Single-component molecular conductor [Pt(dmdt) 2 ]-a three-dimensional ambient-pressure molecular Dirac electron system.

Biao Zhou,Shoji Ishibashi, Tatsuru Ishii,Takahiko Sekine,Ryosuke Takehara,Kazuya Miyagawa,Kazushi Kanoda,Eiji Nishibori,Akiko Kobayashi

CHEMICAL COMMUNICATIONS（2019）

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摘要

The single-component molecular conductor [Pt(dmdt)(2)] is a sought-after ambient-pressure molecular Dirac electron system, which exhibits a high temperature-insensitive conductivity and temperature-dependent magnetic susceptibility nearly vanishing below 120 K. First-principles DFT calculations reveal that Dirac cones emerge along the a* direction, and form Dirac nodal lines.

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