Context. The stellar origin of the elements molybdenum (Mo, Z = 42) and ruthenium (Ru, Z = 44) is still a matter of debate. Studying their abundances provides valuable insights into nucleosynthesis processes and the broader evolution of neutron-capture elements. Aims. The aim of this work is to present new observations of Mo and Ru, together with nearby neutron-capture elements strontium (Sr) and zirconium (Zr) for a new sample of 154 giant stars, located in the Galactic disk with metallicities −1 < [Fe/H] < +0.3. Methods. The abundances were determined under the assumption of the local thermodynamic equilibrium by fitting synthetic spectra. The abundances of Mo were derived from the Mo I lines at 5506 and 5533 Å, while the abundances of Ru were determined from Ru I lines at 4584, and 4757 Å. The abundances of Sr and Zr were measured using lines of Sr II at 4077 and 4215 Å and lines of Zr I at 5385, 6127, and 6134 Å. Results. We derived Sr, Zr, and Mo abundances for all stars in our sample, and Ru for 110 stars. For most of the giant stars observed in this work, Mo and Ru abundances were determined for the first time. We compare our observations with the signatures from different nucleosynthesis processes. Conclusions. Both the [Mo/Fe] and [Ru/Fe] in our stars show a decreasing trend with respect to increasing [Fe/H]. This pattern is similar to that of [Zr/Fe], whereas [Sr/Fe] exhibits a relatively flat trend with metallicity. These results are compatible with our previous measurements obtained for dwarf stars over the same metallicity range. Compared to the s-process ratios, all stars show a lower [Zr/Mo] and a higher [Ru/Mo], as expected from classical nucleosynthesis. Still, it is unclear if additional contributions from neutrino-wind components or the i-process is needed to explain the observed scatter of [Zr/Mo] and [Ru/Mo] in the Milky Way disk. Indeed, such a dispersion is consistent with the variations also seen in r-II stars at low metallicity and could therefore result from the combined contributions of r-process and s-process to galactic chemical evolution. The observed [Zr/Mo] and [Ru/Mo] scatter in r-II stars should be constrained by future investigations to define if any contributions of additional nucleosynthesis components are needed.
This work describes the formalism for estimating thermonuclear reaction rates for astrophysical applications, emphasizing modern statistical approaches such as Monte-Carlo sampling and Bayesian models. We discuss related topics including the calculation of resonance energies from nuclear Q values, indirect estimates of particle partial widths, and matching of reaction rates at elevated temperatures to statistical-model results. We have evaluated available experimental data on cross sections, resonance energies and strengths, partial widths, life-times, spin-parities, and spectroscopic factors. Based on these results, we have estimated numerical values of 78 experimental charged-particle thermonuclear reaction rates for target nuclei in the A = 2 to 40 mass region, for temperatures ranging from 1 MK to 10 GK. For each reaction, three rate values are provided: low, median, and high, corresponding to the 16th, 50th, and 84th percentiles, respectively, of the cumulative reaction rate probability density distribution. Additionally, we present the factor uncertainty of each rate at each temperature grid point. These results enable users to sample the reaction rate probability density in nucleosynthesis calculations, facilitating uncertainty estimates of nuclidic abundances. The rates presented here refer to their laboratory values. For use in stellar model simulations, these values need to be corrected for the effects of thermal excitations of the interacting nuclei. For each reaction, we include graphs that illustrate the fractional contributions to the overall reaction rate along with the associated uncertainty. These visuals are designed to assist both stellar modelers and nuclear experimentalists by identifying the primary sources of rate uncertainty at specific stellar temperatures. A graphical comparison with earlier Monte-Carlo rates is also provided.
Observed abundances of Z ∼ 40 elements in metal-poor stars vary from star to star, indicating that the rapid and slow neutron capture processes may not contribute alone to the synthesis of elements beyond iron. The weak r -process was proposed to produce Z ∼ 40 elements in a subset of old stars. Thought to occur in the ν -driven ejecta of a core-collapse supernova, ( α , xn ) reactions would drive the nuclear flow toward heavier masses at T = 2−5 GK. However, current comparisons between modeled and observed yields do not bring satisfactory insights into the stellar environment, mainly due to the uncertainties of the nuclear physics inputs where the dispersion in a given reaction rate often exceeds 1 order of magnitude. Involved rates are calculated with the statistical model where the choice of an α -optical-model potential ( α OMP) leads to such a poor precision. The first experiment on ^87 Rb( α , xn ) reactions at weak r -process energies is reported here. Total inclusive cross sections were assessed at E _c.m. = 8.1−13 MeV (3.7−7.6 GK) with the active target MUlti-Sampling Ionization Chamber. With an N = 50 seed nucleus, the measured values agree with statistical model estimates using the α OMP Atomki-V2 . A reevaluated reaction rate was incorporated into new nucleosynthesis calculations, focusing on ν -driven ejecta conditions known to be sensitive to this specific rate. These conditions were found to fail to reproduce the lighter heavy element abundances in metal-poor stars.
A measurement of the excitation spectrum of Kr-94 via one-neutron transfer to the ground state of Kr-93 using the Kr-93(d,p)Kr-94 reaction at 8A MeV, observing the outgoing protons, performed with the IRIS facility at TRIUMF is reported. Two states in Kr-94, at 1.50 +/- 0.14 MeV and 2.20 +/- 0.14 MeV, were observed. An adiabatic- wave approximation analysis of the differential cross sections leads us to identify the lower energy state as being populated with neutron transfer to the 3s(1/2) orbital. This leads to the first observation of the lowest 0(+) excited state in Kr-94, hence signaling shape co-existence. Theoretical calculations performed within the in-medium similarity renormalization group framework are presented that also show the existence of a low-energy 0(+) state, aligning qualitatively with the observation.
Approximately 30%–40% of classical novae generate dust between 20 and 100 days following the eruption. However, there has yet to be a definitive identification of presolar stardust grains originating from classical novae. While multiple studies have suggested a nova origin for specific grains, aligning simultaneously all measured isotopic ratios of a specific grain with those predicted from simulations remains challenging. Using Monte Carlo simulations, this work investigates how uncertainties in thermonuclear reaction rates influence the isotopic ratios predicted in simulations of classical novae, specifically impacting the identification of presolar grains. In particular, we address two questions: (i) What is the impact of uncertainties in reaction rates on the range of isotopic ratios predicted by classical nova simulations? (ii) Which reaction rate uncertainties most significantly influence the predicted abundance ratios in presolar grains? Our results show that current reaction rate uncertainties affect the isotopic ratios of ^12 C/ ^13 C, ^14 N/ ^15 N, ^16 O/ ^17 O, ^16 O/ ^18 O, ^24 Mg/ ^25 Mg, ^24 Mg/ ^26 Mg, ^26 Al/ ^27 Al, and ^28 Si/ ^29 Si by less than 20% in either carbon–oxygen or oxygen–neon (ONe) novae, especially when considering the mixing of matter throughout the entire envelope. However, the isotopic ratios of ^28 Si/ ^30 Si, ^32 S/ ^33 S, and ^32 S/ ^34 S in ONe novae are exceptions: their variability greatly exceeds a factor of 2 due to the uncertainties in the reaction rates of ^30 P(p, γ ) ^31 S, ^33 S(p, γ ) ^34 Cl, and ^34 S(p, γ ) ^35 Cl, respectively. These results highlight the significant influence of specific reaction rates on the predicted abundance ratios and underscore the necessity for accurate nuclear measurements to reduce these uncertainties.
The alpha optical model potential (alpha-OMP ) is a phenomenological approach used to describe elastic scattering where multiple reaction channels are open. It is one of the most critical inputs for the calculation of thermonuclear reaction rates in explosive stellar environments, but uncertainties within the alpha-OMP lead to imprecise predictions hindering comparisons between calculations and observations. In order to improve the precision of the alpha-OMP, additional nuclear physics data are required. In this paper, a measurement of the 86Sr(alpha, alpha) elastic scattering cross section at multiple energies is reported. A local optical potential is constructed via a fully Bayesian analysis of the elastic scattering data. The resulting uncertainties on the low-energy cross sections relevant to nuclear astrophysics are then calculated and shown to be on the order of 50%.
Classical novae are common cataclysmic events involving a binary system of a white dwarf and a main-sequence or red giant companion star. In metal-poor environments, these explosions produce ejecta differently from their solar counterparts due to the accretion of subsolar-metallicity material onto the white dwarf. In particular, it has been suggested that the nucleosynthesis flow in such low-metallicity nova explosions extends up to the Cu-Zn region, much beyond the expected endpoint, around Ca, predicted for solar-metallicity classical novae. This behavior resembles a weak rp-process, and such nuclear activity has never been observed in accreting white dwarf binaries with typical accretion flows. In this work, we study the characteristics of the weak rp-process for four nova models with metallicities Z = 2 x 10-9, 10-7, 2 x 10-6, and 2 x 10-5, and explore the impact of the nuclear physics uncertainties via a Monte Carlo sensitivity study. We identify nuclear reactions whose uncertainties affect the production of intermediate-mass nuclei under these conditions. These reactions and relevant nuclear quantities are targets for measurements at stable or radioactive beam facilities to reduce their rate uncertainties.
We present here an extended nuclear network, with 90 species, designed for being coupled with hydrodynamic simulations, which includes neutrons, protons, electrons, positrons, and the corresponding neutrino and anti-neutrino emission. This network is also coupled with temperature, making it extremely robust and, together with its size, unique of its kind. The inclusion of electron captures on free protons makes the network very appropriate for multidimensional studies of Type Ia supernova explosions, especially when the exploding object is a massive white dwarf. The results obtained with the proposed medium-sized network compare fairly well, to a few percent, with those computed with the extended network WinNet (> 2000 isotopes) in scenarios reproducing the gross physical conditions of current Type Ia supernova explosion models. In those cases where the carbon and oxygen fuel ignites at high density, the high-temperature plateau typical of the nuclear statistical equilibrium regime is well defined and stable, allowing large integration time steps. We show that the inclusion of electron captures on free protons substantially improves the estimation of the electron fraction of the mixture. Therefore, the pressure is better determined than in networks where electron captures are excluded, which will ultimately lead to more reliable hydrodynamic models. Explosive combustion of helium at low density, occurring near the surface layer of a white dwarf, is also better described with the proposed network, which gives nuclear energy generation rates much closer to WinNet than typical reduced alpha networks.
The elemental abundances between strontium and silver ( Z = 38–47) observed in the atmospheres of very metal-poor stars in the Galaxy may contain the fingerprint of the weak r -process and ν p -process occurring in early core-collapse supernovae explosions. In this work, we combine various astrophysical conditions based on a steady-state model to cover the richness of the supernova ejecta in terms of entropy, expansion timescale, and electron fraction. The calculated abundances based on different combinations of conditions are compared with stellar observations, with the aim of constraining supernova ejecta conditions. We find that some conditions of the neutrino-driven outflows consistently reproduce the observed abundances of our sample. In addition, from the successful combinations, the neutron-rich trajectories better reproduce the observed abundances of Sr–Zr ( Z = 38–40), while the proton-rich ones, Mo–Pd ( Z = 42–47).
In the last decade nuclear reaction measurements using heavy ion storage rings became an important tool for nuclear astrophysics studies. The new CRYRING Array for Reaction MEasurements (CARME), recently commissioned at the low energy CRYRING@ESR storage ring (GSI/FAIR), is designed to take this novel approach one step further and perform direct nuclear reaction measurements at stellar energies, as well as indirect studies of nuclear properties of interest for nuclear astrophysics. CRYRING is unique worldwide in being able to store high quality, isotopically pure, radioactive beams produced in-flight at the low energies required for nuclear astrophysics. This paper describes the first in-beam reaction measurement with CARME at CRYRING, the first beam on (conventional) target measurement for FAIR Phase-0, and the data analysis approach required by this unprecedented, unique experimental approach.
We have measured the cross section of the $^{83}$Rb(p,$\gamma)^{84}$Sr radiative capture reaction in inverse kinematics using a radioactive beam of $^{83}$Rb at incident energies of 2.4 and $2.7 A$ MeV. Prior to the radioactive beam measurement, the $^{84}$Kr(p,$\gamma)^{85}$Rb radiative capture reaction was measured in inverse kinematics using a stable beam of $^{84}$Kr at an incident energy of $2.7 A$ MeV. The effective relative kinetic energies of these measurements lie within the relevant energy window for the $\gamma$ process in supernovae. The central values of the measured partial cross sections of both reactions were found to be $0.17-0.42$ times the predictions of statistical model calculations. Assuming the predicted cross section at other energies is reduced by the same factor leads to a slightly higher calculated abundance of the $p$ nucleus $^{84}$Sr, caused by the reduced rate of the $^{84}$Sr($\gamma$,p)$^{83}$Rb reaction derived from the present measurement.
The ^{22}Mg(α,p)^{25}Al reaction rate has been identified as a major source of uncertainty for understanding the nucleosynthesis flow in Type-I x-ray bursts. We report a direct measurement of the energy- and angle-integrated cross sections of this reaction in a 3.3-6.9 MeV center-of-mass energy range using the MUlti-Sampling Ionization Chamber (MUSIC). The new ^{22}Mg(α,p)^{25}Al reaction rate is a factor of ∼4 higher than the previous direct measurement of this reaction within temperatures relevant for x-ray bursts, resulting in the ^{22}Mg waiting point of x-ray burst nucleosynthesis flow to be significantly bypassed via the (α,p) reaction.
The lighter heavy elements of the first r-process peak, between strontium and silver, can be synthesized in the moderately neutron-rich neutrino–driven ejecta of either core–collapse supernovae or neutron star mergers via the weak r–process. This nucleosynthesis scenario exhibits uncertainties from the absence of experimental data from ( α , xn ) reactions on neutron–rich nuclei, which are currently based on statistical model estimates. We have performed a new impact study to identify the most important ( α , xn ) reactions that can affect the production of the lighter heavy elements under different astrophysical conditions using new, constrained ( α , xn ) reaction rates based on the Atomki-V2 α OMP. Our results show how when reducing the nuclear physics uncertainties, we can use abundance ratios to constrain the astrophysical conditions/environment. This can be achieved in the near future, when the key ( α , xn ) reaction rates will be measured experimentally in radioactive beam facilities.
Globular clusters contain multiple stellar populations, with some previous generation of stars polluting the current stars with heavier elements. Understanding the history of globular clusters is helpful in understanding how galaxies merged and evolved and therefore constraining the site or sites of this historic pollution is a priority. The acceptable temperature and density conditions of these polluting sites depend on critical reaction rates. In this paper, three experimental studies helping to constrain astrophysically important reaction rates are briefly discussed.
The r-process has been shown to be robust in reproducing the abundance distributions of heavy elements, such as europium, seen in ultra-metal poor stars. In contrast, observations of elements 26 < Z < 47 display overabundances relative to r-process model predictions. A proposed additional source of early nucleosynthesis is the weak r-process in neutrino-driven winds of core-collapse supernovae. It has been shown that in this site (α,n) reactions are both crucial to nucleosynthesis and the main source of uncertainty in model-based abundance predictions. Aiming to improve the certainty of nucleosynthesis predictions, the cross section of the important reaction 86Kr(α,n)89Sr has been measured at an energy relevant to the weak r-process. This experiment was conducted in inverse kinematics at TRIUMF with the EMMA recoil mass spectrometer and the TIGRESS gamma-ray spectrometer. A novel type of solid helium target was used.
The $\gamma$-process nucleosynthesis in core-collapse supernovae is generally accepted as a feasible process for the synthesis of neutron-deficient isotopes beyond iron. However, crucial discrepancies between theory and observations still exist: the average production of $\gamma$-process yields from massive stars are too low to reproduce the solar distribution in galactic chemical evolution calculations, and the yields of the Mo and Ru isotopes are by a further factor of 10 lower than the yields of the other $\gamma$-process nuclei. We investigate the $\gamma$-process in 5 sets of core-collapse supernova models published in literature with initial masses 15, 20, and 25 M$_{\odot}$ at solar metallicity. We compared the $\gamma$-process overproduction factors from the different models. To highlight the possible effect of nuclear physics input, we also considered 23 ratios of two isotopes close to each other in mass, relative to their solar values. Further, we investigated the contribution of C-O shell mergers in the supernova progenitors as an additional site of the $\gamma$-process. Our analysis shows that a large scatter among the different models exists for both the $\gamma$-process integrated yields and the isotopic ratios. We found only 10 ratios that agree with their solar values, all the others differ by at least a factor of 3 from the solar values in all the considered sets of models. The $\gamma$-process within C-O shell mergers mostly influence the isotopic ratios that involve intermediate and heavy proton-rich isotopes with $\rm A>100$.
Astrophysical reactions involving radioactive isotopes (RI) often play an important role in high-temperature stellar environments. The experimental studies on the reaction rates for those are still limited mainly due to the technical difficulties in producing high-quality RI beams. A direct measurement of those reactions would be still challenging in many cases, however, we can make a reliable evaluation of the reaction rates by an indirect method or by studying the resonance prorerties. Here we ntroduce recent examples of experimental studies on such RI-involving astrophysical reactions, performed at Center for Nuclear Study, the University of Tokyo, using the low-energy RI beam separator CRIB. One is for the neutron-induced destruction reactions of 7Be in the Big-Bang nucleosynthesis, and the other is the study on the 22Mg(α, p) reaction relevant in X-ray bursts, which was performed with the resonant scattering method from the inverse reaction channel.
Experimental determination of the cross sections of proton capture on radioactive nuclei is extremely difficult. Therefore, it is of substantial interest for the understanding of the production of the p-nuclei. For the first time, a direct measurement of proton-capture cross sections on stored, radioactive ions became possible in an energy range of interest for nuclear astrophysics. The experiment was performed at the Experimental Storage Ring (ESR) at GSI by making use of a sensitive method to measure (p,γ) and (p,n) reactions in inverse kinematics. These reaction channels are of high relevance for the nucleosyn-thesis processes in supernovae, which are among the most violent explosions in the universe and are not yet well understood. The cross section of the 118Te(p,γ) reaction has been measured at energies of 6 MeV/u and 7 MeV/u. The heavy ions interacted with a hydrogen gas jet target. The radiative recombination process of the fully stripped 118Te ions and electrons from the hydrogen target was used as a luminosity monitor. An overview of the experimental method and preliminary results from the ongoing analysis will be presented.
We have measured the cross section of the $^{83}$Rb(p,$\gamma)^{84}$Sr radiative capture reaction in inverse kinematics using a radioactive beam of $^{83}$Rb at incident energies of 2.4 and $2.7 A$ MeV. Prior to the radioactive beam measurement, the $^{84}$Kr(p,$\gamma)^{85}$Rb radiative capture reaction was measured in inverse kinematics using a stable beam of $^{84}$Kr at an incident energy of $2.7 A$ MeV. The effective relative kinetic energies of these measurements lie within the relevant energy window for the $\gamma$ process in supernovae. The central values of the measured partial cross sections of both reactions were found to be $0.17-0.42$ times the predictions of statistical model calculations. Assuming the predicted cross section at other energies is reduced by the same factor leads to a slightly higher calculated abundance of the $p$ nucleus $^{84}$Sr, caused by the reduced rate of the $^{84}$Sr($\gamma$,p)$^{83}$Rb reaction derived from the present measurement.