Many observations strongly support the hypothesis that nuclei may fission through several independent fission modes (multimodal fission) interpreted as different prescission shapes and fission paths in a multidimensional potential energy landscape where shell effects are dominant. Mass distributions of the fission fragments are sensitive to the potential energy landscape and appear to be single humped (symmetric) or double humped (asymmetric). In many cases a mixture of both modes is observed. We propose here our study on 180Hg. Binary fission fragments formed in the reaction 68Zn + 112Sn → 180Hg at different excitation energies around the Coulomb barrier were detected using the double-arm time-of-flight technique with the spectrometers CORSET. The experiment was performed at JYFL (Jyvaskyla, Finland). We will discuss an analysis of the mass distributions in terms of fission modes predicted by a five-dimensional fission model. We have found out that the mass distributions can be well reproduced by considering a symmetric fission mode and two asymmetric modes at (AL ≈ 80, AH ≈ 100) and (AL ≈ 70 and AH ≈ 110).
Neutron dark decays have been suggested as a solution to the discrepancy between bottle and beam experiments, providing a dark matter candidate that can be searched for in halo nuclei. The free neutron in the final state following the decay of ^{6}He into ^{4}He+n+χ provides an exceptionally clean detection signature when combined with a high efficiency neutron detector. Using a high-intensity ^{6}He^{+} beam at Grand Accélérateur National d'Ions Lourds, a search for a coincident neutron signal resulted in an upper limit on a dark decay branching ratio of Br_{χ}≤4.0×10^{-10} (95% C.L.). Using the dark neutron decay model proposed originally by Fornal and Grinstein, we translate this into an upper bound on a dark neutron branching ratio of O(10^{-5}), improving over global constraints by one to several orders of magnitude depending on m_{χ}.
This paper reports partial results of a (n, n’γ) measurement on nickel. The inelastic channel was measured using the Gamma Array for Inelastic Neutron Scattering (GAINS) spectrometer at the 100-m measurement cabin of the Geel Electron Linear Accelerator (GELINA) neutron source of the European Commission’s Joint Research Centre (EC-JRC) in Geel, Belgium. Using γ spectroscopy, we were able to extract angle-integrated production cross sections for several γ rays but we report here only the results for the main transition in 58Ni. We discuss however in detail the observed discrepancy between our data and other experiments (especially the work of Voss et al.). We also shortly comment on the quality of the neutron-target optical model potential in describing the inelastic data in this mass region. The calculations were performed using the talys 1.9 code in the default settings.
GAINS (Gamma Array for Inelastic Neutron Scattering), currently installed at the GELINA (Geel Electron Linear Accelerator) neutron source of the EC-JRC (European Commission-Joint Research Centre), is one of the best instruments available worldwide for measuring high resolution, low uncertainty neutron inelastic cross-section data relevant for both fundamental research and nuclear physics applications (like Generation IV facilities). It features 12 HPGe detectors coupled with a 235 U fission chamber for neutron flux monitoring. The paper presents a short history of the GAINS development over the years and reviews some of the main experimental results together with plans for future experiments.
The necessary improvement of evaluated nuclear data for nuclear applications development is possible through new and high-quality measurements, often combined with appropriate nuclear-reaction modelling. In particular, improving inelastic cross-section evaluations requires new and high-quality data. We measure (n, n’γ) cross-sections using prompt γ-ray spectroscopy and neutron energy determination by time-of-flight. To extract, from these partial data, the total inelastic cross-section, we rely on theoretical model as well as nuclear structure data such as γ ray emission probabilities. This structure information, tabulated in databases, comes with uncertainty. This directly affects the precision of our results, regardless of how good the measurement is. In this paper, we will present the issue of limited precision structure data and its impact on nuclear reaction data quality in the case of neutron inelastic scattering measurements. We will also discuss how to foresee and mitigate the issue.
The necessary improvement of evaluated nuclear databases for appplication will be achieved with improvement of models and new, precise data. In particular, the effect of inelastic neutrons scattering can be of importance for reactors. In order to test the models, we performed measurement of (n, n’γ) and (n, 2nγ) cross-sections on 183 W. These data will help constrain the calculation codes and ensure a better evaluation of the total (n, x n) cross section. The experimental setup and the data analysis method will be presented. The preliminary experimental results for the 183 W isotope will be compared to predictions from Talys nuclear reaction code.
GRAPhEME is a γ-spectrometer developed by CNRS/IPHC Strasbourg (France), in collaboration with EC-JRC Geel (Belgium) and IFIN-HH Bucharest (Romania). With its 6 High Purity Planar Germanium detectors and one fission chamber, GRAPhEME, installed at the EC-JRC GELINA facility, was optimized for measurements of accurate (n, xnγ) cross sections on actinides. The experimental methodology is based on the prompt γ-ray spectroscopy coupled to time-of-flight measurements. In this paper, we present an overview of fifteen years of experiments with GRAPhEME at EC-JRC GELINA facility, illustrated by main achievements to highlight the performances reached by our spectrometer. Beyond the experimental work, a close collaboration with theoreticians has emerged allowing the use of the data produced with GRAPhEME to test and constraint nuclear reaction codes like TALYS, CoH and EMPIRE. In a near future, GRAPhEME will be available to start measurement campaigns at the new neutron beam facility SPIRAL2/NFS. There, studies of (n, 2n) and (n, 3n) reactions will be possible and will complete the work done at EC-JRC GELINA on (n, n ) reactions. Despite the amount of cross section data provided by GRAPhEME up to now, the prompt γ-ray spectroscopy method presents some weaknesses that our collaboration tries to overcome. This goes through new calculation schemes based on theoretical modeling constrained on experimental data to infer the total (n, xn) cross section, new instrument to measure conversion electrons but also by being proactive in dissemination activities to make the nuclear structure community aware of our needs about new accurate nuclear structure information on actinides.
In the context of the development of Gen. IV nuclear reactors, the GIF (Generation IV. International Forum) has selected six innovative technologies. Among them, one can highlight the concept of breeding for 232 Th/ 233 U and 238 U/ 239 Pu fuel cycles. But those nuclei, crucial for such cycles, suffer from a lack of precise knowledge (nuclear structure, reaction cross sections). In particular, it has been demonstrated that neutron inelastic scattering reaction cross sections are not known with sufficient precision for the isotopes 238 U and 239 Pu, and not known at all experimentally for 233 U. In order to perform simulations of innovative reactor cores for the development of those technologies, the knowledge of the reaction cross section has to be improved which implies that new measurements have to be done. The GRAPhEME (GeRmanium array for Actinides PrEcise MEasurements) experimental setup, developed by the IPHC laboratory from CNRS and installed at the EC-JRC-Geel GELINA facility is a powerful tool to answer this need [1, 2]. Combining the prompt γ-ray spectroscopy and the time-of-flight methods, it measures partial (n, xnγ) reaction cross sections. This paper reports on the improvements made on the GRAPhEME setup and data analysis methodology to tackle the challenge of (n, xnγ) cross section measurements on high activity actinides. Results obtained so far on 233 U are presented compared to TALYS calculations.
The production of useful and high-quality nuclear data requires measurements with high precision and extensive information on uncertainties and possible correlations. Analytical treatment of uncertainty propagation can become very tedious when dealing with a high number of parameters. Even worse, the production of a covariance matrix, usually needed in the evaluation process, will require lenghty and error-prone formulas. To work around these issues, we propose using random sampling techniques in the data analysis to obtain final values, uncertainties and covariances and for analyzing the sensitivity of the results to key parameters. We demonstrate this by one full analysis, one partial analysis and an analysis of the sensitivity to branching ratios in the case of (n,n’γ) cross section measurements.
The extended dataset of 56 Fe(n,n’γ) cross sections measured by our group more than a decade ago at GELINA (Geel Linear Accelerator) was used in many recent evaluations like ENDF, JEFF and CIELO. Despite the special measures we took to ensure reliability and accuracy, concerns were raised by various groups with regard to several features of this dataset (absolute normalization and/or shape) and therefore the 56 Fe(n,inl) cross section is still under the evaluation by the International Nuclear Data Evaluation Network (INDEN). Consequently, a new experiment is now under preparation aiming to take advantage of the numerous experimental improvements of the GAINS (Gamma Array for Inelastic Neutron Scattering) setup implemented over the years. While γ spectroscopy combined with the time-of-flight method will remain the main technique involved, several other experimental details will differ substantially.
To probe the neutron inelastic scattering off 232 Th, an experiment took place at the EC-JRC Geel conducted with the experimental setup GRAPhEME to detect emitted γ-rays. The prompt γ-ray spectroscopy method was used and 70 experimental 232 Th(n, n’γ) cross sections were obtained from the experimental data. Combining these cross sections, nuclear-structure data available in databases and hypotheses to complete the latter, neutron inelastic level production cross sections in 232 Th and the total inelastic cross section were calculated. For the first time, the total inelastic cross section of an actinide nucleus was derived on the total neutron energy range from experimental data only. Comparisons of (n, n’) cross section data with evaluated data reveal a good agreement between them all above 300 keV of neutron energy. TALYS calculations are compatible but lower than the evaluated data.
The next years will see the completion of several new facilities at Istituto Nazionale di Fisica Nucleare – Laboratori Nazionali del Sud (LNS) opening up new possibilities in the fields of nuclear structure, nuclear dynamics, nuclear astrophysics and applications. These include a new line for high-intensity cyclotron beams, a new facility for in-flight production of radioactive ion beams, the PANDORA plasma trap for multidisciplinary studies and a high-power laser for basic science and applied physics. The nuclear physics community has organized a workshop to discuss the new physics opportunities that will be possible in the middle term (5–7 years) by employing state-of-the-art detection systems. A detailed discussion of the outcome from the workshop is presented in this report.
The β-decay of the even-even nucleus 70Kr with Z=N+2, has been investigated at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center using the BigRIPS fragment separator, the ZeroDegree Spectrometer, the WAS3ABI implantation station and the EURICA HPGe cluster array. Fifteen γ-rays associated with the β-decay of 70Kr into 70Br have been identified for the first time, defining ten populated states below Eexc=3300 keV. The half-life of 70Kr was derived with increased precision and found to be t1/2=45.19±0.14 ms. The β-delayed proton emission probability has also been determined as εp=0.545(23)%. An increase in the β-strength to the yrast 1+ state in comparison with the heaviest Z=N+2 system studied so far (62Ge decay) is observed that may indicate increased np correlations in the T=0 channel. The β-decay strength deduced from the results is interpreted in terms of the proton-neutron quasiparticle random-phase approximation (pnQRPA) and also with a schematic model that includes isoscalar and isovector pairing in addition to quadrupole deformation. The application of this last model indicates an approximate realization of pseudo-SU(4) symmetry in this system.
We have refurbished and tested a neutron array composed of 81 BC400 plastic scintillator detectors dedicated for neutron measurements in future fusion-fission experiments The Neutron Array (NA) detectors, installed at the 9 MV Tandem accelerator facility of the Horia Hulubei National Institute for R&D in Physics and Nuclear Engineering (IFIN-HH), have been refurbished and the data acquisition system has been updated. We present the characteristics and performances of the NA and of the associated electronics.
Introduction: Sleep is an active metabolic process, extremely important for homeostasis. An important and continuously studied subject is the link between sleep and smoking/ smoking withdrawal, smoking being a major cause of mortality worldwide. Aims and objectives: We studied the influence of smoking/smoking withdrawal on addictions, symptoms and on sleep architecture in patients with sleep disorders. Material and method: 301 patients diagnosed via polysomnography with sleep disorders, retrospectively studied (Jan 2017-Sept 2020) were divided in active smokers-S, former smokers-FS, non-smokers-NS. The comparative analysis was performed using SPSS Statistics (v21.00). Results: with statistically significance (p<0.05): NS had more addictions, and their sleep disorders were more symptomatic than in S. The findings can be explained by the extremely high anxiety status of the NS. S and FS had the tendency to sleep more superficially (N1, N2), while the N3 stage was significantly more consistent in S than in ExS/FS. There were no differences in REM sleep percentage between groups. Conclusion: Because of its impact on sleep (especially on its quality and architecture, less on its quantity), the smoker status of the patient diagnosed with sleep disorders should be assess, the same as the level of anxiety of these patients.
Inclusive energy spectra have been measured for light charged particles emitted in the bombardment of Ta target by48Ca ions at 261 MeV and 471 MeV. The reaction products were analyzed and detected by means of a (∆E-E) telescope placed in the focal plane of a magnetic spectrometer located at forward angles with respect to the beam direction. In all the reactions studied light charged particles with an energy close to the respective calculated kinematic limit for a two-body exit channel are produced with relatively great probability. The results obtained make it possible to draw some conclusions about the reaction mechanism involving the emission of light charged particles.
Today's development of nuclear installations rely on numerical simulation for which the main input are evaluated nuclear data. Inelastic neutron scattering (n, xn) is a reaction of importance because it modifies the neutron population, the neutron energy distribution and may create new isotopes. The study of this reaction on tungsten isotopes is interesting because it is a common structural material. Additionally, tungsten isotopes are a good testing field for theories. The IPHC group started an experimental program with the GRAPhEME setup installed at the neutron beam facility GELINA to measure (n, xn γ) reaction cross sections using prompt gamma spectroscopy and neutron energy determination by time-of-flight. The obtained experimental data provide constraints on nuclear reaction mechanisms models for 182,184,186 W. Indeed, to reproduce correctly the experimental (n, n' γ) cross-sections, the reaction codes must include accurate models of the reaction mechanism, nuclear de-excitation process and use correct nuclear structure information.
The reduced transition probabilities $B(E2;{0}_{\text{g.s.}}^{+}\ensuremath{\rightarrow}{2}_{1}^{+},{2}_{2}^{+})$ in $^{70}\mathrm{Zn}$ and the full $B(E2;{0}_{\text{g.s.}}^{+}\ensuremath{\rightarrow}{2}^{+})$ strength up to ${\mathrm{S}}_{n}=7.79\phantom{\rule{4pt}{0ex}}\mathrm{MeV}$ in $^{68}\mathrm{Ni}$ have been determined at the LISE/GANIL facility using the Coulomb-excitation technique at intermediate beam energy on a $^{208}\mathrm{Pb}$ target. The $\ensuremath{\gamma}$ rays emitted in-flight were detected with an array of $46{\mathrm{BaF}}_{2}$ crystals. The angles of the deflected nuclei were determined in order to disentangle and extract the Coulomb and nuclear contributions to the excitation of the ${2}^{+}$ states. The measured $B(E2;{0}_{\text{g.s.}}^{+}\ensuremath{\rightarrow}{2}_{1}^{+})$ of 1432(124) ${e}^{2}\phantom{\rule{0.16em}{0ex}}{\mathrm{fm}}^{4}$ for $^{70}\mathrm{Zn}$ falls in the lower part of the published values which clustered either around 1600 or above $2000\phantom{\rule{3.33333pt}{0ex}}{e}^{2}\phantom{\rule{0.16em}{0ex}}{\mathrm{fm}}^{4}$, while the $B(E2;{0}_{\text{g.s.}}^{+}\ensuremath{\rightarrow}{2}_{2}^{+})$ of 53(7) ${e}^{2}\phantom{\rule{0.16em}{0ex}}{\mathrm{fm}}^{4}$ agrees very well with the two published values. The relatively low $B(E2;{0}_{\text{g.s.}}^{+}\ensuremath{\rightarrow}{2}_{1}^{+})$ of 301(38) ${e}^{2}\phantom{\rule{0.16em}{0ex}}{\mathrm{fm}}^{4}$ for $^{68}\mathrm{Ni}$ agrees with previous studies and confirms a local magicity at $Z=28$, $N=40$. Combining the results of the low-energy spectra of $^{68}\mathrm{Ni}$ and $^{70}\mathrm{Zn}$ and their shell-model interpretations, it is interesting to notice that four different shapes (spherical, oblate, prolate, and triaxial) are present. Finally, a summed $E2$ strength of only about $150\phantom{\rule{4pt}{0ex}}{e}^{2}\phantom{\rule{0.16em}{0ex}}{\mathrm{fm}}^{4}$ has been found experimentally at high excitation energy, likely due to proton excitations across the $Z=28$ gap. The experimental distribution of this high-energy $E2$ excitation agrees with shell-model calculations, but its strength is about two times weaker.
Neutron-removal cross-section ( σ-xn ) measurements of neutron-rich light nuclei were performed on the COMBAS fragment-separator with a multi-detector Si telescope at intermediate energies (22-34) MeV/nucleon. The removals of one neutron from8Li and9Be, two neutrons from6 He and10 Be and four neutrons from 8 He were observed from the reactions on a Si-CsI(Tl) telescope. Results of σ-xn for6 He,8 He,8 Li,9 Be and10 Be nuclei were obtained and compared with those of previously measured data. The data indicate that4 He is a good core within6 He and8 He. Furthermore, we found that9,10 Be nuclei disintegrated by one- and two- neutron removal reaction, respectively.
Results for fusion and breakup fusion reaction ( 6 Li+ 194 Pt) are presented and compared with other experimental data and model calculations. A strong isotopic effect is observed when comparing our data with results from ( 6 Li+ 198 Pt)