In the past decade, photo-induced superconducting-like behaviors have been reported in a number of materials driven by intense pump fields. Of particular interest is the high-Tc cuprate YBCO, where such effect has been reported up to the so-called pseudogap temperature T* 300-400 K. In a recent experiment, a transient magnetic field which is proportional to and in the same direction of an applied field has been observed outside the sample, suggestive of flux exclusion due to the Meissner effect. In this paper, we present an alternative interpretation of these experiments based on a mechanism that we term the flux-Floquet instability of the sine-Gordon (SG) model. We take as our premise the model of preformed Cooper pairs in the pseudogap phase. Starting from the local superconducting order parameter in equilibrium, we introduce an extended SG model to describe the dynamics of the relative phase between the layers of a bilayer. We demonstrate that a combination of external magnetic field and strong terahertz drive used in experiments by Fava et al. results in a novel Floquet instability in the model. This instability leads to currents at the edges of the bilayer formed by defects or grain boundaries, with the current flowing in the opposite direction of the equilibrium screening current, producing a giant paramagnetic magnetization in the same direction as the applied field. We show how this scenario can fit most of the available data. To the extent that this model can account for the data, we conclude that the experiments have the important consequence of revealing the presence of local pairing in the pseudogap phase. More broadly our results reveal a new instability in the SG equation that is of fundamental interest, with potential applications such as providing a mechanism for generating large magnetic fields at ultrafast time scales in Josephson devices.

Experiments that subject underdoped YBa2Cu3O6+x (YBCO) to intense terahertz pulses at temperatures between the transition temperature [Formula: see text] and the pseudogap scale T∗ have revealed a reflectivity edge that resembles that of the superconducting state, together with second harmonic generation of a probe pulse modulated at a similar frequency. These have been interpreted in terms of parametric amplification of the lower Josephson plasmon mode. Since this mode is often associated with coherent oscillations between bilayers in the YBCO structure, these experiments have led to the suggestion that the intense pump has created (or revealed) in-plane pair coherence up to [Formula: see text] K. In this paper we propose an alternative explanation by assuming the existence of local pair amplitude and phase at equilibrium for [Formula: see text]. The phase correlation spans only a few lattice constants and we do not assume any pump-induced enhancement of this correlation, either in-plane or between bilayers. Instead, the coherent drive, via a parametric amplification process, induces coherence in the Josephson currents between members of bilayers. When combined with a Floquet framework, the reflectivity data can be explained. The key point is that in the lower Josephson plasmon, the coupling between bilayers is mainly capacitive; the Josephson current between bilayers can be set to zero without strongly affecting the parametric amplification process. Importantly, while superconducting coherence may not be created by the pump, the pseudogap phase must possess a local pairing amplitude at equilibrium. Consequently, these experiments have strong implications for the understanding of the pseudogap phase.

The hyperbolic mode (HM) refers to a polariton mode in a polar insulator where the dielectric function is negative in some direction of propagation. Within a frequency window the light occupies a greatly expanded region in momentum space. The HM in hexagonal Boron Nitride (hBN) has been under intense study and we consider placing a metal directly on top of hBN and ask whether its physical properties can be strongly affected. While the problem resembles superficially the electron phonon coupling problem, there are important differences. Due to the longitudinal nature of the HM mode the coupling is driven by time dependent charge fluctuations which results in a coupling that strongly increases with the energy difference of the initial and final states. We find a significant frequency and momentum dependence of the self energy which allows us to identify the dimensionless coupling constant λ_0 that controls this effect. There is a suppression of the quasi-particle weight but it turns out that the leading correction to the velocity renormalization is canceled. We compute the single particle spectral function which shows a side band that can be measured experimentally. The virtual exchange of HM leads to a repulsive interaction which is ineffective to leading order because of the energy dependence. We are motivated to seek pairing by going to second order. Unfortunately we find that the leading contributions exactly cancel. This cancellation is not an accident and we give an explanation of why this cancellation would take place.

The search for new quantum spin liquid materials relies on systems with strong frustration such as spins on an ideal kagome lattice. However, lattice imperfections can have substantial effects which are as yet not well understood. In recent work, the two-dimensional kagome system YCu_3(OH)_6[(Cl_xBr_(1-x))_3-y(OH)_y] has emerged as a leading candidate hosting a Dirac spin liquid which appears to survive at least for x<0.4, associated with alternating-bond hexagon (ABH) disorder. Here in magnetic samples with x=0.58, y=0.1 we report unusual in-plane ferromagnetic canting (FM) of the in-plane antiferromagnet (AFM), with an unusually wide regime of short-ranged order, and propose theoretical models to explain this behavior. First, we show that Kitaev type exchanges naturally arise on the kagome lattice to second order in the known Dzyaloshinskii-Moriya exchanges, and that these interactions can produce the unusual in-plane FM canting from antichiral AFM. Second, we propose a phenomenological model of weakly-FM-canted spin clusters to describe the short-ranged regime and analyze quantum fluctuations in an ABH toy model to show how ABH disorder can stabilize this regime. The combination of experimental observation and theory suggests that kagome-Kitaev interactions and ABH disorder are necessary for describing the magnetic fluctuations in this family of materials, with potential implications for the proposed proximate spin liquid phase.

Can strong repulsive interactions be shown to give rise to pairing in a controlled way? We find that for a single flavor-polarized band, there is a small expansion parameter in the low density limit, once the Bloch wavefunction form factor is taken into account. A perturbative expansion is possible, even if the interaction is much stronger than the Fermi energy EF. As a matter of principle, our work shows analytically how strong pairing can emerge from strong repulsion. We illustrate our method with two examples: a two-dimensional Dirac model and a one-dimensional tight-binding model with two orbitals. In the latter case, using density matrix renormalization group, we show that the analytical theory indeed guided us to discover the parameter regime where p-wave pairing with order-1 strength is dominant.

Pair density modulation is a phenomenon recently observed in exfoliated flakes of iron-based superconductors, in which the superconducting gap oscillates strongly with the same periodicity as the underlying crystalline lattice. We propose a model that explains this modulation in systems with broken intra-unit-cell symmetries through the emergence of nematic superconductivity, which further breaks the four-fold rotation symmetry. This results in a sublattice texture on the Fermi surface, aligned with the anisotropic superconducting gap of the nematic s± + d state. This gives rise to distinctive gap maxima and minima located on the two inequivalent iron sublattices while still being a zero-momentum pairing state. We discuss how further investigation of such modulations can give insight into the nature of the superconducting pairing, such as the signs of the order parameters and visualization of a phase transition to a mixed two-component state using local probes.

Experiments that subject underdoped YBa 2 Cu 3 O 6+ x (YBCO) to intense terahertz pulses at temperatures between the transition temperature T c and the pseudogap scale T ∗ have revealed a reflectivity edge that resembles that of the superconducting state, together with second harmonic generation of a probe pulse modulated at a similar frequency. These have been interpreted in terms of parametric amplification of the lower Josephson plasmon mode. Since this mode is often associated with coherent oscillations between bilayers in the YBCO structure, these experiments have led to the suggestion that the intense pump has created (or revealed) in-plane pair coherence up to T ∗ ≈ 400 K. In this paper we propose an alternative explanation by assuming the existence of local pair amplitude and phase at equilibrium for T c < T < T ∗ . The phase correlation spans only a few lattice constants and we do not assume any pump-induced enhancement of this correlation, either in-plane or between bilayers. Instead, the coherent drive, via a parametric amplification process, induces coherence in the Josephson currents between members of bilayers. When combined with a Floquet framework, the reflectivity data can be explained. The key point is that in the lower Josephson plasmon, the coupling between bilayers is mainly capacitive; the Josephson current between bilayers can be set to zero without strongly affecting the parametric amplification process. Importantly, while superconducting coherence may not be created by the pump, the pseudogap phase must possess a local pairing amplitude at equilibrium. Consequently, these experiments have strong implications for the understanding of the pseudogap phase.

Recent experiments on the Kagome spin liquid candidate material YCu_{3}(OH)_{6}Br_{2}[Br_{1-y}(OH)_{y}] suggest the presence of Dirac fermionic spinons near the magnetization plateau at 1/9. Theories suggest that the spinons are charge neutral spin-1/2 excitations, in a 2π/3 flux, which triples the unit cell. Generally a gap is expected, and there is no symmetry protection for the Dirac nodes in this system. The question arises as to what causes the nodes and stabilizes them. In this work, we propose a node-creation and node-pinning mechanism driven by Dzyaloshinskii-Moriya (DM) interactions. Employing Gutzwiller-projected variational Monte Carlo calculations, we demonstrate that DM interactions induce a band closing phase transition in the spinon spectrum. There is a change in the Chern number when the bands are inverted. Together with the DM-generated internal gauge flux, the coupling to the spinon orbital magnetization counteracts the band reopening. This interplay energetically pins the Dirac nodes over a range of parameters, resulting in a pinning mechanism distinct from the usual one from symmetry protection.

The hyperbolic mode (HM) refers to a polariton mode where the dielectric function is negative in some direction of propagation. Within a frequency window the light occupies a greatly expanded region in momentum space. We compute the photon density of states and find that the zero point fluctuation in the RMS electric field can reach MV/cm, comparable to the largest field used in pump probe experiments in the THz scale. The HM in hexagonal Boron Nitride (hBN) has been under intense study and we consider placing a material directly on top of or sandwiched between hBN crystals. We consider two examples. First the material is a metal and we calculate the modification of the quasi-particle spectral weight, Fermi velocity and pairing interaction. Next we consider a material that is close to the Mott transition. We find that a substantial shift in the metal-insulator transition is possible, but the effect decays rapidly with distance, so that only a few monolayers are affected. We provide estimates and suggestions for a number of materials of interest.

Strong optical drives have been shown to induce transient superconducting-like response in materials above their equilibrium T_c. Many of these materials already exhibit short-range superconducting correlations in equilibrium. This motivates the question: can external driving enhance coherence in systems with superconducting correlations but no long-range order? We explore this scenario in the two-dimensional XY model with a periodically modulated stiffness using overdamped Langevin dynamics. We find that, even though the modulation leaves the average coupling unchanged, the drive can markedly increase long-range, time-averaged correlations in systems well above the equilibrium Berezinskii-Kosterlitz-Thouless temperature. The outcome depends on the ratio of the drive frequency to the intrinsic relaxation rate: faster drives primarily heat the system, suppressing correlations and conductivity. For slower drives, the optical conductivity is modified so that the real part exhibits a prolonged effective Drude scattering time, while the imaginary part has a strengthened low-frequency 1/ω behavior. We map out these regimes across temperature, frequency, and amplitude, and rationalize them via simple analytics and vortex-thermalization arguments. Overall, we identify a generic nonequilibrium route to enhance coherence in XY-like systems, with potential relevance to experiments reporting light-induced superconductivity.

We predict that the spin-polarized electrons in a two-dimensional triangular lattice with strong electron-electron repulsion gives rise to f-wave pairing. The key point is that the first-order interaction, which is usually pair-breaking, vanishes or nearly vanishes in certain f-wave channels due to symmetry constraints. As a result, these f-wave pairing channels are governed by the subleading-order processes which enable pairing when the perturbation theory is controlled. We illustrate this using the Hubbard model on the triangular lattice with on-site and nearest-neighbor repulsion, where we find a T_c∼ 1% of electron's bandwidth. For a general screened interaction, the same idea works asymptotically, but a third-order calculation is needed to fully determine the strength of f-wave pairing.

In metals, electrons in a magnetic field undergo cyclotron motion, leading to oscillations in physical properties called quantum oscillations. This phenomenon has never been seen in a robust insulator because there are no mobile electrons. We report an exception to this rule. We study a Mott insulator on a kagome lattice which does not order magnetically down to milli-Kelvin temperatures despite antiferromagnetic interactions. We observe a plateau at magnetization equal to 1 9 Bohr magneton per magnetic ion, accompanied by oscillations in the magnetic torque, reminiscent of quantum oscillations in metals. The temperature dependence obeys Fermi distribution. These phenomena are consistent with a quantum spin liquid state whose excitations are fermionic spinons with a Dirac-like spectrum coupled to an emergent gauge field.

The spin-1/2 kagome Heisenberg antiferromagnets are believed to host exotic quantum entangled states. Recently, the reports of 1/9 magnetization plateau and magnetic oscillations in a kagome antiferromagnet YCu_{3}(OH)_{6}Br_{2}[Br_{x}(OH)_{1-x}] (YCOB) have made this material a promising candidate for experimentally realizing quantum spin liquid states. Here, we present measurements of the specific heat C_{p} in YCOB in high magnetic fields (up to 41.5 T) down to 0.46 K, and the 1/9 plateau feature has been confirmed. Moreover, the temperature dependence of C_{p}/T in the vicinity of 1/9 plateau region can be fitted by a linear in T term which indicates the presence of a Dirac spectrum, together with a constant term, which indicates a finite density of states contributed by other spinon Fermi surfaces. Surprisingly, the constant term is highly anisotropic in the direction of the magnetic field. Additionally, we observe a double-peak feature near 30 T above the 1/9 plateau which is another hallmark of fermionic excitations in the specific heat. This combination of gapless behavior and the double-peak structure strongly suggests that the 1/9 plateau in YCOB is nontrivial and hosts fermionic quasiparticles.

Pair density modulation is a superconducting state, recently observed in exfoliated iron-based superconductor flakes, in which the superconducting gap oscillates strongly with the same periodicity as the underlying crystalline lattice. We propose a microscopic model that explains this modulation through a combination of glide-mirror symmetry breaking and the emergence of nematic superconductivity. The first ingredient results in a sublattice texture on the Fermi surface, which is aligned with the anisotropic superconducting gap of the nematic s_±+d state. This gives rise to distinctive gap maxima and minima located on the two inequivalent iron sublattices while still being a zero-momentum pairing state. We discuss how further investigation of such modulations can give insight into the nature of the superconducting pairing, such as the signs of the order parameters and visualization of a phase transition to a mixed two-component state using local probes.

We propose cyclotron resonance as an optical probe for emergent fractionalized excitations in U(1) quantum spin liquids, focusing on kagome antiferromagnets. In contrast to conventional systems, where cyclotron resonance directly couples to charged carriers, spinons in spin liquids are charge-neutral and interact only through an emergent gauge field, making direct probing challenging. We identify two key mechanisms by which an external physical electromagnetic field induces emergent electric and magnetic fields, enabling indirect coupling to spinons. Using these mechanisms, we compute the absorption rate of the cyclotron resonance response for Dirac spinons forming Landau levels. Our analysis shows that, although the absorption per layer is small, the absence of a skin-depth limitation in insulating spin liquids allows for cumulative absorption comparable to graphene in realistic sample sizes for the recently discovered spin-liquid candidate material YCu3(OH)6Br2 [Br1-y(OH)y]. Our proposed cyclotron-resonance measurement is a decisive, practical test for spinon Landau levels, providing quantitative expectations where clear experimental evidence has so far been lacking.

Superconducting (SC) states that break space-group symmetries of the underlying crystal can exhibit nontrivial spatial modulation of the order parameter. Previously, such states were intimately associated with the breaking of translational symmetry1,2, resulting in the density-wave orders3-8, with wavelengths spanning several unit cells9-19. However, a related basic concept has long been overlooked20: when only intra-unit-cell symmetries of the space group are broken, the SC states can show a distinct type of nontrivial modulation preserving long-range lattice translation. Here we refer to this new concept as the pair density modulation (PDM) and report the first observation of a PDM state in exfoliated thin flakes of the iron-based superconductor FeTe0.55Se0.45. Using scanning tunnelling microscopy (STM), we discover robust SC gap modulation with the wavelength corresponding to the lattice periodicity and the amplitude exceeding 30% of the gap average. Notably, we find that the observed modulation originates from the large difference in SC gaps on the two nominally equivalent iron sublattices. The experimental findings, backed up by model calculations, suggest that, in contrast to the density-wave orders, the PDM state is driven by the interplay of sublattice symmetry breaking and a peculiar nematic distortion specific to the thin flakes. Our results establish new frontiers for exploring the intertwined orders in strong-correlated electronic systems and open a new chapter for iron-based superconductors.

We consider a planar superconducting-normal metal junction with both inelastic and spin-flip scattering processes present. In the diffusive limit, we use a one-dimensional formulation of the Usadel equation to compute the self-consistent energy dependence of the single-particle density of states as a function of distance from the interface on both the superconducting and metallic sides for various spatial profiles of a pair-breaking spin-flip term. The pair-breaking processes fill in the superconducting gap at zero energy, which is reflected in the zero-bias tunneling conductance in scanning tunneling microscopy/spectroscopy experiments, in the vicinity of the junction. We also investigate the impact of having a partially transparent interface at the junction. We compare our findings with the observed exponential rise in the zero-bias conductance at the 1H step edge in recent experiments on 4Hb-TaS2 [A. K. Nayak et al., Nat. Phys. 17 , 1413 (2021)].

This paper aims to clarify the nature of a surprising ordered phase recently reported in biased Bernal bilayer graphene that occurs at the phase boundary between the isospin-polarized and unpolarized phases. Strong nonlinearity of transport at abnormally small currents, with dI/dV vs. I sharply rising and then falling back, is typical for a charge/spin-density-wave state (CDW or SDW) sliding transport. Here, however, it is observed at an isospin-order phase boundary, prompting a question about the CDW/SDW mechanism and its relation to the quantum critical point. We argue that the observed phase diagram cannot be understood within a standard weak-coupling picture. Rather, it points to a mechanism that relies on an effective interaction enhancement at a quantum critical point. We develop a detailed strong-coupling framework accounting for the soft collective modes that explain these observations.

A localized Zeeman field, intensified at heterostructure interfaces, could play a crucial role in a broad area including spintronics and unconventional superconductors. Conventionally, the generation of a local Zeeman field is achieved through magnetic exchange coupling with a magnetic material. However, magnetic elements often introduce defects, which could weaken or destroy superconductivity. Alternatively, the coupling between a superconductor with strong spin-orbit coupling and a nonmagnetic chiral material could serve as a promising approach to generate a spin-active interface. Here, we leverage an interface superconductor, namely, induced superconductivity in noble metal surface states, to probe the spin-active interface. Our results unveil an enhanced interface Zeeman field, which selectively closes the surface superconducting gap while preserving the bulk superconducting pairing. The chiral material, i.e., trigonal tellurium, also induces Andreev bound states (ABS) exhibiting spin polarization. The field dependence of ABS manifests a substantially enhanced interface Landé g -factor ( g eff ~ 12), thereby corroborating the enhanced interface Zeeman energy.