The sequential resonant excitation of a 2-level quantum system results in the emission of a state of light showing time-entanglement encoded in the photon-number-basis - notions that can be extended to 3-level quantum systems as discussed in a recent proposal. Here, we report the experimental implementation of a sequential two-photon resonant excitation process of a solid-state 3-level system, constituted by the biexciton-, exciton-, and ground-state of a semiconductor quantum dot. The resulting light state exhibits entanglement in time and energy, encoded in the photon-number basis, which could be used in quantum information applications, e.g., dense information encoding or quantum communication protocols. Performing energy- and time-resolved correlation experiments in combination with extensive theoretical modelling, we are able to partially retrieve the entanglement structure of the generated state.

Solid-state quantum light sources based on semiconductor quantum dots (QDs) are increasingly employed in photonic quantum information applications. Especially when moving towards real-world scenarios outside shielded lab environments, the efficient and robust coupling of nanophotonic devices to single-mode optical fibers offers substantial advantage by enabling “plug-and-play” operation. In this work we present a fiber-pigtailed cavity-enhanced source of flying qubits emitting single indistinguishable photons at clock-rates exceeding 1 GHz. This is achieved by employing a fully deterministic technique for fiber-pigtailing optimized QD-devices based on hybrid circular Bragg grating (hCBG) micro-cavities. The fabricated fiber-pigtailed hCBGs feature emission lifetimes of <80 ${< } 80$ ps, corresponding to a Purcell factor of ∼9, a suppression of multi-photon emission events with g (2)(0) < 1 %, a photon-indistinguishability >80 ${ >} 80$ % and a measured single-photon coupling efficiency of 53 % in a high numerical aperture single-mode fiber, corresponding to 1.2 Megaclicks per second at the single-photon detectors under 80 MHz excitation clock-rates. Furthermore, we show that high multi-photon suppression and indistinguishability prevail for excitation clock-rates exceeding 1 GHz. Our results show that Purcell-enhanced fiber-pigtailed quantum light sources based on hCBG cavities are a prime candidate for applications of quantum information science.

We present Purcell-enhanced (F P > 25) semiconductor InAs quantum dot decay times of T 1 < 30 ps, enabled by deterministic hybrid circular Bragg gratings (hCBGs). We investigate the benefits of these short T 1-times on the two-photon indistinguishability for quasi-resonant and strictly resonant excitation and observe visibilities of >= 96% at 12.5 ns time delay of consecutively emitted photons. The strongly Purcell-enhanced decay times enable a high degree of indistinguishability for elevated temperatures of up to 30 K and, moreover, allow for excitation of up to 1.28 GHz repetition rate. Our work highlights the prospects of highly Purcell-enhanced solid-state quantum emitters for applications in quantum information and technologies operating at GHz clock rates.

Single indistinguishable photons at telecom C-band wavelengths are essential for quantum networks and the future quantum internet. However, high-throughput technology for single-photon generation at 1550 nm remained a missing building block to overcome present limitations in quantum communication and information technologies. Here, we demonstrate the high-throughput fabrication of quantum-photonic integrated devices operating at C-band wavelengths based on epitaxial semiconductor quantum dots. Our technique enables the deterministic integration of single pre-selected quantum emitters into microcavities based on circular Bragg gratings. Respective devices feature the triggered generation of single photons with ultra-high purity and record-high photon indistinguishability. Further improvements in yield and coherence properties will pave the way for implementing single-photon non-linear devices and advanced quantum networks at telecom wavelengths. An efficient way of realising a large number of telecom single-photon emitters for quantum communication is still missing. Here, the authors use a wide-field imaging technique for fast localization of single InAs/InP quantum dots, which are then integrated into circular Bragg grating cavities featuring high single-photon purity and indistinguishability.

Semiconductor quantum dots (QDs) enable the generation of single and entangled photons, which are useful for various applications in photonic quantum technologies. Specifically for quantum communication via fiber-optical networks, operation in the telecom C-band centered around 1550 nm is ideal. The direct generation of QD-photons in this spectral range with high quantum-optical quality, however, remained challenging. Here, we demonstrate the coherent on-demand generation of indistinguishable photons in the telecom C-band from single QD devices consisting of InAs/InP QD-mesa structures heterogeneously integrated with a metallic reflector on a silicon wafer. Using pulsed two-photon resonant excitation of the biexciton-exciton radiative cascade, we observe Rabi rotations up to pulse areas of 4π and a high single-photon purity in terms of g(2)(0) = 0.005(1) and 0.015(1) for exciton and biexciton photons, respectively. Applying two independent experimental methods, based on fitting Rabi rotations in the emission intensity and performing photon cross-correlation measurements, we consistently obtain preparation fidelities at the π-pulse exceeding 80%. Finally, performing Hong-Ou-Mandel-type two-photon interference experiments, we obtain a photon-indistinguishability of the full photon wave packet of up to 35(3)%, representing a significant advancement in the photon-indistinguishability of single photons emitted directly in the telecom C-band.

Quantum communication networks rely on quantum cryptographic protocols including quantum key distribution (QKD) based on single photons. A critical element regarding the security of QKD protocols is the photon number coherence (PNC), i.e., the phase relation between the vacuum and one-photon Fock state. To obtain single photons with the desired properties for QKD protocols, optimal excitation schemes for quantum emitters need to be selected. As emitters, we consider semiconductor quantum dots, that are known to generate on-demand single photons with high purity and indistinguishability. Exploiting two-photon excitation of a quantum dot combined with a stimulation pulse, we demonstrate the generation of high-quality single photons with a controllable degree of PNC. The main tuning knob is the pulse area giving full control from minimal to maximal PNC, while without the stimulating pulse the PNC is negligible in our setup for all pulse areas. Our approach provides a viable route toward secure communication in quantum networks.

The generation of single photons using solid-state quantum emitters is pivotal for advancing photonic quantum technologies, particularly in quantum communication. As the field continuously advances toward practical use cases and beyond shielded laboratory environments, specific demands are placed on the robustness of quantum light sources during operation. In this context, the robustness of the quantum light generation process against intrinsic and extrinsic effects is a major challenge. Here, we present a robust scheme for the coherent generation of indistinguishable single-photon states with very low photon number coherence using a three-level system in a semiconductor quantum dot. Our approach combines the advantages of adiabatic rapid passage and stimulated two-photon excitation. We demonstrate robust quantum light generation while maintaining the prime quantum-optical quality of the emitted light state. Moreover, we highlight the immediate advantages of the implementation of various quantum cryptographic protocols.

Worldwide enormous efforts are directed towards the development of the so-called quantum internet. Turning this long sought-after dream into reality is a great challenge that will require breakthroughs in quantum communication and computing. To establish a global, quantum-secured communication infrastructure, photonic quantum technologies will doubtlessly play a major role, by providing and interfacing essential quantum resources, e.g., flying- and stationary qubits or quantum memories. Over the last decade, significant progress has been made in the engineering of on-demand quantum light sources based on semiconductor quantum dots, which enable the generation of close-to-ideal single- and entangled-photon states, useful for quantum cryptography tasks. This review focuses on implementations of, and building blocks for, quantum communication using quantum-light sources based on epitaxial semiconductor quantum dots. After reviewing the main notions of quantum cryptography (section 1) and introducing the devices used for single-photon and entangled-photon generation (section 2), it provides an overview of experimental implementations of cryptographic protocols using quantum dot based quantum light sources (section 3). Furthermore, recent progress towards quantum-secured communication networks as well as building blocks thereof is summarized (section 4). The article closes with an outlook, discussing future perspectives in the field and identifying the main challenges to be solved.