simultaneously. The measurements are compared to similar data from (001) GaAs/AlGaAs quantum wells with applied shear strain and asymmetric barrier growth. All of these operations act to reduce the symmetry compared to that of a symmetric (001) quantum well in an identical manner (D-2d -> C-2v). However, by looking at the anisotropy of both Gamma(s) and g* simultaneously we show that the microscopic actions of these symmetry breaking operations are very different. The experiments attest that although symmetry arguments are a very useful tool to identify the allowed spin dependent properties of a material system, only a microscopic approach reveals if allowed anisotropies will manifest. DOI: 10.1103/PhysRevB.87.075304
We present a time-resolved study of energy relaxation and trapping dynamics of polariton condensates in a semiconductor microcavity ridge. The combination of two nonresonant, pulsed laser sources in a GaAs ridge-shaped microcavity gives rise to profuse quantum phenomena where the repulsive potentials created by the lasers allow the modulation and control of the polariton flow. We analyze in detail the dependence of the dynamics on the power of both lasers and determine the optimum conditions for realizing an all-optical polariton condensate transistor switch. The experimental results are interpreted in the light of simulations based on a generalized Gross-Pitaevskii equation, including incoherent pumping, decay, and energy relaxation within the condensate.
The strong light-matter coupling regime and lasing in a GaN microcavity fabricated by incorporating a high optical quality GaN membrane inside an all-dielectric mirror cavity is demonstrated at room temperature. A nonlinear increase of the emission and line narrowing marks the onset of polariton lasing regime with significantly reduced threshold compared with previous reports for bulk GaN microcavity. This combination of low lasing thresholds and ease of fabrication allows incorporation of quantum wells and electrical contacts into the active region, paving the way for electrically driven room temperature (RT) polariton laser devices.
In a polariton, laser coherent monochromatic light is produced by a low-energy state of the system at the bottom of a polariton 'trap', where a condensate of polaritons is formed, requiring no conventional population inversion. Following the recent realization of polariton light-emitting diodes (LEDs) based on GaAs microcavities (MCs) operating up to room temperature, efforts have been directed towards the demonstration of an electrically injected polariton laser. However, until now, low-threshold polariton lasing in GaAs MCs under optical pumping has been reported only at low temperatures. Here, we investigate the temperature dependence of lasing threshold across the border of the strong-to-weak coupling regime transition in high-finesse GaAs MCs under non-resonant optical pumping. Remarkably, we find that although lasing in the strong coupling regime is lost when the temperature is raised from 25 to 70 K, the threshold only doubles, in stark contrast with the expected difference of two orders of magnitude. Our results can be explained by considering temperature-induced thermalization of carriers to high wavevector states, increasing the reservoir's overall carrier lifetime, resulting in an order of magnitude higher steady-state carrier density at 70 K under similar pumping conditions.
A polariton condensate transistor switch is realized through optical excitation of a microcavity ridge with two beams. The ballistically ejected polaritons from a condensate formed at the source are gated using the 20 times weaker second beam to switch on and off the flux of polaritons. In the absence of the gate beam the small built-in detuning creates a potential landscape in which ejected polaritons are channelled toward the end of the ridge where they condense. The low-loss photonlike propagation combined with strong nonlinearities associated with their excitonic component makes polariton-based transistors particularly attractive for the implementation of all-optical integrated circuits.
Optically pumping high quality semiconductor microcavities allows for the spontaneous formation of polariton condensates, which can propagate over distances of many microns. Tightly focussed pump spots here are found to produce expanding incoherent bottleneck polaritons which coherently amplify the ballistic polaritons and lead to the formation of unusual ring condensates. This quantum liquid is found to form a remarkable sunflower-like spatial ripple pattern which arises from self interference with Rayleigh-scattered coherent polariton waves in the Cerenkov regime.
We present a time-resolved study of the logical operation of a polariton condensate transistor switch. Creating a polariton condensate (source) in a GaAs ridge-shaped microcavity with a non-resonant pulsed laser beam, the polariton propagation towards a collector, at the ridge edge, is controlled by a second weak pulse (gate), located between the source and the collector. The experimental results are interpreted in the light of simulations based on the generalized Gross-Pitaevskii equation, including incoherent pumping, decay, and energy relaxation within the condensate.
We measure simultaneously the in-plane electron $g$ factor and spin-relaxation rate in a series of undoped inversion-asymmetric (001)-oriented GaAs/AlGaAs quantum wells by spin-quantum beat spectroscopy. In combination the two quantities reveal the absolute values of both the Rashba and the Dresselhaus coefficients and prove that the Rashba coefficient can be negligibly small despite huge conduction-band potential gradients which break the inversion symmetry. The negligible Rashba coefficient is a consequence of the ``isomorphism'' of conduction- and valence-band potentials in quantum systems where the asymmetry is solely produced by alloy variations.
We show experimentally, using spin quantum beat spectroscopy, that strain applied to an undoped symmetric (001) GaAs/AlGaAs multiple quantum well causes an in-plane anisotropy of the spin-relaxation rate Gamma(s), but leaves the electron Lande g factor isotropic. The spin-relaxation-rate anisotropy gives a direct measure of the bulk inversion asymmetry and the strain contributions to the conduction-band spin splitting. The comparison of the measured strain-splitting coefficient C(3) for the quantum well with the value for bulk GaAs suggests a dependence on electron quantum confinement. The isotropic g factor implies a symmetric conduction electron wave function, whereas the anisotropic spin-relaxation rate requires a nonzero expectation value of the valence-band potential gradient on the conduction-band states. Therefore, the experiment suggests that strain generates an effective valence-band potential gradient, while the conduction-band potential remains symmetrical to a good approximation.
We report a study of the nonlinear birefringence in undoped (110)-oriented GaAs/AlGaAs quantum wells using time-resolved pump-probe Kerr spectroscopy. Due to the optical anisotropy of the (110) quantum well plane, photoexcited carriers can give rise to a nonlinear birefringence and so cause probe polarization rotation independent of the pump polarization, i.e., independent of spin orientation. We develop a methodology for accurate determination of electron-spin lifetimes using the Kerr technique which takes account of this phenomenon and present room-temperature measurements of wavelength and power density dependence of the spin-relaxation rate.
Asymmetric quantum well potentials are expected to produce a conduction band spin-splitting which contributes to Dyakonov–Perel (Sov. Phys. Solid State 13:3023, 1971) spin relaxation. Much experimental work has focused on the effect of an electric field on spin dynamics (Karimov et al., in Phys. Rev. Lett. 91:246601, 2003) and little on asymmetry from alloy engineering. By combining time-resolved Kerr rotation measurements with transient spin grating measurements in GaAs/AlGaAs quantum wells we have compared the conduction band spin-splitting resulting from asymmetric alloy engineering with that from applied electric field. The latter is easily measurable, whilst the former is no greater than that in symmetric wells. These results are consistent with an envelope function approximation model that considers the potential profile in both the conduction and the valence bands (Winkler, in Springer Tracts in Modern Physics, vol. 191, 2003).