We use sensitive dynamic cantilever magnetometry to measure the magnetic hysteresis of individual magnetic Janus particles. These particles consist of hemispherical caps of magnetic material deposited on micrometer-scale silica spheres. The measurements, combined with corresponding micromagnetic simulations, reveal the magnetic configurations present in these individual curved magnets. In remanence, ferromagnetic Janus particles are found to host a global vortex state with vanishing magnetic moment. In contrast, a remanent onion state with significant moment is recovered by imposing an exchange bias to the system via an additional antiferromagnetic layer in the cap. A robust remanent magnetic moment is crucial for most applications of magnetic Janus particles, in which an external magnetic field actuates their motion.
Nanometer-scale magnetization configurations known as magnetic skyrmions have mostly been studied in cubic chiral helimagnets, in which they are Bloch-type and their axes align along the applied magnetic field. In contrast, the orientation of N\'eel-type skyrmions is locked to the polar axis of the host material's underlying crystal structure. In the lacunar spinels $\mathrm{Ga}{\mathrm{V}}_{4}{\mathrm{S}}_{8}$ and $\mathrm{Ga}{\mathrm{V}}_{4}{\mathrm{Se}}_{8}$, the N\'eel-type skyrmion lattice phase exists for externally applied magnetic fields parallel to this axis and withstands oblique magnetic fields up to some critical angle. Here, we map out the stability of the skyrmion lattice phase in both crystals as a function of field angle and magnitude using dynamic cantilever magnetometry. The measured phase diagrams reproduce the major features predicted by a recent theoretical model, including a reentrant cycloidal phase in $\mathrm{Ga}{\mathrm{V}}_{4}{\mathrm{Se}}_{8}$. Nonetheless, we observe a greater robustness of the skyrmion phase to oblique fields, suggesting possible refinements to the model. Besides identifying transitions between the cycloidal, skyrmion lattice, and ferromagnetic states in the bulk, we measure additional anomalies in $\mathrm{Ga}{\mathrm{V}}_{4}{\mathrm{Se}}_{8}$ and assign them to magnetic states confined to polar structural domain walls.
We report a magnetic state in GaV4Se8 which emerges exclusively in samples with mesoscale polar domains and not in polar mono-domain crystals. It is manifested by a sharp anomaly in the magnetic susceptibility and the magnetic torque, distinct from other anomalies observed also in polar mono-domain samples upon transitions between the cycloidal, the Néel-type skyrmion lattice and the ferromagnetic states. We ascribe this additional transition to the transformation of distinct magnetic textures, confined to polar domain walls (DW), to the ferromagnetic (FM) state. The emergence of these DW-confined magnetic states is likely driven by the mismatch of different spin spirals, hosted by the adjacent domains. A clear anomaly in the magneto-current indicates that the DW-confined magnetic states also have strong contributions to the magnetoelectric response. We expect polar DWs to commonly host such confined magnetic edge states and, thus, offer a fertile ground to explore novel forms of magnetism.