Emerging from the intricate interplay of topology and magnetism, the giant anomalous Hall effect (AHE) is the most known topological property of the recently discovered kagomé ferromagnetic Weyl semimetal Co3Sn2S2 with the magnetic Co atoms arranged on a kagomé lattice. Here it is reported that the AHE in Co3Sn2S2 can be fine-tuned by an applied magnetic field orientated within ≈2° of the kagomé plane, while beyond this regime, it stays unchanged. Particularly, it can vanish in magnetic fields parallel to the kagomé plane and even decrease in magnetic fields collinear with the spin direction. This tunable AHE can be attributed to local spin switching enabled by the geometrical frustration of the magnetic kagomé lattice, revealing that spins in a kagomé ferromagnet change their switching behavior as the magnetic field approaches the kagomé plane. These results also suggest a versatile way to tune the properties of a kagomé magnet.
TaCo2Te2 is recently reported to be an air-stable, high mobility van der Waals material with probable magnetic order. Here we investigate the scaling behavior of its magnetoresistance. We measured both the longitudinal (pxx) and Hall (pxy) magnetoresistivities of TaCo2Te2 crystals in magnetic fields parallel to the c axis and found that the magnetoresistance violates the Kohler's rule MR similar to f [H/p0] while obeying the extended Kohler's rule MR similar to f [H/(nT p0)], where MR similar to [pxx(H) - p0]/p0, H is the magnetic field, nT is a thermal factor, and pxx(H) and p0 are the resistivities at H and zero field, respectively. While deviating from those of the densities of electrons (ne) and holes (nh) obtained from the two-band model analysis of the magnetoconductivities, the temperature dependence of nT is close to that of the Hall carrier densities nH calculated from the slopes of pxy(H) curves at low magnetic fields, providing a different way to obtain the thermal factor in the extended Kohler's rule.
Recently, anomalies in the temperature dependences of the carrier density and/or mobility derived from analysis of the magnetoresistivities using the conventional two-band model have been used to unveil intriguing temperature-induced Lifshitz transitions in various materials. For instance, two temperature-driven Lifshitz transitions were inferred to exist in the Dirac nodal-line semimetal ZrSiSe, based on two-band model analysis of the Hall magnetoconductivities where the second band exhibits a change in the carrier type from holes to electrons when the temperature decreases below T = 106 K and a dip is observed in the mobility versus temperature curve at T = 80 K. Here, we revisit the experiments and two-band model analysis on ZrSiSe. We show that the anomalies in the second band may be spurious, because the first band dominates the Hall magnetoconductivities at T > 80 K, making the carrier type and mobility obtained for the second band from the two-band model analysis unreliable. That is, care must be taken in interpreting these anomalies as evidences for temperature-driven Lifshitz transitions. Our skepticism on the existence of such phase transitions in ZrSiSe is further supported by the validation of the Kohler's rule for magnetoresistances at temperatures below 180 K. This work showcases potential issues in interpreting anomalies in the temperature dependence of the carrier density and mobility derived from the analysis of magnetoconductivities or magnetoresistivities using the conventional two-band model.
Magnetism plays a key role in the emergence of topological phenomena in the Weyl semimetal Co3Sn2S2, which exhibits a ferromagnetic (FM) interactions along the c-axis of the crystal and an antiferromagnetic (AFM) interactions within the ab plane. Extensive studies on the temperature dependence of the magnetism with the magnetic field along the c-axis have uncovered a number of magnetic phases. Currently, the nature and origins of the reported magnetic phases are under debate. Here we report on magnetic field orientation effects on the magnetism in Co3Sn2S2. The shape of the hysteresis loop of the Hall resistance at a fixed temperature is found to change from rectangular to bow-tie-like as the magnetic field is tilted from the c-axis towards the ab plane, resembling that reported for magnetic fields along the c-axis as the temperature approaches the Curie temperature from below. Unlike their temperature-dependent counterparts, the newly observed bow-tie-like hysteresis loops show exchange bias. Our results showcase the contribution of the in-plane AFM interactions to the magnetism in Co3Sn2S2 and demonstrate a new way to tune its magnetic phases. They also shed light on the temperature-dependent magnetic phases occurring in the magnetic field along the c-axis of the crystal.
Magnetism plays a key role in the emergence of topological phenomena in the Weyl semimetal Co3Sn2S2, which exhibits a ferromagnetic (FM) interactions along the c-axis of the crystal and an antiferromagnetic (AFM) interactions within the ab plane. Extensive studies on the temperature dependence of the magnetism with the magnetic field along the c-axis have uncovered a number of magnetic phases. Currently, the nature and origins of the reported magnetic phases are under debate. Here we report on magnetic field orientation effects on the magnetism in Co3Sn2S2. The shape of the hysteresis loop of the Hall resistance at a fixed temperature is found to change from rectangular to bow-tie-like as the magnetic field is tilted from the c-axis towards the ab plane, resembling that reported for magnetic fields along the c-axis as the temperature approaches the Curie temperature from below. Unlike their temperature-dependent counterparts, the newly observed bow-tie-like hysteresis loops show exchange bias. Our results showcase the contribution of the in-plane AFM interactions to the magnetism in Co3Sn2S2 and demonstrate a new way to tune its magnetic phases. They also shed light on the temperature-dependent magnetic phases occurring in the magnetic field along the c-axis of the crystal.
We report on temperature-dependent size and anisotropy of the Fermi pockets in graphite revealed by magnetotransport measurements. The magnetoresistances obtained in fields along the c-axis obey an extended Kohler's rule, with the carrier density following prediction of a temperature-dependent Fermi energy, indicating a change in the Fermi pocket size with temperature. The angle-dependent magnetoresistivities at a given temperature exhibit a scaling behavior. The scaling factor that reflects the anisotropy of the Fermi surface is also found to vary with temperature. Our results demonstrate that temperature-driven changes in Fermi surface can be ubiquitous and need to be considered in understanding the temperature-dependent carrier density and magnetoresistance anisotropy in semimetals.
A notable phenomenon in topological semimetals is the violation of Kohler's rule, which dictates that the magnetoresistance MR obeys a scaling behavior of MR = f (H / rho(0)), where MR = [rho(H) - rho(0)]/rho(0) and H is the magnetic field, with rho(H) and rho(0) being the resistivity at H and zero field, respectively. Here, we report a violation originating from thermally induced change in the carrier density. We find that the magnetoresistance of the Weyl semimetal TaP follows an extended Kohler's rule MR = f[H/(n(T)rho(0))], with n(T) describing the temperature dependence of the carrier density. We show that n(T) is associated with the Fermi level and the dispersion relation of the semimetal, providing a new way to reveal information on the electronic band structure. We offer a fundamental understanding of the violation and validity of Kohler's rule in terms of different temperature responses of n(T). We apply our extended Kohler's rule to BaFe2(As1-xPx)(2) to settle a long-standing debate on the scaling behavior of the normal-state magnetoresistance of a superconductor, namely, MR similar to tan(2)theta(H), where theta(H) is the Hall angle. We further validate the extended Kohler's rule and demonstrate its generality in a semiconductor, InSb, where the temperature-dependent carrier density can be reliably determined both theoretically and experimentally.