We experimentally observe a new type of quantum-path interference, in two-dimensional(2D-QPI), in high-harmonic generation (HHG) driven by an orthogonally-polarised highly-bichromatic field. This regime is marked by comparable intensities of the two orthogonal colours. In this highly-bichromatic regime, we demonstrate that 2D-QPI is encoded in the measured harmonic intensity modulations with respect to the relative phase of the two-colour field. The modulations of the odd-order harmonics show a monomodal behaviour, whereas the even harmonics are modulated in a bimodal structure. Our calculations using the strong-field approximation and saddle-point method disentangle contributions from multiple quantum orbits in this HHG regime, revealing that the dipole response for both odd and even harmonics inherits the dynamic symmetry of the orthogonally-polarised driving field. This new type of 2D-QPI offers a novel route to HHG spectroscopy of attosecond electron dynamics by lifting up the dimensionality of the quantum paths involved in the interference.

Superfluid He nanodroplets resonantly excited by extreme ultraviolet (XUV) pulses can relax via interatomic coulombic decay (ICD), generally considered an ultrafast process. Here, we introduce a novel approach to probe the dynamics of ICD in He nanodroplets over timescales ranging from femtoseconds to nanoseconds. Our method relies on detecting XUV fluorescence emitted from the nanodroplets as they are driven into a nanoplasma by subsequent intense infrared pulses. Nanoplasma ignition is facilitated by tunnel ionization of XUV-excited He ^* atoms attached to the droplets; it thus serves as a sensitive probe of their relaxation dynamics. The observed nanosecond-scale decay is attributed to ICD between pairs of He ^* atoms undergoing roaming motion on the droplet surface, as supported by quantum-mechanical and classical model calculations.

Ultrafast optical control of solids has uncovered new phenomena and advanced non-equilibrium condensed matter physics, where photon dressed electronic states - Floquet Bloch states (FBSs) - emerge under a strong oscillating laser field, also known as Floquet engineering. Although FBSs have been extensively investigated using time and angle resolved photoemission spectroscopy, direct evidence of their role in high-harmonic generation spectroscopy (HHGS) has remained elusive. Here, we present combined experimental and theoretical evidence that FBSs can be probed by HHG emission in the wide-bandgap solid magnesium oxide (MgO) driven by few cycle near infrared pulses. Experimentally, we observe clear evidence of FBSs in the HHG yield dependence on the crystal orientation. This specific feature is attributed to nonadiabatic coupling between FBSs and conduction bands near the Brillouin zone edge, where the strong laser field transiently breaks time reversal symmetry. We have confronted the experimental findings with numerical solutions of the time dependent Schrödinger equation, which reproduce the new feature and confirm its Floquet origin. The theoretical results show a coupling inducing a local band structure renormalization and Floquet like hybridization under strong field excitation. It also shows that FBS nonadiabatic dynamics persist in the strong field regime, establishing HHGS as a powerful probe of ultrafast light induced band hybridization in solids.

In this work, experimentally measured characteristics of a kilohertz laser-driven Cu plasma X-ray source that was recently commissioned at the ELI Beamlines facility are reported. The source can be driven either by an in-house developed high-contrast sub-20 fs near-infrared terawatt laser based on optical parametric chirped-pulse amplification technology or by a more conventional Ti:sapphire laser delivering 12 mJ and 45 fs pulses. The X-ray source parameters obtained with the two driving lasers are compared. A measured photon flux of the order up to 1012 Kα photons s−1 (4π)−1 is reported. Furthermore, experimental platforms for ultrafast X-ray diffraction and X-ray absorption and emission spectroscopy based on the reported source are described.

Ptychography is a robust lensless form of microscopy routinely used for applications spanning life and physical sciences. The most common ptychography setup consists in using a detector to record diffraction patterns in the far-field. A near-field version has been more recently introduced, and its potential is yet to be fully exploited. In this work, the sampling requirements for near-field ptychography are analysed. Starting from the characterisation available in literature, the formalism of the fractional Fourier transform is used to generalise analytically the sampling conditions. The results harmonise the far- and near-field regimes and widen the applications of the technique with respect to the current knowledge. This study is supported by simulations and provides clear guidelines on how to optimise the setup and acquisition strategies for near-field ptychography experiments. The results are key to drive the translation of the technique towards low brilliance sources.

Studies employing nonlinear interactions of THz pulses are nowadays a promising scientific research field. To capture these phenomena, THz pulses with energy ranging from hundreds of to the mJ level are necessary. However, techniques that provide pulses with such energy levels are still not widely established. Upscaling methods of laser-solid interaction is limited by the damage threshold of materials, while the mechanism of THz generation from high intensity laser-gas interactions is not fully understood yet. Here, we establish the photocurrent model of laser-driven plasma THz generation in the high-intensity regime by accounting for high-ionization states of the target gas. Our model shows excellent agreement with experimental observations, provides a clear explanation of phenomena in both spectral and temporal domains, and explains the high conversion efficiency from laser to THz. In the experiments, we achieved a generation of 0.2 mJ THz pulses, driven by a Ti:sapphire laser with a conversion efficiency exceeding 1

This study explores nanoparticle-assisted electron injection as a method for controlling beam charge in laser wakefield acceleration through particle-in-cell simulations. We systematically investigate how the material (Li through Au) and size (50-200 nm) of nanoparticles influence electron injection dynamics and beam charge. Our results demonstrate that beam charge (10-600 pC) can be effectively controlled by adjusting these parameters. We identify a saturation threshold in the nanoparticle electric field strength, beyond which beam charge depends on the total number of atoms in the nanoparticle rather than on the electron density after ionization. Significant electron injection occurs across multiple plasma wave periods with distribution patterns influenced by nanoparticle properties, leading to increased beam charge but a broader energy spread. These findings offer practical guidelines for experimental implementation of nanoparticle-assisted injection in laser wakefield accelerators to tailor electron beam characteristics for various applications.