We report second harmonic generation from a titanium indiffused lithium niobate waveguide resonator device whose cavity length is locked to the fundamental pump laser using an on-chip phase modulator. The device remains locked for more than 5 minutes, producing more than 80% of the initial second harmonic power. The stability of the system is seen to be limited by DC-drift, a known effect in many lithium niobate systems that include deposited electrodes. The presented device explores the suitability of waveguide resonators in this platform for use in larger integrated networks.
Efficient sources of many-partite non-classical states are key for the advancement of quantum technologies and for the fundamental testing of quantum mechanics. We demonstrate the generation of time-correlated photon triplets at telecom wavelengths via pulsed cascaded parametric down-conversion in a monolithically integrated source. By detecting the generated states with success probabilities of (6.25 ± 1.09)× 10−11 per pump pulse at injected powers as low as 10 μW, we benchmark the efficiency of the complete system and deduce its high potential for scalability. Our source is unprecedentedly long-term stable, it overcomes interface losses intrinsically due to its monolithic architecture, and the photon-triplet states dominate uncorrelated noise significantly. These results mark crucial progress towards the proliferation of robust, scalable, synchronized and miniaturized quantum technology. © 2018 Optical Society of America OCIS codes: (130.3120) Integrated optics devices; (130.7405) Wavelength conversion devices; (190.4410) Nonlinear optics, parametric processes; (270.4180) Multiphoton processes. References and links 1. D. M. Greenberger, M. A. Horne, A. Shimony, and A. Zeilinger, “Bell’s theorem without inequalities,” Am. J. Phys. 58, 1131–1143 (1990). 2. A. Einstein, B. Podolsky, and N. Rosen, “Can quantum-mechanical description of physical reality be considered complete?,” Phys. Rev. 47, 777–780 (1935). 3. M. Giustina, M. A. M. Versteegh, S. Wengerowsky, J. Handsteiner, A. Hochrainer, K. Phelan, F. Steinlechner, J. Kofler, J.-A. Larsson, C. Abellan, W. Amaya, V. Pruneri, M.W. Mitchell, J. Beyer, T. Gerrits, A. E. Lita, L.K. Shalm, S.W. Nam, T. Scheidl, R. Ursin, B. Wittmann, A. Zeilinger, “A significant-loophole-free test of Bell’s theorem with entangled photons,” Phys. Rev. Lett. 115, 250401 (2015). 4. L. K. Shalm, E. Meyer-Scott, B. G. Christensen, P. Bierhorst, M. A. Wayne, M. J. Stevens, T. Gerrits, S. Glancy, D. R. Hamel, M. S. Allman, K. J. Coakley, S. D. Dyer, C. Hodge, A. E. Lita, V. B. Verma, C. Lambrocco, E. Tortorici, A. L. Migdall, Y. Zhang, D. R. Kumor, W. H. Farr, F. Marsili, M. D. Shaw, J. A. Stern, C. Abellán, W. Amaya, V. Pruneri, T. Jennewein, M. W. Mitchell, P. G. Kwiat, J. C. Bienfang, R. P. Mirin, E. Knill, S. W. Nam, “A strong loophole-free test of local realism,” Phys. Rev. Lett. 115, 250402 (2015). 5. A. Politi, M. Cryan, J. G. Rarity, S. Yu, and J. L. O’Brien, “Silica-on-silicon waveguide quantum circuits,” Science 320, 646 (2008). 6. A. Martin, O. Alibart, M. P. D. Micheli, D. B. Ostrowsky, and S. Tanzilli, “A quantum relay chip based on telecommunication integrated optics technology,” New J. Phys. 14, 025002 (2012). 7. H. Jin, F. M. Liu, P. Xu, J. L. Xia, M. L. Zhong, Y. Yuan, J. W. Zhou, Y. X. Gong, W. Wang, and S. N. Zhu, “On-chip generation and manipulation of entangled photons based on reconfigurable lithium-niobate waveguide circuits,” Phys. Rev. Lett. 113, 103601 (2014). 8. J. W. Silverstone, D. Bonneau, K. Ohira, N. Suzuki, H. Yoshida, N. Iizuka, M. Ezaki, C. M. Natarajan, M. G. Tanner, R. H. Hadfield, V. Zwiller, G. D. Marshall, J. G. Rarity, J. L. O’Brien, and M. G. Thompson, “On-chip quantum interference between silicon photon-pair sources,” Nature Photon. 8, 104–108 (2014). 9. A. Crespi, R. Osellame, R. Ramponi, D. J. Brod, E. F. Galvao, N. Spagnolo, C. Vitelli, E. Maiorino, P. Mataloni, and F. Sciarrino, “Integrated multimode interferometers with arbitrary designs for photonic boson sampling,” Nature Photon. 7, 545–549 (2013). 10. N. Spagnolo, C. Vitelli, M. Bentivegna, D. J. Brod, A. Crespi, F. Flamini, S. Giacomini, G. Milani, R. Ramponi, P. Mataloni, R. Osellame, E. F. Galvao, and F. Sciarrino,“Experimental validation of photonic boson sampling,” Nature Photon. 8, 615–620 (2014). 11. T. E. Keller, M. H. Rubin, Y. Shih, and L.-A. Wu, “Theory of the three-photon entangled state,” Phys. Rev. A 57, 2076–2079 (1998). 12. S. Barz, G. Cronenberg, A. Zeilinger, and P. Walther, “Heralded generation of entangled photon pairs,” Nature Photon. 4, 553–556 (2010). 13. T. Guerreiro, A. Martin, B. Sanguinetti, S. Pelc, J. C. Langrock, M. Fejer, M. N. Gisin, H. Zbinden, N. Sangouard, and T. Thew, R. “Nonlinear interaction between single photons,” Phys. Rev. Lett. 113, 173601 (2014). 14. H. Hübel, D. R. Hamel, A. Fedrizzi, S. Ramelow, K. J. Resch, and T. Jennewein, “Direct generation of photon triplets using cascaded photon-pair sources,” Nature 466, 601–603 (2010). 15. L. K. Shalm, D. R. Hamel, Z. Yan, C. Simon, K. J. Resch, and T. Jennewein, “Three-photon energy-time entanglement,” Nat. Phys. 9, 19–22 (2013). 16. D. R. Hamel, L. K. Shalm, H. Hübel, A. J. Miller, F. Marsili, V. B. Verma, R. P. Mirin, S. W. Nam, K. J. Resch, and T. Jennewein, “Direct generation of three-photon polarization entanglement,” Nature Photon. 8, 801–807 (2014). 17. X. Jia, Z. Yan, Z. Duan, X. Su, H. Wang, C. Xie, and K. Peng, “Experimental realization of three-color entanglement at optical fiber communication and atomic storage wavelengths,” Phys. Rev. Lett. 109, 253604 (2012). 18. Z. Qin, L. Cao, H. Wang, A. M. Marino, W. Zhang, and J. Jing, “Experimental generation of multiple quantum correlated beams from hot rubidium vapor,” Phys. Rev. Lett. 113, 023602 (2014). 19. J. Jing, Z. Qin, L. Cao, H. Wang, A. Marino, and W. Zhang, “Experimental generation of triple quantum correlated beams from cascaded four-wave mixing processes,” in Conference on Lasers and Electro-Optics (CLEO: Science and Innovations), OSA Conference Proceedings of 2014 (Optical Society of America, 2014), p. JTu4A.41. 20. D.-S. Ding, W. Zhang, S. Shi, Z.-Y. Zhou, Y. Li, B.-S. Shi, and G.-C. Guo, “Hybrid-cascaded generation of tripartite telecom photons using an atomic ensemble and a nonlinear waveguide,” Optica 2, 642–645 (2015). 21. M. Khoshnegar, T. Huber, A. Predojevic, D. Dalacu, M. Prilmueller, L. Lapointe, X. Wu, P. Tamarat, B. Lounis, P. Poole, G. Weihs, and H. Majedi, “Bright solid state source of photon triplets,” http://arxiv.org/abs/1510.05898. 22. D. A. Antonosyan, T. V. Gevorgyan, and G. Yu. Kryuchkyan, “Three-photon states in nonlinear crystal superlattices,” Phys. Rev. A 83, 043807 (2011). 23. R. V. Schmidt and I. P. Kaminow, “Metal-diffused optical waveguides in LiNbO3,” Appl. Phys. Lett. 25, 458–460 (1974). 24. K. R. Parameswaran, R. K. Route, J. R. Kurz, R. V. Roussev, M. M. Fejer, and M. Fujimura, “Highly efficient second-harmonic generation in buried waveguides formed by annealed and reverse proton exchange in periodically poled lithium niobate,” Opt. Lett. 27, 179–181 (2002). 25. R. Regener and W. Sohler, “Loss in low-finesse Ti:LiNbO3 optical waveguide resonators,” Appl. Phys. B 36, 143–147 (1985). 26. S. Tanzilli, H. de Riedmatten, H. Tittel, H. Zbinden, P. Baldi, M. De Micheli, D. Ostrowsky, and N. Gisin, “Highly efficient photon-pair source using periodically poled lithium niobate waveguide,” Electron. Lett. 37, 26–28 (2001). 27. S. Krapick, H. Herrmann, V. Quiring, B. Brecht, H. Suche, and C. Silberhorn, “An efficient integrated two-color source for heralded single photons,” New J. Phys. 15, 033010 (2013). 28. S. Krapick, M. S. Stefszky, M. Jachura, B. Brecht, M. Avenhaus, and C. Silberhorn, “Bright integrated photonpair source for practical passive decoy-state quantum key distribution,” Phys. Rev. A 89, 012329 (2014). 29. D. Bonneau, E. Engin, K. Ohira, N. Suzuki, H. Yoshida, N. Iizuka, M. Ezaki, C. M. Natarajan, M. G. Tanner, R. H. Hadfield, S. N. Dorenbos, V. Zwiller, J. L. O’Brien, and M. G. Thompson, “Quantum interference and manipulation of entanglement in silicon wire waveguide quantum circuits,” New J. Phys. 14, 045003 (2012). 30. H. Takesue and K. Shimizu, “Effects of multiple pairs on visibility measurements of entangled photons generated by spontaneous parametric processes,” Opt. Commun. 283, 276 – 287 (2010). 31. S. Krapick and C. Silberhorn, “Analysis of photon triplet generation in pulsed cascaded parametric downconversion sources,” http://arxiv.org/abs/1506.07655. 32. T. Suhara and M. Fujimura, Waveguide Nonlinear-Optic Devices (Springer, 2003), 1st ed. 33. F. Marsili, V. B. Verma, S. J. A., S. Harrington, A. E. Lita, T. Gerrits, I. Vayshenker, B. Baek, M. D. Shaw, R. P. Mirin, and S. W. Nam, “Detecting single infrared photons with 93% system efficiency,” Nature Photon. 7, 210–214 (2013). 34. M. A. Broome, M. P. Almeida, A. Fedrizzi, and A. G. White, “Reducing multi-photon rates in pulsed downconversion by temporal multiplexing,” Opt. Express 19, 22698–22708 (2011). 35. V. B. Verma, B. Korzh, F. Bussières, R. D. Horansky, S. D. Dyer, A. E. Lita, I. Vayshenker, F. Marsili, M. D. Shaw, H. Zbinden, R. P. Mirin, and S. W. Nam, “High-efficiency superconducting nanowire single-photon detectors fabricated from MoSi thin-films,” Opt. Express 23, 33792–33801 (2015) . 36. H. Herrmann, X. Yang, A. Thomas, A. Poppe, W. Sohler, and C. Silberhorn, “Post-selection free, integrated optical source of non-degenerate, polarization entangled photon pairs,” Opt. Express 23, 27981–27991 (2013). 37. G. S. Agarwal and K. Tara, “Nonclassical properties of states generated by the excitations on a coherent state,” Phys. Rev. A 43, 492–497 (1991). 38. E. Schroedinger, “Die gegenwaertige Situation in der Quantenmechanik,” Naturwissenschaften 23, 807–812 (1935). 39. M. Avenhaus, A. Eckstein, P. Mosley, and C. Silberhorn, “Fiber-assisted single-photon spectrograph,” Opt. Lett. 34, 2873–2875 (2009). 40. A. Valencia, M. V. Chekhova, A. Trifonov, and Y. Shih, “Entangled two-photon wave packet in a dispersive medium,” Phys. Rev. Lett. 88, 183601 (2002). 41. G. Brida, M. V. Chekhova, M. Genovese, M. Gramegna, and L. A. Krivitsky, “Dispersion spreading of biphotons in optical fibers and two-photon interference,” Phys. Rev. Lett. 96, 143601 (2006). 42. S.-Y. Baek, O. Kwon, and Y.-H. Kim, “Nonlocal dispersion control of a single-photon waveform,” Phys. Rev. A 78, 013816 (2008).
We present the implementation of a correlation-imaging protocol that exploits both the spatial and spectral correlations of macroscopic twin-beam states generated by parametric downconversion. In particular, the spectral resolution of an imaging spectrometer coupled to an EMCCD camera is used in a proof-of-principle experiment to encrypt and decrypt a simple code to be transmitted between two parties. In order to optimize the trade-off between visibility and resolution, we provide the characterization of the correlation images as a function of the spatiospectral properties of twin beams generated at different pump power values.
We present a single-photon detector providing system detection efficiencies of at least (86.7 ± 0.9) % from 1450 nm to 1640 nm. It comprises bilayer superconducting WSi nanowires in conjunction with all-dielectric structures for optical impedance matching.
We present an alternative approach to the fabrication of highly efficient superconducting nanowire single-photon detectors (SNSPDs) based on tungsten silicide. Using well-established technologies for the deposition of dielectric mirrors and anti-reflection coatings in conjunction with an embedded WSi bilayer photon absorber structure, we fabricated a bandwidth-enhanced detector. It exhibits system detection efficiencies (SDE) higher than $\left(87.1\pm1.3\right)\,\%$ in the range from $1450\,\mathrm{nm}$ to $1640\,\mathrm{nm}$, with a maximum of $\left(92.9\pm1.1\right)\,\%$ at $1515\,\mathrm{nm}$. Our measurements indicate SDE enhancements of up to $\left(18.4\pm1.7\right)\,\%$ over a single-absorber WSi SNSPD. The latter has been optimized for 1550 nm for comparison and exhibits maximum SDE of $\left(93.5\pm1.2\right)\,\%$ at 1555 nm. We emphasize that our technological approach has been tested with, but is not limited to, the wavelengths and absorber material presented here. It could be adapted flexibly for multi-color detector systems from the ultraviolet to the mid-infrared wavelength range. This bears the potential for significant improvements in many current quantum optical experiments and applications as well as for detector commercialization.
Superconducting detectors are now well-established tools for low-light optics, and in particular quantum optics, boasting high-efficiency, fast response and low noise. Similarly, lithium niobate is an important platform for integrated optics given its high second-order nonlinearity, used for high-speed electro-optic modulation and polarization conversion, as well as frequency conversion and sources of quantum light. Combining these technologies addresses the requirements for a single platform capable of generating, manipulating and measuring quantum light in many degrees of freedom, in a compact and potentially scalable manner. We will report on progress integrating tungsten transition-edge sensors (TESs) and amorphous tungsten silicide superconducting nanowire single-photon detectors (SNSPDs) on titanium in-diffused lithium niobate waveguides. The travelling-wave design couples the evanescent field from the waveguides into the superconducting absorber. We will report on simulations and measurements of the absorption, which we can characterize at room temperature prior to cooling down the devices. Independently, we show how the detectors respond to flood illumination, normally incident on the devices, demonstrating their functionality.
Efficient sources of many-partite non-classical states are key for the advancement of quantum technologies and for the fundamental testing of quantum mechanics. We demonstrate the generation of time-correlated photon triplets at telecom wavelengths via pulsed cascaded parametric down-conversion in a monolithically integrated source. By detecting the generated states with success probabilities of (6.25 ± 1.09) × 10(-11) per pump pulse at injected powers as low as 10 μW, we benchmark the efficiency of the complete system and deduce its high potential for scalability. Our source is unprecedentedly long-term stable, it overcomes interface losses intrinsically due to its monolithic architecture, and the photon-triplet states dominate uncorrelated noise significantly. These results mark crucial progress towards the proliferation of robust, scalable, synchronized and miniaturized quantum technology.
The practical prospect of quantum communication and information processing relies on sophisticated single-photon pairs, which feature a controllable waveform, narrow spectrum, excellent purity, fiber compatibility, and miniaturized design. For practical realizations, stable, miniaturized, low-cost devices are required. Sources with one or some of the above characteristics have already been demonstrated, but it is quite challenging to obtain a source with all of the described characteristics simultaneously. Here we report on an integrated single-longitudinal-mode, non-degenerate, narrowband photon pair source that exhibits all the requirements needed for quantum applications. The device is composed of a periodically poled, Ti-indiffused, lithium niobate waveguide with high reflective dielectric mirror coatings deposited on the waveguide end-faces. Photon pairs with wavelengths around 890 and 1320 nm are generated via type II phase-matched parametric downconversion (PDC). Clustering in this dispersive cavity restricts the whole conversion spectrum to one single-longitudinal mode in a single cluster, yielding a narrow bandwidth of only 60 MHz. The high conversion efficiency in the waveguide, together with the spectral clustering in the doubly resonant waveguide, leads to a high brightness of 3 x 10(4) pairs/(s mW MHz). This source exhibits prominent single-longitudinal-mode purity and remarkable temporal shaping capability. In particular, due to temporal broadening, we can observe that the coherence time of the two-photon component of the PDC state is actually longer than that of the single-photon states. The miniaturized monolithic design enables this source to have various fiber communication applications.
We present a miniaturized integrated waveguide source providing 11.3±0.7 photon-triplet states per hour, measured with off-the-shelf components. By double-stage heralding and integration times of 83 hours, we achieve statistical significance of more than 27 σ.
The measurement of light characteristics at the single- and few photon level plays a key role in many quantum optics applications. Often photodetection is preceded with the transmission of quantum light over long distances in optical fibers with their low loss window near 1550nm. Nonetheless, the detection of the photonic states at telecommunication wavelengths via avalanche photodetectors has long been facing severe restrictions. Only recently, demonstrations of the first free-running detector techniques in the telecommunication band have lifted the demand of synchronizing the signal with the detector. Moreover, moderate cooling is required to gain single-photon sensitivity with these detectors. Here we implement a liquid-nitrogen cooled negative-feedback avalanche diode (NFAD) at telecommunication wavelengths and investigate the properties of this highly flexible, free-running single-photon sensitive detector. Our realization of cooling provides a large range of stable operating temperatures and has advantages over the relatively bulky commercial refrigerators that have been used before. We determine the region of NFAD working parameters most suitable for single-photon sensitive detection enabling a direct plug-in of our detector to a true photon counting task.
We analyze the generation rates and preparation fidelities of photon triplet states in pulsed cascaded parametric down-conversion (PDC) under realistic experimental circumstances. As a model system, we assume a monolithically integrated device with negligible interface loss between the two consecutive PDC stages. We model the secondary down-conversion process in terms of a lossy channel and provide a detailed analysis of noise contributions. Taking variable pump powers into account, we estimate the impact of higher-order photon contributions and conversion processes on the achievable coincidence probabilities. At mean photon numbers of ⟨ m⟩∼0.25 photons per pulse behind the first PDC stage, we expect around 4.0 genuine photon triplets per hour. Additionally, we discuss fundamental limitations of our model system as well as feasible improvements to the detectable photon triplet rate.
We report on a bright, nondegenerate type-I parametric down-conversion source, which is well suited for passive decoy-state quantum key distribution. We show the photon-number-resolved analysis over a broad range of pump powers and we prove heralded higher-order n-photon states up to n = 4. The inferred photon click statistics exhibit excellent agreements to the theoretical predictions. From our measurement results we conclude that our source meets the requirements to avert photon-number-splitting attacks.
We implemented a compact integrated non-degenerate source which comprises a periodically poled waveguide with highly reflective dielectric mirror coatings to obtain narrowband photon pairs based on type II parametric down-conversion. Our engineered source exploits clustering in the dispersive cavity to restrict the conversion to a predominantly single mode operation with a narrowband linewidth and high spectral purity. The miniaturized monolithic design makes our source a versatile device for various applications in quantum communication and information processing.
We report on an integrated non-degenerate narrowband photon pair source produced at 890 nm and 1320nm via type II parametric down-conversion in a periodically poled waveguide with high-reflective dielectric mirrors deposited on the waveguide end faces. The conversion spectrum consists of three clusters and only 3 to 4 longitudinal modes with about 150 MHz bandwidth in each cluster. The high conversion efficiency in the waveguide, together with the spectral clustering in the double resonator, leads to a high brightness of 3×10^3pairs/(s·mW·MHz). The compact and rugged monolithic design makes the source a versatile device for various applications in quantum communication.
We present a pulsed and integrated, highly non-degenerate parametric down-conversion (PDC) source of heralded single photons at telecom wavelengths, paired with heralding photons around 800 nm. The active PDC section is combined with a passive, integrated wavelength division demultiplexer on-chip, which allows for the spatial separation of signal and idler photons with efficiencies of more than 96.5%, as well as with multi-band reflection and anti-reflection coatings which facilitate low incoupling losses and a pump suppression at the output of the device of more than 99%. Our device is capable of preparing single photons with efficiencies of 60% with a coincidences-to-accidentals ratio exceeding 7400. Likewise, it shows practically no significant background noise compared to continuous wave realizations. For low pump powers, we measure a conditioned second-order correlation function of g(2) = 3.8 × 10−3, which proves almost pure single-photon generation. In addition, our source can feature a high brightness of 〈npulse〉 = 0.24 generated photon pairs per pump pulse at pump power levels below 100 μW. The high quality of the pulsed PDC process in conjunction with the integration of highly efficient passive elements makes our device a promising candidate for future quantum networking applications, where an efficient miniaturization plays a crucial role.
Summary form only given. Recent progress in quantum information processing has highlighted the benefits of integrated optic devices for quantum applications (e.g.[l]). The miniaturization of systems with increased complexity drastically reduces the required space and paves the way for future commercialization.In the past five years, several groups have demonstrated promising approaches to achieve quantum interference and photonic gates on-chip (e.g.[2]). However, in all of these experiments the preparation of the photon pairs has been performed outside the integrated devices employing bulk crystal parametric down-conversion (PDC) sources, while the efficient coupling between these sources and the integrated circuit remains as a bottleneck for the design of systems with increasing complexity. On the other hand remarkable efforts have been devoted to the development of integrated PDC sources for photon pair generation inside channel waveguides [3]. The main benefits of guided-wave PDC processes include high conversion efficiencies and spatial mode control. We combine the prospects of an efficient type-I PDC source based on Titanium-indiffused periodically poled Z-cut Lithium Niobate waveguides (Ti:PPLN) with a passive wavelength division demultiplexing coupler on-chip, shown in Figure 1. The coupler allows for excellent spatial separation generated photon pairs. The non-degenerate decay of pump photons at 532 nm into signal and idler photons provides us with a photon pair at wavelengths of 1575 nm and 800 nm, respectively. Thus low-loss fiber transmission of the prepared states at 1575 nm can be accomplished on the one hand, while on the other hand efficient heralding of conditioned states can be implemented with off-the-shelf silicon-based detectors. The quality and efficiency of our source was improved by the deposition of endface-coatings. This allows for the efficient launching of pump light into the waveguide and it simultaneously provides a close-toperfect tran- mission of signal and idler at the output of our source, reflecting the pump light by more than 99%. In conditioned coincidence measurements in the picosecond pulsed regime we achieved heralding of single photons with almost no influence of background radiation, expressed by high coincidences-toaccidentals ratios up to CAR > 7400. The preparation exceeded 60% of efficiency in the low pump power regime, accompanied with ultra-low second-order correlation functions of g(2) (0) <; 4.10-3. These figures of merit in conjunction with the integration of active and passive elements make our source a candidate for a basic building block in more complex and miniaturized quantum network realizations in the future.