Measurements of the longitudinal and transverse spin relaxation times of holes in an ensemble of vertically tunnel‐coupled self‐assembled InAs/InAlGaAs quantum dots (QDs), emitting in the telecom spectral range, are reported. The spin coherence is determined using the spin mode‐locking method in the inhomogeneous ensemble of QDs. Modeling the signal allows us to extract the hole spin coherence time to be in the range of μs. The longitudinal spin relaxation time μs is measured using the spin inertia method. The parameters investigated allow us to suggest that the main relaxation mechanism at low magnetic fields is related to the electron–hole spin exchange.
Hybrid ferromagnet-semiconductor systems possess new outstanding properties, which emerge when bringing magnetic and semiconductor materials into contact. In such structures, the long-range magnetic proximity effect couples the spin systems of the ferromagnet and semiconductor on distances exceeding the carrier wave function overlap. The effect is due to the effective p-d exchange interaction of acceptor-bound holes in the quantum well with d-electrons of the ferromagnet. This indirect interaction is established via the phononic Stark effect mediated by the chiral phonons. Here, we demonstrate that the long-range magnetic proximity effect is universal and observed in hybrid structures with diverse magnetic components and potential barriers of various thicknesses and compositions. We study hybrid structures consisting of a semimetal (magnetite Fe3O4) or dielectric (spinel NiFe2O4) ferromagnet and a CdTe quantum well separated by a nonmagnetic (Cd,Mg)Te barrier. The proximity effect is manifested in the circular polarization of the photoluminescence corresponding to the recombination of photoexcited electrons with holes bound to shallow acceptors in the quantum well induced by magnetite or spinel itself, in contrast to interface ferromagnet in case of metal-based hybrid systems. A nontrivial dynamics of the proximity effect is observed in the studied structures due to recombination-induced dynamic polarization of electrons in the quantum well. It enables the determination of the exchange constant Δexch ≈ 70 μeV in a magnetite-based structure. The universal origin of the long-range exchange interaction along with the possibility of its electrical control offers prospects for the development of low-voltage spintronic devices compatible with existing solid-state electronics.
Quantum measurement back action is fundamentally unavoidable when manipulating electron spins. Here we demonstrate that this back action can be efficiently exploited to tune the spin relaxation of localized electrons induced by the hyperfine interaction. In optical pump-probe experiments, powerful probe pulses suppress the spin relaxation of electrons on Si donors in an InGaAs epilayer due to the quantum Zeno effect. By contrast, an increase of the probe power leads to a speed up of the spin relaxation for electrons in InGaAs quantum dots due to the quantum anti-Zeno effect. The microscopic description shows that the transition between the two regimes occurs when the spin dephasing time is comparable to the probe pulse repetition period.
The effective g factor of holes is measured in modulation-doped ZnSe/(Zn,Mg)(S,Se) quantum wells and from surface-state p-doped CdTe/(Cd,Mg)Te quantum wells by time-resolved pump-probe Kerr rotation. The measurements are performed at a temperature of 1.7 K and in magnetic fields up to 5 T applied in the Voigt geometry with orientation perpendicular to the quantum-well growth axis. The absolute value of the in-plane hole g factor increases with growing magnetic field in both studied heterostructures. A theoretical model is developed that considers the influence of magnetic field and interface mixing of heavy-hole and light-hole states on the g factor. The model results are in good agreement with the experimental data.
We demonstrate the realization of the resonant spin amplification (RSA) effect in Faraday geometry where a magnetic field is applied parallel to the optically induced spin polarization so that no RSA is expected. However, model considerations predict that it can be realized for a central spin interacting with a fluctuating spin environment. As a demonstrator, we choose an ensemble of singly-charged (In,Ga)As/GaAs quantum dots, where the resident electron spins interact with the surrounding nuclear spins. The observation of RSA in Faraday geometry requires intense pump pulses with a high repetition rate and can be enhanced by means of the spin-inertia effect. Potentially, it provides the most direct and reliable tool to measure the longitudinal g factor of the charge carriers.