The symmetry of normal metal/ferromagnet bilayers allows spin-orbit torques (SOTs) to simultaneously have two distinct angular dependences on the magnetization direction m. The most well-studied forms of SOT consist of the conventional fieldlike and dampinglike torques, which we label as "lowest-order" SOT. There are additional SOT forms associated with spin polarization different from that of the lowest-order SOT, and which contain an extra factor of m dependence. We label these as "higher-order" SOT. Understanding SOT-driven magnetization dynamics requires detailed information about the full angular dependence. In this paper, we measure both the lowest-order and higher-order angular dependences of SOTs in three types of bilayers, Pt/Co, Ta/CoFeB, and W/CoFeB, using harmonic Hall measurements. It is found that the higher-order SOT is negligible for Pt/Co and Ta/CoFeB, whereas it is dominant over the lowest-order one for W/CoFeB. Macrospin simulations show that the higher-order SOT can significantly affect the magnetization dynamics, which is qualitatively in line with SOT-induced switching experiments.
Spin-orbit torques (SOTs) have been investigated most widely in normal metal/ferromagnet bilayers where the spin Hall effect of normal metal is a main source of spin currents. Recently, ferromagnets are found to also serve as spin-current sources through spin-orbit coupling. In this work, we theoretically investigate SOT acting on ferromagnet2 in ferromagnet1/normal metal/ferromagnet2 trilayers, which is caused by the spin Hall and spin swapping effects of ferromagnet1. Our result provides an analytical expression of SOT in the trilayers, which may be useful for quantifying the spin Hall and spin swapping effects of ferromagnets and also for designing and interpreting SOT experiments where a ferromagnet is used as a spin-current source instead of a normal metal.
We theoretically investigate spin-orbit torques in insulator/ferromagnet/normal-metal structures with a focus on interfacial spin-orbit coupling effect at an insulator/ferromagnet interface. Based on the spin drift-diffusion formalism generalized to consider transverse spin currents in a ferromagnet and the boundary condition to consider transverse spin currents leaving from a ferromagnet, we find that interfacial spin-orbit coupling at the insulator/ferromagnet interface contributes to dampinglike spin-orbit torque, which is important for current-driven magnetization dynamics, even when the interfacial spin-orbit coupling generates the only fieldlike component. We also calculate spin-orbit torques in a single ferromagnet sandwiched by two dissimilar insulators, which provides additional information about interfacial spin-orbit interaction at insulator/ferromagnet interfaces.
Exploiting spin transport increases the functionality of electronic devices and enables such devices to overcome physical limitations related to speed and power. Utilizing the Rashba effect at the interface of heterostructures provides promising opportunities toward the development of high-performance devices because it enables electrical control of the spin information. Herein, the focus is mainly on progress related to the two most compelling devices that exploit the Rashba effect: spin transistors and spin-orbit torque devices. For spin field-effect transistors, the gate-voltage manipulation of the Rashba effect and subsequent control of the spin precession are discussed, including for all-electric spin field-effect transistors. For spin-orbit torque devices, recent theories and experiments on interface-generated spin current are discussed. The future directions of manipulating the Rashba effect to realize fully integrated spin logic and memory devices are also discussed.
The harmonic Hall measurement is widely used to determine the equivalent field of current-induced spin-orbit torque in ferromagnet/normal metal bilayers. We report that this method suffers from various thermoelectric artifacts that have not been considered. We propose and experimentally demonstrate how to eliminate major thermoelectric artifacts using, namely, the four-direction (4-D) methods interchanging current and field polarities, which allow us to determine the magnitudes and angular dependences of spin-orbit torques more accurately than a conventional method. The proposed 4-D method will be useful for searching suitable materials for device applications operated by spin-orbit torques.
Based on a spin drift-diffusion model, we theoretically investigate the spin-orbit torque in ferromagnet/normal metal/insulator trilayers with considering the Rashba interfacial spin-orbit coupling at the normal metal/insulator interface. We find that the spin-orbit torque shows the opposite normal-metal-thickness dependences for the bulk spin-orbit coupling effect in the normal metal layer and for the interfacial spin-orbit coupling effect at the normal metal/insulator interface, offering a way to disentangle these two spin-orbit coupling effects. Moreover, we show that the conventional interpretation based on the bulk spin-orbit coupling effect overestimates the spin Hall angle and underestimates the spin diffusion length of the normal metal layer, when the interfacial contribution is non-negligible. Our result, a concise analytic expression of the spin-orbit torque considering both bulk and interface spin-orbit coupling effects, will be useful to design and interpret experiments on spin-orbit torque experiments in ferromagnet/normal metal/insulator trilayers.
Non-magnetic (NM) metals with strong spin-orbit coupling have been recently explored as a probe of interface magnetism on ferromagnetic insulators (FMI) by means of the spin Hall magnetoresistance (SMR) effect. In NM/FMI heterostructures, increasing the spin mixing conductance (SMC) at the interface comes as an important step towards devices with maximized SMR. Here we report on the study of SMR in Pt/Fe3O4 bilayers at cryogenic temperature, and identify a strong dependence of the determined real part of the complex SMC on the interface roughness. We tune the roughness of the Pt/Fe3O4 interface by controlling the growth conditions of the Fe3O4 films, namely by varying the thickness, growth technique, and post-annealing processes. Field-dependent and angular-dependent magnetoresistance measurements sustain the clear observation of SMR. The determined real part of the complex SMC of the Pt/Fe3O4 bilayers ranges from 4.96 × 1014 Ω−1 m−2 to 7.16 × 1014 Ω−1 m−2 and increases with the roughness of the Fe3O4 underlayer. We demonstrate experimentally that the interface morphology, acting as an effective interlayer potential, leads to an enhancement of the spin mixing conductance.
An accurate method is developed to extract the spin–orbit (SO) effective fields by analyzing harmonic Hall voltage measurements and deriving detailed analytical equations that consider both the z component of the applied magnetic field and the second-order perpendicular magnetic anisotropy. The method is tested by analyzing the results of a macrospin simulation. The SO effective fields that are extracted from the analysis are consistent with the input SO effective fields that are used in the macrospin simulation over the entire range of the polar magnetization angle and for a wide range (0–2) of the ratio of the planar to the anomalous Hall voltage considered in this study. The accuracy of the proposed method is demonstrated via a systematic study that involves comparing its results with those of a conventional analytical method. A way to extract information about complex spin–orbit interactions from simple voltage measurements has been developed by a team in Korea. Recent research has shown that a current can switch the direction of electron spins in a ferromagnet when a ferromagnetic layer is placed on a non-magnetic one. This phenomenon is driven by the so-called spin-orbit torque, but its underlying mechanisms are unclear. The framework developed by Sang Ho Lim and co-workers from Korea University obtains information about these spin-orbit fields from simple measurements of the harmonic Hall voltage. Their analytical equations could improve the understanding of magnetization switching in magnetic materials since, unlike earlier equations, they include both the magnetic field applied perpendicular to the films and the second-order perpendicular magnetic anisotropy. An accurate method, with detailed analytical equations, is developed to extract the spin–orbit (SO) effective fields through analysis of the results of harmonic Hall voltage measurements. Both the z component of the applied magnetic field (its directions, together with the axes and the Hall bars, are shown in the left figures) and the second-order perpendicular magnetic anisotropy are taken into account. The contour plots (right figures) showing the deviation (in %) from input values of the damping-like (ΔHDL) and field-like (ΔHFL) SO effective fields clearly demonstrate a significant improvement in the accuracy of the results obtained from the new refined method.
Spin-orbit torques arising from the spin-orbit coupling of non-magnetic heavy metals allow electrical switching of perpendicular magnetization. However, the switching is not purely electrical in laterally homogeneous structures. An extra in-plane magnetic field is indeed required to achieve deterministic switching, and this is detrimental for device applications. On the other hand, if antiferromagnets can generate spin-orbit torques, they may enable all-electrical deterministic switching because the desired magnetic field may be replaced by their exchange bias. Here we report sizeable spin-orbit torques in IrMn/CoFeB/MgO structures. The antiferromagnetic IrMn layer also supplies an in-plane exchange bias field, which enables all-electrical deterministic switching of perpendicular magnetization without any assistance from an external magnetic field. Together with sizeable spin-orbit torques, these features make antiferromagnets a promising candidate for future spintronic devices. We also show that the signs of the spin-orbit torques in various IrMn-based structures cannot be explained by existing theories and thus significant theoretical progress is required.