Prompt fission neutron spectra (PFNS) are crucial to any neutronic simulation of critical nuclear systems. An experimental setup dedicated to the measurements of PFNS of very high accuracy was developed at the Los Alamos Neutron Science Center (LANSCE) some ten years ago. It allows for the measurement of PFNS for neutron induced fission at the Weapon Neutron Research (WNR) neutron source of the LANSCE. A measurement of the PFNS from the 235U(n,f) reaction was realized recently and is currently analyzed. Preliminary results are presented here and are compared to present nuclear data evaluations.
A fundamental framework to describe nuclear matter as a function of pressure and nuclear isospin asymmetry is the nuclear Equation of State (EoS). Constraining the parameters of the EoS is one of the central issues in nuclear physics, especially since the slope parameter L has not yet been constrained well experimentally. It has been identified that a precise determination of the neutron-removal cross section in neutron-rich nuclei, which correlates with the neutron-skin thickness, would provide a more precise constraint on L. To this end, an experiment was performed at the (RB)-B-3 part of the FAIR Phase-0 program. The reactions are studied in inverse kinematics with neutron-rich tin isotopes in the mass range of A = 124-134 on carbon targets of different thicknesses. The reaction products have been measured at beam energies of 400-900 MeV/u in a kinematically complete manner. In this communication, the analysis of Sn-124 + C-12 at 900 MeV/u is presented. The charge-exchange reactions, resulting processes, and their role in the calculation of other reaction cross sections are discussed.
Missing mass spectroscopy of the unbound C-8 nucleus was performed by the one-neutron transfer 9C(p,d)8C reaction at 55 MeV/nucleon. Besides the known ground state, two new resonant states were observed, the first at an excitation energy of 3.40(25) MeV with a width of 3.0(5) MeV, the second at 18.6(5) MeV with a width of 3.9(11) MeV. Spin and parity J(pi)=2(+) were assigned to the first resonance from the distorted-wave Born approximation analysis of the experimental differential cross section. The excitation energy of the 2(+) resonance in C-8 supports the persistence of the subshell closure at the semimagic number Z = 6, as is the case for N = 6. The mirror energy difference relative to the 2(+ )state in 8He, Delta E-x=-0.14(25) MeV, is compatible with zero. Both states represent resonances in the continuum, unbound by about 1.4 and 6.9 MeV, respectively, above the particle thresholds. A simple theoretical model emphasizes the difference in unboundedness to account for a symmetry in mirror energies. This unique system is expected to provide a salient test of theoretical models, which include the treatment of the continuum.
Missing mass spectroscopy of the unbound $^{8}\mathrm{C}$ nucleus was performed by the one-neutron transfer $^{9}\mathrm{C}(p,d)^{8}\mathrm{C}$ reaction at 55 MeV/nucleon. Besides the known ground state, two new resonant states were observed, the first at an excitation energy of 3.40(25) MeV with a width of 3.0(5) MeV, the second at 18.6(5) MeV with a width of 3.9(11) MeV. Spin and parity ${J}^{\ensuremath{\pi}}={2}^{+}$ were assigned to the first resonance from the distorted-wave Born approximation analysis of the experimental differential cross section. The excitation energy of the ${2}^{+}$ resonance in $^{8}\mathrm{C}$ supports the persistence of the subshell closure at the semimagic number $Z$ = 6, as is the case for $N$ = 6. The mirror energy difference relative to the ${2}^{+}$ state in $^{8}\mathrm{He}, \mathrm{\ensuremath{\Delta}}{E}_{\mathrm{x}}=\ensuremath{-}0.14$(25) MeV, is compatible with zero. Both states represent resonances in the continuum, unbound by about 1.4 and 6.9 MeV, respectively, above the particle thresholds. A simple theoretical model emphasizes the difference in unboundedness to account for a symmetry in mirror energies. This unique system is expected to provide a salient test of theoretical models, which include the treatment of the continuum.
Nuclear fission is still one of the most complex physical processes due to the interplay between macroscopic and microscopic nuclear properties that decide the output. An example of this coupling is the presence of nuclear dissipation as an important ingredient that contributes to drive the dynamics and has a clear impact on the time of the process. However, different theoretical interpretations and scarce experimental data make it poorly understood. At low excitation energy, the relative yields of fragments even and odd atomic numbers show a clear difference, which can be quantified with the so-called even-odd effect. This seemingly mundane property can be used to obtain information about the energy dissipated during the process and the role of structure in its dynamics. In this paper, the study of the even-odd effect for elasticand transfer-induced fission data is discussed. A clear connection with particular fragment shells and the dissipation energy is found, as detailed in Ref. [1]. In addition, preliminary results from quasi-fission data show the formation of a relatively large even-odd effect, which suggests a process with low dissipation mainly consisting in the exchange of nucleon pairs.
The $^{18}\mathrm{Ne}(d,t)^{17}\mathrm{Ne}$ and $^{18}\mathrm{Ne}(d,^{3}\mathrm{He})^{17}\mathrm{F}$ single-nucleon pickup reactions were measured at 16.5 MeV/nucleon in inverse kinematics together with elastic and inelastic scattering channels. The full set of measured exclusive differential cross sections was compared with the mirror reaction channels on stable $^{18}\mathrm{O}$ after consistent reanalysis using coupled reaction channels calculations. Within this interpretation scheme, most of the spectroscopic factors extracted for the population of unbound states in $^{17}\mathrm{F}$ match within uncertainties with their mirror partners in $^{17}\mathrm{O}$. However, for the deeply bound neutron removal channel to $^{17}\mathrm{Ne}$, a significant symmetry breaking with the mirror proton-removal channel leading to $^{17}\mathrm{N}$ is evidenced by an overall single-particle strength reduction.
The Coulomb excitation of Sn-124,Sn-128,Sn-130,Sn-132,Sn-134 isotopes in the electric field of a Pb target have been studied using the (RB)-B-3 setup as a part of the FAIR Phase-0 program. The experiment was motivated by the possibility of using the nuclear dipole response to infer valuable information on the slope of the symmetry energy of the nuclear equation of state. Measurements were performed in inverse kinematics at relativistic energies of 750 MeV/u and 904 MeV/u. The analysis method and preliminary results for the decay channel with a single outgoing neutron for Sn-124 are reported.
Properties of the nuclear equation of state (EoS) can be probed by measuring the dynamical properties of nucleus-nucleus collisions. In this study, we present the directed flow (v1), elliptic flow (v2) and stopping (VarXZ) measured in fixed target Sn + Sn collisions at Image 1 with the SπRIT Time Projection Chamber. We perform Bayesian analyses in which EoS parameters are varied simultaneously within the Improved Quantum Molecular Dynamics-Skyrme (ImQMD-Sky) transport code to obtain a multivariate correlated constraint. The varied parameters include symmetry energy, S0, and slope of the symmetry energy, L, at saturation density, isoscalar effective mass, ms⁎/mN, isovector effective mass, mv⁎/mN and the in-medium cross-section enhancement factor η. We find that the flow and VarXZ observables are sensitive to the splitting of proton and neutron effective masses and the in-medium cross-section. Comparisons of ImQMD-Sky predictions to the SπRIT data suggest a narrow range of preferred values for ms⁎/mN, mv⁎/mN and η.
The ^18Ne(d,t)^17Ne and ^18Ne(d,^3He)^17F single-nucleon pickup reactions were measured at 16.5 MeV/nucleon in inverse kinematics together with elastic and inelastic scattering channels. The full set of measured exclusive differential cross sections was compared with the mirror reaction channels on stable ^18O after consistent reanalysis using coupled reaction channels calculations. Within this interpretation scheme, most of the spectroscopic factors extracted for the population of unbound states in ^17F match within uncertainties with their mirror partners in ^17O. However, for the deeply-bound neutron removal channel to ^17Ne, a significant symmetry breaking with the mirror proton-removal channel leading to ^17N is evidenced by an overall single-particle strength reduction.
The low-lying structure of ^15C has been investigated via the neutron-removal ^16C(d,t) reaction. Along with bound neutron sd-shell hole states, unbound p-shell hole states have been firmly confirmed. The excitation energies and the deduced spectroscopic factors of the cross-shell states are an important measure of the [(p)^-1(sd)^2] neutron configurations in ^15C. Our results show a very good agreement with shell-model calculations using the SFO-tls interaction for ^15C. However, a modification of the p-sd and sd-sd monopole terms was applied in order to reproduce the N=9 isotone ^17O. In addition, the excitation energies and spectroscopic factors have been compared to the first calculations of ^15C with the ab initio self-consistent Green's function method employing the NNLO_sat interaction. The results show the sensitivity to the size of the N=8 shell gap and highlight the need of going beyond the current truncation scheme in the theory.
The boundaries of the Chart of Nuclides contain exotic isotopes that possess extreme proton-toneutron asymmetries. Here we report on strong evidence of 9N, one of the most exotic proton-rich isotopes where more than one half of its constitute nucleons are unbound. With seven protons and two neutrons, this extremely proton-rich system would represent the first-known example of a ground-state five-proton emitter. The invariant-mass spectrum of its decay products can be fit with two peaks whose energies are consistent with the theoretical predictions of an open-quantum-system approach, however we cannot rule out the possibility that only a single resonance-like peak is present in the spectrum.
In the last decades, measurements of spallation, fragmentation and Coulex induced fission reactions in inverse kinematics have provided valuable data to accurately investigate the fission dynamics and nuclear structure at large deformations of a large variety of stable and non-stable heavy nuclei. To go a step further, we propose now to induce fission by the use of quasi-free (p,2p) scattering reactions in inverse kinematics, which allows us to reconstruct the excitation energy of the compound fissioning system by using the four-momenta of the two outgoing protons. Therefore, this new approach might permit to correlate the excitation energy with the charge and mass distributions of the fission fragments and with the fission probabilities, given for the first time direct access to the simultaneous measurement of the fission yield dependence on temperature and fission barrier heights of exotic heavy nuclei, respectively. The first experiment based on this methodology was realized recently at the GSI/FAIR facility and a detailed description of the experimental setup is given here.
During the last decade, the use of inverse kinematics in the experimental study of fission is bringing a wealth of new observables obtained in single measurements, allowing their analysis and their correlations. An ongoing application of this technique is the basis of a series of experiments performed with the variable -mode, large -acceptance VAMOS++ spectrometer at GANIL. A recent experiment has been focused on the survival of the nuclear structure effects at high excitation energy in fission and quasi-fission. The full isotopic identification of fragments, the fission dynamics and the ratio between the production of fragments with even and odd atomic numbers, the so-called proton even -odd effect, are shown. The latter shows a different mechanism for fission and quasi -fission that could be used to separate fission from quasi-fission.
Nuclei in the vicinity of 78Ni are important benchmarks for nuclear structure, which can reveal changes in the shell structure far from stability. Spectroscopy of the odd-odd isotope 78Cu was performed for the first time in an experiment with the EURICA setup at the Radioactive Isotope Beam Factory at RIKEN Nishina Center. Excited states in the neutron-rich isotope were populated following the beta decay of 78Ni produced by in-flight fission and
Despite the recent experimental and theoretical progress in the investigation of the nuclear fission process, a complete description still represents a challenge in nuclear physics because it is a very complex dynamical process, whose description involves the coupling between intrinsic and collective degrees of freedom, as well as different quantum-mechanical phenomena. To improve on the existing data on nuclear fission, we produce fission reactions of heavy nuclei in inverse kinematics by using quasi-free (p,2p) scattering, which induce fission through particle-hole excitations that can range from few to ten's of MeV. The measurement of the four-momenta of the two outgoing protons allows to reconstruct the excitation energy of the fissioning compound nucleus and therefore to study the evolution of the fission yields with temperature. The realization of this kind of experiment requires a complex experimental setup, providing full isotopic identification of both fission fragments and an accurate measurement of the momenta of the two outgoing protons. This was realized recently at the GSI/FAIR facility and here some preliminary results are presented.
Nuclear fission is a complex dynamical process, whose description involves the coupling between intrinsic and collective degrees of freedom, as well as different quantum-mechanical phenomena. For this reason, to this day it still lacks a satisfactory and complete microscopic description. In addition to the importance of describing fission itself, studies of the r-process in astrophysics depend on fission observables to constrain the theoretical models that explain the isotopic abundances in the Universe. To improve on the existing data, fission reactions of heavy nuclei in inverse kinematics are produced in quasi-free (p,2p) scattering reactions, which induce fission through particle-hole excitations that can range from few to tens of MeV. In order to study the evolution of the fission yields with temperature, the excitation energy of the fissioning system must be reconstructed, which is possible by measuring the four-momenta of the two outgoing protons. Performing this kind of experiment requires a complex experimental setup, providing full isotopic identification of both fission fragments and an accurate measurement of the momenta of the two outgoing protons. This was realized recently at the GSI/FAIR facility and some of the results obtained for the charge distributions are presented in this work.
Excited states in Cu-78 were observed for the first time following the ss decay of Ni-78 created by in-flight fission of U-238. Based on the coincidence relationships between the observed gamma-ray transitions, it was possible to construct a level scheme comprising eight excited states with tentative spin assignments for 5 of them. In addition to the gamma-decaying states, an isomeric state with a lifetime of 3.8(4) ms was found to decay by internal conversion.
The experimental data collected during the S515 experiment performed by the R3B collaboration at GSI/FAIR represent a great opportunity to investigate nucleon knockout reactions of exotic nuclei in the region of Sn using complete kinematics measurements. These cross sections can be used in the future to investigate the quenching in the knockout of the minority species (neutrons or protons) in nuclei far from stability. Some of the arguments put forward are the underestimation of the knockout of deeply bound nucleons, final state interactions or the role of short-range correlations (SRC). Recently, several works based on inclusive measurements have shown that these SRCs could reduce the single nucleon knockout cross sections by around 50%, depending on the neutron excess (N/Z) of the initial projectile. The S515 data can help us to go further in this investigation because it allows to correlate the knockout cross sections of one, two or more nucleons with the number of protons and neutrons emitted from the target and which can be detected by the CALIFA and NeuLAND detectors, respectively, and perform complete kinematical studies on the nature of the event (SRC, evaporation, emission of clusters, final-state interactions...). Here the results obtained for the charge distribution of reaction residues are presented, which is one of the first steps of the still on-going analysis.
The low-lying structure of 15C has been investigated via the neutron-removal d(16C, t) reaction. The experiment was performed at GANIL using a secondary 16C beam produced by fragmentation in the LISE spectrometer at 17.2 MeV/nucleon with an intensity of 5 × 104 pps and 100% purity. The angle and energy of the light ejectile were detected by three MUST2 telescopes. The missing mass technique was used to reconstruct the excitation energy of 15C. In this spectrum, two bound states were observed (gs and the first excited state) and two unbound resonant states above the neutron separation threshold (S n = 1.218 MeV). From the differential cross sections, information on the angular momentum of the transferred nucleon and spectroscopic factors were deduced. The excitation energies and the deduced spectroscopic factors of the negative parity states placed above the neutron separation energy are an important measurement of the 2p-1h configurations in 15C. Our results show good agreement with shell-model calculations with the YSOX interaction and show a sensitivity to the N=8 shell gap.
A new experimental fission approach is presented in the context of the R3B (Reactions with Relativistic Radioactive Beams) collaboration, at the GSI/FAIR facility, in which knockout reactions in inverse kinematics are used to induce fission of 238U that will allow to characterise the excitation energy of the fission process and all the fission products. The CALIFA (CALorimeter for In-Flight detection of γ-rays and high energy charged pArticles) calorimeter, a key part of the R3B set-up, is used to reconstruct the momenta of the two protons from the (p, 2p) reactions. Preliminary results show that kinematic variables and first estimates for nucleon-removal cross sections are well reconstructed and in good agreement with other experimental measurements.