The 35Cl(n, p)35S reaction plays a key role in neutron dosimetry for Boron Neutron Capture Therapy, in the synthesis of the isotope 36S, whose astrophysical origin remains unresolved, and in the design of next-generation molten-salt reactors. Its relevance has motivated its inclusion in the High Priority Request List (HPRL) of NEA. The goal of this work is to determine the 35Cl(n, p)35S cross-section from thermal energy to 120 keV for the first time ever in a single measurement, thus reducing systematic uncertainties related to the normalization to the thermal value. This had been a subject of concern in previous evaluations of this reaction. We made use of the Time-of-Flight technique with microMEGAS detectors at Experimental Area 2 (EAR-2) of n_TOF facility at CERN. The 10B (n, α ) 7Li and 235U(n, f) reactions were used as references. Rutherford Back-scattering Spectrometry was performed at Centro Nacional de Aceleradores (CNA) in Sevilla, in order to accurately determine the masses of the irradiated samples. We obtained a thermal cross-section of 0.470 ± 0.009 barns. The 1/v energy dependence of the cross-section is observed up to the first resonance at 0.398 keV, the resonances up to 120 keV are analyzed and resonance parameters extracted using SAMMY. Maxwellian Averaged Cross-Section (MACS) was calculated for k_B T from 1 to 100 keV, and lower values compared to estimations from ENDF were found, e.g., 1.07 ± 0.20 mb at k_BT=30 keV. The thermal cross-section and first two resonances are in agreement with the latest evaluation in ENDF/B-VIII.1, while remarkably lower resonance strengths were found for high energy resonances.

Neutron capture reactions provide essential nuclear physics input for modeling the synthesis of heavy elements in stars. The growing precision of stellar spectroscopy and isotopic measurements in presolar SiC grains now demands cross sections with improved accuracy over the full energy range, and access to unstable nuclei relevant to slow (s-) process branchings and the intermediate (i-) process. This article reviews recent progress in direct neutron capture measurements, focusing on time-of-flight (TOF) experiments at CERN n_TOF and complementary activation techniques. Substantial advances have been achieved for stable s-only and bottleneck isotopes, significantly improving constraints on s-process models. In parallel, the combination of high instantaneous neutron fluxes and advanced detector systems has facilitated first-time neutron capture measurements on several radioactive branching-point nuclei. Feasibility studies, however, reveal current limitations related to sample availability, background conditions, and restricted energy coverage. In this context, the complementarity between TOF and activation emerges as a central strategy. Future developments, including high-flux facilities and novel inverse kinematics experiments in ion storage rings, are expected to extend the boundaries of neutron capture measurements, overcoming current limitations and helping unlock new frontiers in our understanding of stellar nucleosynthesis.

The neutron capture cross section of 64Ni is an important parameter in nuclear astrophysics that is needed to accurately simulate stellar nucleosynthesis and validate stellar models. 64Ni is among the seeds of the s-process and its capture cross section has been found to have an important effect on the predicted abundances of many nuclei synthesized in Asymptotic Giant Branch (AGB) and massive stars. Despite its relevance, the measurements of the 64Ni(n,γ) available in the literature are scarce and discrepant. For this reason, a new accurate time-of-flight measurement has been performed at the n_TOF facility at CERN, taking advantage of its high instantaneous neutron flux, and using a highly enriched 64Ni sample. The first preliminary results show important discrepancies with respect to the cross sections recommended in the most recent releases of the evaluated nuclear data libraries. In particular, a large resonance reported at 9.52 keV is not observed. As a consequence, a significant reduction in the Maxwellian-Averaged Cross Section (MACS) obtained from evaluated data libraries in the 5–25 keV thermal energy region is expected.

Background: The ^35Cl(n, p)^35S reaction is of special interest in three different applications. First, in Boron Neutron Capture Therapy due to the presence of ^35Cl in brain and skin tissue. Second, it is involved in the creation of ^36S, whose astrophysical origin remains unresolved. Third, in the designing of fast nuclear reactors of new generation based on molten salts. Purpose: To measure the ^35Cl(n, p)^35S cross-section from thermal energy to 120 keV, determine the resonance parameters in this range and Maxwellian Averaged Cross-Section (MACS). Method: We made use of the Time-of-Flight technique with microMEGAS detectors at Experimental Area 2 (EAR-2) of n_TOF facility at CERN. The ^10B(n, α)^7Li and ^235U(n, f) reactions were used as references. Rutherford Back-scattering Spectrometry technique was performed at Centro Nacional de Aceleradores (CNA) in Sevilla, in order to accurately determine the masses of the irradiated samples. Results: We obtain a thermal cross-section of 0.470 ± 0.009 barns. The 1/v energy dependence of the cross-section is observed up to the first resonance at 0.398 keV, the resonances up to 120 keV are analyzed and MACS calculated for k_B T from 1 to 100 keV. Conclusions: The ^35Cl(n, p)^35S cross-section has been obtained over a wide energy range for the first time, with high accuracy across the aforementioned range. The thermal cross-section and first two resonances are in agreement with latest evaluation in ENDF/B-VIII.1, while lower resonance strength was found for high energy resonances. These data are used to calculate the MACS for different k_B T.

This Eur. Phys. J. A volume 58 is dedicated to the life and work of Dr. Franz Käppeler from Karlsruhe Institute for Technology (KIT) who died on 20 November 2021, after a short illness. He was one of the leading experimentalists in the field of experimental nuclear astrophysics in Germany and worldwide for decades. Many of the authors of this volume knew Franz personally and many others were directly or indirectly inspired by his work and personality. All references in this introductory article refer to publications in this volume, not necessary to actual work by Dr. Käppeler.

The theoretical description of the 56Fe neutron induced reaction cross sections is the subject of many studies within the nuclear data community. Based on these studies, issues were discovered in the evaluated cross sections of the 56Fe(n,γ) reaction. Those issues were addressed by implementing changes in the ENDF/B-VIII.0 evaluation. The aim of this work is to provide a physical interpretation for these changes by exploring the direct radiative capture mechanism for 56Fe. For the calculations, a dedicated code (PDIX) was utilized. The first results of the direct capture cross section of 56Fe are presented and discussed.

The experimental setup of the new measurement of 239Pu fission and capture cross-section in the n_TOF time-of-flight facility at CERN is presented. The measurement aims to address the needs and demands of nuclear data users. The experiment incorporates an innovative fast Fission Fragment Detector and the n_TOF Total Absorption Calorimeter, enabling the implementation of the fission tagging technique. Preliminary results exhibit the robust performance of the detector systems, along with the high quality of the new 239Pu samples. These samples were exclusively produced for this measurement by the European Commission’s Joint Research Centre in Geel.

The isotopic abundances in presolar SiC grains of AGB origin provide important and precise constraints to those star nucleosynthesis models. By comparing the values of the s-element abundances resulting from calculations with the ones measured in these dust grains, it turns out that new measurements of weak-interaction rates in ionized plasmas, as well as of neutron-capture cross sections, are needed, especially in the region near the neutron magic numbers 50 and 82.

The increasing worldwide interest in Lead-cooled Fast Reactors (LFRs) substantiates the need to validate the analytical codes and methods used to support their design. For neutronic analyses, this is chiefly reflected in assessing the impact of nuclear data uncertainties on the integral and local parameters resulting from such analyses. The aim of refining nuclear data moves continuous efforts for more accurate measurements, be them differential or integral, for which adequate facilities are required. The availability at the ENEA's Casaccia research center of a fast source reactor – RSV TAPIRO – provides a unique opportunity to perform new integral experiments in support of fast reactors, including LFRs, owing to the well-characterized neutron spectrum of the thermal column. A series of experiments has been envisaged, dealing with the use of Lead in a reactor. The experiments concern the propagation of neutrons through blocks of materials representing relevant elements of a reactor core, and ranging from pure Lead to mixtures reproducing portions of the reflector and shield in LFRs. The paper is focused on the feasibility study of some of these experiments in which Lead and mixture blocks are inserted in the so-called thermal column of the RSV TAPIRO reactor and irradiated by the neutron flux emerging from the Copper reflector surrounding the reactor core.

We show examples of the impact of the Maxwellian averaged capture cross sections determined at n_TOF over the past 20 years on AGB stellar nucleosynthesis models. In particular, we developed an automated procedure to derive MACSs from evaluated data libraries, which are subsequently used as input to stellar models computed by means of the FuNS code. In this contribution, we present a number of s-process abundances obtained using different data libraries as input to stellar models, with a focus on the role of n_TOF data.

Neutron cross section measurements are often made relative to a neutron cross section standard. Thus, the accuracy of the neutron standards determines the best possible accuracy of the neutron measurements. The 235U(n,f) cross section is widely used as reference, while it is considered a standard at thermal point and between 0.15 to 200 MeV. For this reason, additional cross section data for the 235U(n,f) reaction are useful in order to improve the accuracy and to extend the energy range of the standard. In this work, preliminary results of the measurement of the 235U(n,f) cross-section relative to the standard 10B(n,a) reaction are presented. The high accuracy measurement was performed at the experimental area EAR-1 of the n_TOF facility at CERN, aiming at covering the energy range from the thermal region up to approximately 100 keV. The samples were produced at JRC-Geel in Belgium, while the experimental setup was based on Micromegas detectors.

The n_TOF facility at CERN is a neutron Time-Of-Flight facility based on a spallation neutron source. During the Second Long Shutdown (LS2) , a new experimental zone was designed and delivered. This new experimental area -the NEAR station - is located very close to the lead spallation target, at a distance of just ~3m. In this way, the high luminosity of the n_TOF neutron spallation source can be fully exploited. Towards the characterization of the new experimental area as well for the benchmarking of the performed simulations, the multi-foil activation measurement will be implemented. Eleven threshold and seven capture reference reactions will be utilized for the unfolding of the NEAR neutron beam energy spectrum that stretches from the meV to the GeV region.

Theoretical predictions as well as experiments performed at storage rings have shown that the lifetimes of β-radionuclides can change significantly as a function of the ionization state. In this paper we describe an innovative approach, based on the use of a compact plasma trap to emulate selected stellar-like conditions. It has been proposed within the PANDORA project (Plasmas for Astrophysics, Nuclear Decay Observation and Radiation for Archaeometry) with the aim to measure, for the first time in plasma, nuclear β-decay rates of radionuclides involved in nuclear-astrophysics processes. To achieve this task, a compact magnetic plasma trap has been designed to reach the needed plasma densities, temperatures, and charge-states distributions. A multi-diagnostic setup will monitor, on-line, the plasma parameters, which will be correlated with the decay rate of the radionuclides. The latter will be measured through the detection of the γ-rays emitted by the excited daughter nuclei following the β-decay. An array of 14 HPGe detectors placed around the trap will be used to detect the emitted γ-rays. For the first experimental campaign three isotopes, 176Lu, 134Cs, and 94Nb, were selected as possible physics cases. The newly designed plasma trap will also represent a tool of choice to measure the plasma opacities in a broad spectrum of plasma conditions, experimentally poorly known but that have a great impact on the energy transport and spectroscopic observations of many astrophysical objects. Status and perspectives of the project will be highlighted in the paper.

After CERN’s Long Shutdown 2, the n_TOF facility infrastructure was largely upgraded. The biggest change is the installation of a new lead spallation target, the performance of which needs to be carefully examined. During Summer 2021, the facility’s two flight paths were characterised in terms of neutron beam energy distribution, profile and resolution. In this work, the characterisation of the facility is described and the first results are given.

An accurate measurement of the 140Ce(n,γ) energy-dependent cross-section was performed at the n_TOF facility at CERN. This cross-section is of great importance because it represents a bottleneck for the s-process nucleosynthesis and determines to a large extent the cerium abundance in stars. The measurement was motivated by the significant difference between the cerium abundance measured in globular clusters and the value predicted by theoretical stellar models. This discrepancy can be ascribed to an overestimation of the 140Ce capture cross-section due to a lack of accurate nuclear data. For this measurement, we used a sample of cerium oxide enriched in 140Ce to 99.4%. The experimental apparatus consisted of four deuterated benzene liquid scintillator detectors, which allowed us to overcome the difficulties present in the previous measurements, thanks to their very low neutron sensitivity. The accurate analysis of the p-wave resonances and the calculation of their average parameters are fundamental to improve the evaluation of the 140Ce Maxwellian-averaged cross-section.

Experiments performed on Storage Rings have shown that lifetimes of beta-radionuclides can change dramatically as a function of theionization state. PANDORA (Plasmas for Astrophysics, Nuclear Decay Observation and Radiation for Archaeometry) aims at measuring, for the first time, nuclear β-decay rates in stellar-like conditions, especially for radionuclides involved in nuclear-astrophysics processes (BBN, s- processing, CosmoChronometers, Early Solar System formation). Compact magnetic plasma traps, where plasmas reach density ne ~10n -1014 cm-3 , and temperature Te ~0.1-30 keV, are suitable for such studies. The decay rates can be measured as a function of the charge state distribution of the inplasma ions. The collaboration is now designing the plasma trap able to reach the needed plasma densities, temperatures and charge states distributions. A first list of radioisotopes, including tens of physics cases of potential interest is now available. Possible physics cases include, among the others, 2 °4 Tl, 63 Ni, 6 °Co, 171 Tm, 147 Pm, 85 Kr, 176 Lu and the pairs 187 Re-187 Os and 87 Sr-87 Rb, which play a crucial role as cosmo-clock. Physics cases are now under evaluation in terms of lifetime measurements feasibility in a plasma trap.

. Neutron capture cross sections are one of the most important nuclear inputs to models of stellar nucleosynthesis of the elements heavier than iron. The activation technique and the time-of-flight method are mostly used to determine the required data experimentally. Recent developments of experimental techniques allow for new experiments on radioactive isotopes. Monte Carlo based analysis methods give new insights into the systematic uncertainties of previous measurements. We present an overview over the state-of-the-art experimental techniques, a detailed new evaluation of the 197 Au(n, γ ) cross section in the keV-regime and the corresponding re-evaluation of 63 more isotopes, which have been measured in the past relative to the gold cross section.

The doubly magic nucleus 16O has a small neutron-capture cross section of just a few tens of microbarns in the astrophysical energy region. Despite this, 16O plays an important role as a neutron poison in the astrophysical slow neutron capture (s) process due to its high abundance. We present in this paper a re-evaluation of the available experimental data for 16O()17O and derive a new recommendation for the Maxwellian-averaged cross sections between kT = 5 and 100 keV. Our new recommendations are lower up to kT = 60 keV compared to the previously recommended values but up to 14% higher at kT = 100 keV. We explore the impact of this different energy dependence on the weak s-process during core helium burning (kT = 26 keV) and shell carbon burning (kT = 90 keV) in massive stars where 16O is the most abundant isotope.

To allow new experimental data and improvements in evaluation procedure to be used in a timely manner in producing standards evaluations, an IAEA Data Development Project was initiated. For this project, it was decided that, in addition to the traditional activities related to standards, studies should be done on the possibility of extending the energy ranges of the standards and whether to include "reference data" that are not as well known as the standards but can be very useful in the measurements of certain types of cross sections. Activities include; an update of the experimental database for the traditional standards; improvements in smoothing procedures for capture cross sections, a review of the status of Cf-252 spontaneous fission neutron spectrum measurements; new work on the U-235 thermal neutron induced fission neutron spectrum that is not a standard but is important for reactor applications; improved calculations for fission neutron spectra; consideration of the Au-197 capture reaction as a reference cross section for capture cross-section measurements at energies of importance to astrophysics; and a study of reference cross sections for prompt gamma-ray production in fast neutron-induced reactions. A review of the progress made by this project will be given.