Numerous methods have been developed to retrieve the full temporal properties of ultrafast infrared laser pulses, and are presently implemented on laser facilities all around the world. We present here a technique, developed for the XUV domain, suitable to characterize any femtosecond to picosecond pulse, that can be routinely produced on the high variety of existing sources of high harmonics, free electron lasers, and plasma-based XUV lasers. Especially, the versatility is such that no limitation on any property of any potential source exists. Our technique relies on a frequency-resolved cross-correlation measurement between an infrared pulse and an XUV pulse, combined with a transient multiphoton absorption in gases. It provides temporal information on the longest of the two pulses: intensity profile, pulse duration, and possible presence of pre- or postpulses. More importantly, the measurement of resolved XUV spectra and the use of iterative phase-retrieval algorithms give access to phase information. The simplicity of the technique makes its implementation on various XUV beamlines straightforward.

We compared ultrafast spin dynamics in laser-excited Ni85Co15 alloy and pure Ni thin films exhibiting magnetic weak stripe domains using x-ray resonant magnetic scattering. By relying on extreme ultraviolet pulses obtained via high-harmonic generation, we simultaneously probed our samples using four energies around the Co and Ni M 2 , 3 edges. Our results show a significant laser-induced reduction of the intensity of the magnetic scattering peaks on fs timescales and clearly highlight that this effect depends sensitively on the probing wavelength: different quenching amplitudes and characteristic timescales are found when changing the probing energy. More particularly, in our alloyed thin film, we observe a delay of about 17 fs in the scattered intensity dynamics between probing energies close to the Ni and Co edges, respectively. This delay is not observed in the pure Ni sample and is therefore most likely induced by the presence of Co in the thin film, reflecting the different ultrafast magnetic responses of the two 3d metals in these alloys.

A new technique gives access to temporal and spectral characteristics of femtosecond duration XUV pulses. It is based on a frequency resolved cross-correlation be-tween XUV and IR lasers, through a transient absorption in gases.

Controlling magnetization without using magnetic fields is a technology-driven strong motivation in the quest for new electronic devices allowing for fast control with low energy consumption. A lot of results exist for ultrafast demagnetization in pure material (as pure Ni for example) but it is essential to understand this phenomenon in alloys or hetero structures since these systems present the highest potential for applications. We describe how we are using the chemical selectivity and the optical properties of the high harmonics to study the demagnetization induced by femtosecond laser pulses in thin nickel cobalt films presenting weak stripes magnetic domains.

This paper focuses on day-ahead electricity load forecasting for substations of the distribution network in France; therefore, the corresponding problem lies between the instability of a single consumption and the stability of a countrywide total demand. Moreover, this problem requires to forecast the loads of over one thousand substations; consequently, it belongs to the field of multiple time series forecasting. To that end, the paper applies an adaptive methodology that provided excellent results at a national scale; the idea is to combine generalized additive models with state-space representations. However, extending this methodology to the prediction of over a thousand time series raises a computational issue. It is solved by developing a frugal variant that reduces the number of estimated parameters: forecasting models are estimated only for a few time series and transfer learning is achieved by relying on aggregation of experts. This approach yields a reduction of computational needs and their associated emissions. Several variants are built, corresponding to different levels of parameter transfer, to find the best trade-off between accuracy and frugality. The selected method achieves competitive results compared to individual models. Finally, the paper highlights the interpretability of the models, which is important for operational applications.

We use time-resolved resonant magnetic scattering experiments to investigate the laser induced demagnetization of Co/Pt multilayers with large perpendicular magnetic anisotropy. Our pump-probe approach, which relies on extreme ultraviolet pulses obtained via high-harmonic generation, allows us to monitor the temporal evolution of the system in an element-selective fashion, thus to disentangle the contributions from permanent and proximity-induced magnetic moments. By analyzing the data gathered at the Co M2,3 and Pt O3 edges, we are able to show that after femtosecond laser irradiation, both components display a very similar loss of magnetic order, with almost identical demagnetization amplitudes and characteristic times, but a small delay (10–20 fs) of the Pt magnetization quenching with respect to Co. Comparing our experiments with literature results, therefore, suggests that in these 3d–5d multilayers and alloys, the different constituents remain strongly coupled after optical excitation; no matter whether the thin films possess a preferred in-plane or out-of-plane easy magnetization direction.

Instruments based on the magneto-optical Kerr effect are routinely used to probe surface magnetic properties. These tools rely on the characterization of the polarization state of reflected light from the sample to collect information on its magnetization. Here, we present a theoretical optimization of common setups based on the magneto-optical Kerr effect. A detection scheme based on a simple analyzer and photodetector and one made from a polarizing beam splitter and balanced photodetectors are considered. The effect of including a photoelastic modulator (PEM) and a lock-in amplifier to detect the signal at harmonics of the modulating frequency is studied. Jones formalism is used to derive general expressions that link the intensity of the measured signal to the magneto-optical Fresnel reflection coefficients for any orientation of the polarizing optical components. Optimal configurations are then defined as those that allow measuring the Kerr rotation and ellipticity while minimizing nonmagnetic contributions from the diagonal Fresnel coefficients in order to improve the signal-to-noise ratio (SNR). The expressions show that with the PEM, setups based on polarizing beam splitters inherently offer a twofold higher signal than commonly used analyzers, and the experimental results confirm that the SNR is improved by more than 150%. Furthermore, we find that while all proposed detection schemes measure Kerr effects, only those with polarizing beam splitters allow measuring the Kerr rotation directly when no modulator is included. This accommodates, for instance, time-resolved measurements at relatively low laser pulse repetition rates. Ultrafast demagnetization measurements are presented as an example of such applications.

The time profile of a lasing signal at 391.4 nm emitted by a weakly ionized gas of nitrogen molecules at low pressure is measured under double excitation with intense femtosecond laser pulses at 800 nm. An abrupt decrease in emission occurs at the time of arrival of the second pulse. It is explained by a transfer of population from ground to first excited ionic level and by a disruption of coherence, terminating the conditions for lasing in a V-scheme without population inversion.

Laser-plasma accelerators (LPA) deliver relativistic electron beams with high peak current and low emittance, with energies up to the GeV-level in only few centimetres. However, the divergence and the energy spread of these beams remain too large for potential light source applications. A magnetic transfer line can be used to manipulate the electron beam phase-space and select the transmitted energies with a slit located at its center. We will show that with a proper focusing optics along the line, one can tune the energy spread of the beam at a given energy without loss and produce undulator radiation with controlled bandwidth. We present analytic studies, numerical simulations and experimental results on the controled electron beam transport and application to undulator radiation with a control of the bandwidth.

The Free Electron Laser (FEL) application of Laser Plasma Acceleration (LPA) requires the handling of the energy spread and divergence. The COXINEL manipulation line, designed and built at SOLEIL for this purpose, consists of high gradient quadrupoles for divergence handling and a decompression chicane for energy sorting, enabling FEL amplification with baseline parameters. Installed at Laboratoire d’Optique Appliquee (LOA), it uses robust electrons generated and accelerated by ionization injection using a 30 TW laser. We report here on the work progress towards a FEL demonstration. The LPA measured electron beam characteristics deviates from the baseline reference case. After the installation of the equipment, the electron beam transport has first been optimized. The electron position and dispersion are independently adjusted. Then, undulator radiation has been measured. The spectral purity is controlled via the energy spread adjusted in the slit located in the chicane. FEL effect demonstration is within reach, with currently achieved performance on different LPA experiments.

Cavity-free lasing of N 2 + induced by a femtosecond laser pulse at 800 nm is nearly totally suppressed by a delayed twin control pulse. We explain this surprising effect within the V-scheme of lasing without population inversion. A fast transfer of population between nitrogen ionic states X 2 Σ g + and A 2 Π u , induced by the second pulse, terminates the conditions for amplification in the system. The appearance of short lasing bursts at delays corresponding to revivals of rotational wave packets is explained along the same lines.

Laser plasma acceleration (LPA) enables the generation of an up to several GeV electron beam with a short bunch length and high peak current within a centimeter scale. In view of undulator type light source applications, electron beam manipulation has to be applied. We report here on detailed electron beam transport for an LPA electron beam on the COXINEL test line, that consists of strong permanent quadrupoles to handle the electron beam divergence, a magnetic chicane to reduce the energy spread and a second set of quadrupoles for adjusting the focusing inside the undulator. After describing the measured LPA characteristics, we show that we can properly transport the electron beam along the line, thanks to several screens. We also illustrate the influence of the chromatic effects induced by the electron beam energy spread, both experimentally and numerically. We then study the sensitivity of the transport to the electron beam pointing and skewed quadrupolar components.

Since the laser invention [1, 2], the advent of Free Electron Lasers (FEL) [3, 4] in the X-ray domain half a century later, has opened new areas for matter investigation with higher temporal resolution. In parallel, the development of laser plasma acceleration (LPA) [5] that delivers today several GeV beam acceleration [6] in a short distance appears also very promising. The qualification of the LPA for FEL application can thus be viewed as an important challenge [7]. Nevertheless, present LPA electron beam parameters (e. g. energy spread and beam divergence) do not meet conventional accelerator state-of-the-art performance and FEL application requires a specific beam handling. In such a prospect, the COXINEL beam manipulation line [8, 9] using variable permanent magnet quadrupoles for emittance growth mitigation and de-mixing chicane for the energy spread handling developed at SOLEIL has been installed for using electrons produced with an intense laser of Laboratoire d'Optique Appliquee (LOA). Strategies for controlling electron beam position and dispersion have been elaborated and demonstrated [10]. Finally, undulator spontaneous emission has been measured at the end of the line.

The recent spectacular development of laser plasma ac- celerators that now can deliver GeV electron beams in an extremelyshortdistancemakesthemverypromising. Ap- plications for light sources based on undulator radiation and free electron laser appear as an intermediate step to move from an acceleration concept to an accelerator qual- ification. However, the presently achieved divergence and energy spread require some electron beam manipulations. The COXINEL test line was designed for enabling Free Elec- tron Laser operation with baseline reference parameters. It comprises variable permanent magnet quadrupoles for di- vergence handling, a magnetic chicane for electron energy sorting, a second set of quadrupole for chromatic focusing and an undulator for synchrotron radiation emission and/or free electron laser gain medium. The transport along the line is controlled [1]. The synchrotron radiation emitted by the undulator radiation is studied under different conditions of detection (CCD camera, spectrometer), electron beam manipulation and undulator parameters. These observations pave the way towards Laser Plasma Acceleration based Free Electron Laser.

Laser plasma acceleration (LPA) capable of providing femtosecond and GeV electron beams in cm scale distances brings a high interest for different applications, such as free electron laser and future colliders. Nevertheless, LPA high divergence and energy spread require an initial strong focus to mitigate the chromatic effects. The reliability, in particular with the pointing fluctuations, sets a real challenge for the control of the dispersion along the electron beam transport. We examine here how the magnetic defects of the first strong quadrupoles, in particular, the skew terms, can affect the brightness of the transported electron beam, in the case of the COXINEL transport line, designed for manipulating the electron beam properties for a free electron laser application. We also show that the higher the initial beam divergence, the larger the degradation. Experimentally, after having implemented a beam pointing alignment compensation method enabling us to adjust the position and dispersion independently, we demonstrate that the presence of non-negligible skew quadrupolar components induces a transversal spread and tilt of the beam, leading to an emittance growth and brightness reduction. We are able to reproduce the measurements with beam transport simulations using the measured electron beam parameters.

Undulator based synchrotron light sources and Free Electron Lasers (FELs) are valuable modern probes of matter with high temporal and spatial resolution. Laser Plasma Accelerators (LPAs), delivering GeV electron beams in few centimeters, are good candidates for future compact light sources. However the barriers set by the large energy spread, divergence and shot-to-shot fluctuations require a specific transport line, to shape the electron beam phase space for achieving ultrashort undulator synchrotron radiation suitable for users and even for achieving FEL amplification. Proof-of-principle LPA based undulator emission, with strong electron focusing or transport, does not yet exhibit the full specific radiation properties. We report on the generation of undulator radiation with an LPA beam based manipulation in a dedicated transport line with versatile properties. After evidencing the specific spatio-spectral signature, we tune the resonant wavelength within 200–300 nm by modification of the electron beam energy and the undulator field. We achieve a wavelength stability of 2.6%. We demonstrate that we can control the spatio-spectral purity and spectral brightness by reducing the energy range inside the chicane. We have also observed the second harmonic emission of the undulator.

LUNEX5 (free electron Laser Using a New accelerator for the Exploitation of X-ray radiation of 5th generation) aims at investigating the production of short, intense, coherent pulses in the 40-4 nm spectral range [1]. It comprises two types of accelerators connected to a single Free Electron Laser (FEL) for advanced seeding configurations (seeding with High order Harmonic in Gas, echo). A 400 MeV superconducting Linear Accelerator, adapted for studies of advanced FEL schemes, will enable future upgrade towards high repetition rate and multi-user operation by splitting part of the macropulse to different FEL lines. A 0.4 1 GeV Laser Wake Field Accelerator (LWFA) [2] will also be qualified by the FEL application. After the Conceptual Design Report, R&D has been launched on different sub components. Transport calculation of longitudinal and transverse manipulation of a LWFA electron beam enables to provide theoretical amplification, a test experiment is under preparation.

The original version of this Article contained an error in the last sentence of the first paragraph of the Introduction and incorrectly read ‘A proper electron beam control is one of the main challenges towards the Graal of developing a compact alternative of X-ray free-electron lasers by coupling LWFA gigaelectron-volts per centimetre acceleration gradient with undulators in the amplification regime in equation 11, nx(n-β) x β: n the two times and beta the two times should be bold since they are vectorsin Eq. 12, β should be bold as well.’ The correct version is ‘A proper electron beam control is one of the main challenges towards the Graal of developing a compact alternative of X-ray free-electron lasers by coupling LWFA gigaelectron-volts per centimetre acceleration gradient with undulators in the amplification regime.’This has been corrected in both the PDF and HTML versions of the Article.

We demonstrate experimentally the control of the polarization (ellipticity and polarization axis) of femtosecond high-order harmonics. The method relies on a two-color (omega - 2 omega) configuration, where both omega and 2 omega generating fields have linear polarizations with a variable crossing angle. We correlate our measurements with the conservation rules of energy and linear momentum accounting for harmonic generation in a two-color field. We evidence that the generation process, and especially the number of omega and 2 omega photons absorbed for generating a given harmonic, strongly depends on the crossing angle. Finally, relying on a simple formalism, we derive analytical formulae for calculating both polarization axis and ellipticity of the separate harmonics. The model corroborates our results and represents a base for future investigations.