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PLA group research is focused on reactive and unusual complexes of the rare earths and actinides. We use these to make new catalysts for difficult transformations such as hydrocarbon C-H bond functionalisation and conversions of abundant small molecules such as dinitrogen and carbon oxygenates. The most unusual metal compounds also teach us about electronic structure and bonding in these poorly-understood, yet often earth-abundant heavy elements. This is important to help us exploit the technology critical rare earths, e.g. in quantum science applications, and for the safe stewardship of our nuclear waste legacies. Our labs have state-of-the-art equipment for the synthesis of highly air-sensitive complexes, and the study of their reactivity towards small, inert molecules. We combine anaerobic, organometallic techniques with new methodologies to control f-block cation reactivity, elicit unprecedented behaviours, and isolate molecules with previously unseen electronic structures and reactivities from across the f-block, generating key advances in our understanding of f-block bonding and reactivity to feed into each of these areas.
PLA group research is focused on reactive and unusual complexes of the rare earths and actinides. We use these to make new catalysts for difficult transformations such as hydrocarbon C-H bond functionalisation and conversions of abundant small molecules such as dinitrogen and carbon oxygenates. The most unusual metal compounds also teach us about electronic structure and bonding in these poorly-understood, yet often earth-abundant heavy elements. This is important to help us exploit the technology critical rare earths, e.g. in quantum science applications, and for the safe stewardship of our nuclear waste legacies. Our labs have state-of-the-art equipment for the synthesis of highly air-sensitive complexes, and the study of their reactivity towards small, inert molecules. We combine anaerobic, organometallic techniques with new methodologies to control f-block cation reactivity, elicit unprecedented behaviours, and isolate molecules with previously unseen electronic structures and reactivities from across the f-block, generating key advances in our understanding of f-block bonding and reactivity to feed into each of these areas.
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Paul Ewing, Pankaj Mahji, Callum Prentice,Claire M Young, Karlotta van Rees,Polly Louise Arnold,Eli Zysman-Colman, Andrew D Smith
crossref(2024)
Ryte Rutkauskaite,Xiaobin Zhang,Adam W. Woodward,Yanlin Liu, Gabriel Herrera,Jamie Purkis,Sean D. Woodall,Mark Sarsfield,Georg Schreckenbach, Louise S. Natrajan,Polly L. Arnold
CHEMICAL SCIENCEno. 18 (2024): 6965-6978
Paul Ewing, Pankaj Mahji, Callum Prentice,Claire M Young, Karlotta van Rees,Polly Louise Arnold,Eli Zysman-Colman, Andrew D Smith
crossref(2024)
Anthony Wong,Francis Y.T. Lam, Matthew Hernandez, Jaden Lara,T. Michael Trinh,Rory P. Kelly,Tatsumi Ochiai,Guodong Rao,R. David Britt,Nikolas Kaltsoyannis,Polly L. Arnold
Chem Catalysispp.100964, (2024)
Paul Ewing, Pankaj Mahji, Callum Prentice,Claire M Young, Karlotta van Rees,Polly Louise Arnold,Eli Zysman-Colman, Andrew D Smith
Chemical Science (2024)
Amy E. Kynman, Stella Christodoulou,Erik T. Ouellette, Appie Peterson, Sheridon N. Kelly,Laurent Maron,Polly Arnold
CHEMICAL COMMUNICATIONSno. 73 (2023): 10924-10927
COMMUNICATIONS CHEMISTRYno. 1 (2023)
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