Spectral manipulation of single photons as an essential quantum technology provides a feasible method for highly efficient quantum interconnects between quantum systems with different transition linewidths via flying photons, which expands the capabilities of quantum networks. In this Letter, we propose a scalable scheme based on side-end cavity and time-dependent phase modulation, which allows the spectral compression of single photons by hundreds of times and even more, with an efficiency higher than active spectrum filtering. In addition, the achievable frequency shifts of single photons can reach hundreds of gigahertz. These techniques allow the implementation of a high-efficiency quantum interface between single photons and atomic quantum memories, as well as high-visibility quantum interference between two independent single photons. Our scheme opens up a way for hybrid quantum networks involving quantum systems with different transition linewidths.

Semiconductor quantum dots (QDs) coupled with optical microcavities provide an excellent platform for generating high-performance single-photon sources. However, the current microcavity structures are difficult to solve the tradeoff between single-photon purity and indistinguishability without additional filtering, due to challenges in suppressing broad phonon sideband spectrum and two-photon emission in the practical experiments. To address these issues, we have developed a novel asymmetric microcavity that supports two nondegenerate polarized modes, both resonant with a single quantum dot. One cavity mode is broadband and is used for excitation to reduce two-photon emission intensity, while the other is narrowband and is used for collection to enhance the indistinguishability of single-photon sources. This asymmetric microcavity also has the ability to overcome at least half of the photon efficiency loss under polarization filtering. Moreover, our model has employed an excitation pulse that resonates with cavity modes eliminating spectral distortion of intracavity fields, and efficiently achieving deterministic population inversion of QDs compared to an elliptical cavity. Our scheme paves the way to develop the excellent performance single-photon sources with higher brightness, near-unity purity, and indistinguishability without any additional filtering in practical experiments.

To fully exploit the potential of quantum technologies, quantum networks are needed to link different systems, enhancing applications in computing, cryptography and metrology. Central to these networks are quantum relays that can facilitate long-distance entanglement distribution and quantum communication. In this work, we present a modular and scalable quantum relay architecture using a high-quality single-photon source. The proposed network incorporates three untrusted intermediate nodes and is capable of a repetition rate of 304.52 MHz. We use a measurement-device-independent protocol to demonstrate secure key establishment over fibres covering up to 300 km. This study highlights the potential of single-photon sources in quantum relays to enhance information transmission, expand network coverage and improve deployment flexibility, with promising applications in future quantum networks.

The emergence of quantum mechanics and general relativity has transformed our understanding of the natural world significantly. However, integrating these two theories presents immense challenges, and their interplay remains untested. Recent theoretical studies suggest that the single-photon interference covering huge space can effectively probe the interface between quantum mechanics and general relativity. We developed an alternative design using unbalanced Michelson interferometers to address this and validated its feasibility over an 8.4 km free-space channel. Using a high-brightness single-photon source based on quantum dots, we demonstrated single-photon interference along this long-distance baseline. We achieved a phase measurement precision of 16.2 mrad, which satisfied the measurement requirements for a gravitational redshift at the geosynchronous orbit by 5 times the standard deviation. Our results confirm the feasibility of the single-photon version of the Colella-Overhauser-Werner experiment for testing the quantum effects in curved spacetime.

In the quest to build general-purpose photonic quantum computers, fusion-based quantum computation has risen to prominence as a promising strategy. This model allows a ballistic construction of large cluster states which are universal for quantum computation, in a scalable and loss-tolerant way without feed-forward, by fusing many small n-photon entangled resource states. However, a key obstacle to this architecture lies in efficiently generating the required essential resource states on photonic chips. One such critical seed state that has not yet been achieved is the heralded three-photon Greenberger-Horne-Zeilinger (3-GHZ) state. Here, we address this elementary resource gap, by reporting the first experimental realization of a heralded dual-rail encoded 3-GHZ state. Our implementation employs a low-loss and fully programmable photonic chip that manipulates six indistinguishable single photons of wavelengths in the telecommunication regime. Conditional on the heralding detection, we obtain the desired 3-GHZ state with a fidelity 0.573+-0.024. Our work marks an important step for the future fault-tolerant photonic quantum computing, leading to the acceleration of building a large-scale optical quantum computer.

In the quest to realize a scalable quantum network, semiconductor quantum dots (QDs) offer distinct advantages, including high single-photon efficiency and indistinguishability, high repetition rate (tens of gigahertz with Purcell enhancement), interconnectivity with spin qubits, and a scalable on-chip platform. However, in the past two decades, the visibility of quantum interference between independent QDs rarely went beyond the classical limit of 50%, and the distances were limited from a few meters to kilometers. Here, we report quantum interference between two single photons from independent QDs separated by a 302 km optical fiber. The single photons are generated from resonantly driven single QDs deterministically coupled to microcavities. Quantum frequency conversions are used to eliminate the QD inhomogeneity and shift the emission wavelength to the telecommunication band. The observed interference visibility is 0.67 +/- 0.02 (0.93 +/- 0.04) without (with) temporal filtering. Feasible improvements can further extend the distance to similar to 600 km. Our work represents a key step to long-distance solid-state quantum networks.

Heralded entangling quantum gates are an essential element for the implementation of large-scale optical quantum computation. Yet, the experimental demonstration of genuine heralded entangling gates with free-flying output photons in linear optical system, was hindered by the intrinsically probabilistic source and double-pair emission in parametric down-conversion. Here, by using an on-demand single-photon source based on a semiconductor quantum dot embedded in a micropillar cavity, we demonstrate a heralded controlled-NOT (CNOT) operation between two single photons for the first time. To characterize the performance of the CNOT gate, we estimate its average quantum gate fidelity of (87.8±1.2)%. As an application, we generated event-ready Bell states with a fidelity of (83.4±2.4)%. Our results are an important step towards the development of photon-photon quantum logic gates.

Verification of a quantum advantage in the presence of noise is a key open problem in the study of near-term quantum devices. In this work, we show how to assess the quality of photonic interference in a linear optical quantum device (boson sampler) by using a maximum likelihood method to measure the strength at which various noise sources are present in the experiment. This allows us to use a sparse set of samples to test whether a given boson-sampling experiment meets known upper bounds on the level of noise permissible to demonstrate a quantum advantage. Furthermore, this method allows us to monitor the evolution of noise in real time, creating a valuable diagnostic tool. Finally, we observe that sources of noise in the experiment compound, meaning that the observed value of the mutual photon indistinguishability, which is the main imperfection in our study, is an effective value taking into account all sources of error in the experiment.

In the quest to realize a scalable quantum network, semiconductor quantum dots (QDs) offer distinct advantages including high single-photon efficiency and indistinguishability, high repetition rate (tens of GHz with Purcell enhancement), interconnectivity with spin qubits, and a scalable on-chip platform. However, in the past two decades, the visibility of quantum interference between independent QDs rarely went beyond the classical limit of 50% and the distances were limited from a few meters to kilometers. Here, we report quantum interference between two single photons from independent QDs separated by 302 km optical fiber. The single photons are generated from resonantly driven single QDs deterministically coupled to microcavities. Quantum frequency conversions are used to eliminate the QD inhomogeneity and shift the emission wavelength to the telecommunication band. The observed interference visibility is 0.67\pm0.02 (0.93\pm0.04) without (with) temporal filtering. Feasible improvements can further extend the distance to ~600 km. Our work represents a key step to long-distance solid-state quantum networks.

Intensity squeezing-i.e., photon number fluctuations below the shot-noise limit-is a fundamental aspect of quantum optics and has wide applications in quantum metrology. It was predicted in 1979 that intensity squeezing could be observed in resonance fluorescence from a two-level quantum system. However, its experimental observation in solid states was hindered by inefficiencies in generating, collecting, and detecting resonance fluorescence. Here, we report the intensity squeezing in a single-mode fiber-coupled resonance fluorescence single-photon source based on a quantum dot-micropillar system. We detect pulsed single-photon streams with 22.6% system efficiency, which show sub-shot-noise intensity fluctuation with an intensity squeezing of 0.59 dB. We estimate a corrected squeezing of 3.29 dB at the first lens. The observed intensity squeezing provides the last piece of the fundamental picture of resonance fluorescence, which can be used as a new standard for optical radiation and in scalable quantum metrology with indistinguishable single photons.

We show a method for assessing the quality of photonic quantum interference (boson sampling) in the regime of fewer samples than outcomes. We present an error budget for a state of the art boson sampler.

Quantum computing experiments are moving into a new realm of increasing size and complexity, with the short-term goal of demonstrating an advantage over classical computers. Boson sampling is a promising platform for such a goal; however, the number of detected single photons is up to five so far, limiting these small-scale implementations to a proof-of-principle stage. Here, we develop solid-state sources of highly efficient, pure, and indistinguishable single photons and 3D integration of ultralow-loss optical circuits. We perform experiments with 20 pure single photons fed into a 60-mode interferometer. In the output, we detect up to 14 photons and sample over Hilbert spaces with a size up to 3.7×10^{14}, over 10 orders of magnitude larger than all previous experiments, which for the first time enters into a genuine sampling regime where it becomes impossible to exhaust all possible output combinations. The results are validated against distinguishable samplers and uniform samplers with a confidence level of 99.9%.

Quantum computing experiments are moving into a new realm of increasing size and complexity, with the short-term goal of demonstrating an advantage over classical computers. Boson sampling is a promising platform for such a goal, however, the number of involved single photons was up to five so far, limiting these small-scale implementations to a proof-of-principle stage. Here, we develop solid-state sources of highly efficient, pure and indistinguishable single photons, and 3D integration of ultra-low-loss optical circuits. We perform an experiment with 20 single photons fed into a 60-mode interferometer, and, in its output, sample over Hilbert spaces with a size of 10^14 -over ten orders of magnitude larger than all previous experiments. The results are validated against distinguishable samplers and uniform samplers with a confidence level of 99.9