Because PM2.5 concentrations are not regularly monitored in Mbarara, Uganda, this study was implemented to test whether correlations exist between weather parameters and PM2.5 concentration, which could then be used to estimate PM2.5 concentrations. PM2.5 was monitored for 24 h periods once every week for eight months, while weather parameters were monitored every day. The mean dry and wet season PM2.5 concentrations were 70.1 and 39.4 µg/m3, respectively. Diurnal trends for PM2.5 levels show bimodal peaks in the morning and evening. The univariate regression analysis between PM2.5 and meteorological factors for the 24 h averages yields a significant correlation with air pressure when all data are considered, and when the data are separated by season, there is a significant correlation between PM2.5 concentration and wind speed in the dry season. A strong correlation is seen between diurnal variations in PM2.5 concentration and most weather parameters, but our analysis suggests that in modeling PM2.5 concentrations, the importance of these meteorological factors is mainly due to their correlation with underlying causes including diurnal changes in the atmospheric boundary layer height and changes in sources both hourly and seasonally. While additional measurements are needed to confirm the results, this study contributes to the knowledge of short-term and seasonal variation in PM2.5 concentration in Mbarara and forms a basis for modeling short-term variation in PM2.5 concentration and determining the effect of seasonal and diurnal sources on PM2.5 concentration.
Air pollution is the leading environmental cause of death globally, and most mortality occurs in resource-limited settings such as sub-Saharan Africa. The African continent experiences some of the worst ambient air pollution in the world, yet there are relatively little African data characterizing ambient pollutant levels and source admixtures. In Uganda, ambient PM2.5 levels exceed international health standards. However, most studies focus only on urban environments and do not characterize pollutant sources. We measured daily ambient PM2.5 concentrations and sources in Mbarara, Uganda from May 2018 through February 2019 using Harvard impactors fitted with size-selective inlets. We compared our estimates to publicly available levels in Kampala, and to World Health Organization (WHO) air quality guidelines. We characterized the leading PM2.5 sources in Mbarara using x-ray fluorescence and positive matrix factorization. Daily PM2.5 concentrations were 26.7 µg m−3 and 59.4 µg m−3 in Mbarara and Kampala, respectively (p < 0.001). PM2.5 concentrations exceeded WHO guidelines on 58
The atmospheric boundary layer height is important for constraining air pollution and meteorological models. This study attempted to validate the MODIS-estimated atmospheric boundary layer height (ABLH), and variation in the ABLH in Uganda was evaluated. The ABLH was estimated from MODIS data using the mixing ratio profile gradient method and compared to the ABLH estimated from radiosonde data using three different methods. Unlike in studies in other regions of the world, correlations between ABLH estimated using MODIS and radiosonde data were weak, implying limited usefulness of MODIS data for determining ABLH. However, the diurnal variation in MODIS-derived ABLH and particulate matter (PM10) was consistent with the expected inverse relationship between PM10 mass concentration and ABLH, and the mean MODIS-derived ABLH values were significantly lower during wet seasons than dry seasons, as expected.
Long-term particulate matter (PM10) measurements were conducted during the period January 2016 to September 2017 at three sites in Uganda (Mbarara, Kyebando, and Rubindi) representing a wide range of urbanization. Spatial, temporal and diurnal variations are assessed in this paper. Particulate matter (PM10) samples were collected for 24-h periods on PTFE filters using a calibrated pump and analyzed gravimetrically to determine the average density. Particulate levels were monitored simultaneously using a light scattering instrument to acquire real time data from which diurnal variations were assessed. The PM10 levels averaged over the sampling period at Mbarara, Kyebando, and Rubindi were 5.8, 8.4, and 6.5 times higher than the WHO annual air quality guideline of 20 µg·m−3, and values exceeded the 24-h mean PM10 guideline of 50 µg·m−3 on 83, 100, and 86% of the sampling days. Higher concentrations were observed during dry seasons at all sites. Seasonal differences were statistically significant at Rubindi and Kyebando. Bimodal peaks were observed in the diurnal analysis with higher morning peaks at Mbarara and Kyebando, which points to the impact of traffic sources, while the higher evening peak at Rubindi points to the influence of dust suspension, roadside cooking and open-air waste burning. Long-term measurement showed unhealthy ambient air in all three locations tested in Uganda, with significant spatial and seasonal differences.