Neutron-rich lanthanides were produced via in-flight fission of a U-238 primary beam at the RIBF, RIKEN Nishina Center to measure half-lives (T-1/2) and beta-delayed neutron emission probabilities (P-n) in order to constrain r-process abundance calculations. Pm159-166, Sm161-168, Eu165-170, and Gd167-172 ions were implanted in the Advanced Implantation Detector Array (AIDA), and beta-delayed neutrons and gamma-rays were detected by the surrounding detector array (BRIKEN). For the validation of T-1/2 values derived from implantation-beta (i-beta) time correlations, gamma-spectroscopic methods were used as well. The experimental results of the beta-delayed gamma-spectroscopy of Pm-162 are presented here as an example. A half-life value from gamma-decay curves was derived with a comparable uncertainty to the result from the i-beta method, and a mean value well within the 1 sigma range.

Production cross sections were measured for fragments produced by an 85 MeV/u 198Pt beam incident on a beryllium target. Event-by-event particle identification of A, Z, and q for the reaction products was performed by employing energy loss, time-of-flight, magnetic rigidity, and total kinetic energy measurements. Over 70 nuclei in the Hf-Pt region were identified, including three isotopes first observed in this work: 191,192Hf and 189Lu. Due to the existence of multiple charge states between H-like and C-like ions, a new analysis method was introduced, incorporating Monte Carlo calculations of charge state fractions for a given charge state of the projectile residue just after the reaction. For the first time, charge-state probability distribution functions after the reaction have been deduced from experimental data. This study provides insight into how to produce key nuclides near N=126 and the ability of a fragmentation residue to retain electrons from the primary beam.

At the RIKEN Nishina Center, exotic neutron-rich isotopes of Ba, La, Ce, Pr, and Nd were measured. This work reports their half-lives (T1/2) and β-delayed neutron-emission probabilities (Pxn). The setup consisted of the BigRIPS in-flight separator for particle identification, the Advanced Implantation Detector Array (AIDA) for ions and β detection, and the BRIKEN neutron counter for neutron detection. Using this arrangement, 4 new T1/2 and 14 new P1n were measured. Furthermore, 38 T1/2 and 2 P1n values were remeasured, decreasing the uncertainties for some of them. In addition to improving predictions of nucleosynthesis models that describe the production of the rare-earth peak at A ∼ 160 via the r-process, these additional experimental data should help to constrain theoretical models for calculations of T1/2 and Pxn in this region.

Half-lifes ( T 1/2 ) of exotic neutron-rich isotopes of Ba, La, Ce, Pr, and Nd were measured at the RIKEN Nishina Center. The experimental setup consisted of the BigRIPS in-flight separator for ion selection identification, the Advance Implantation Detector Array (AIDA) for ions and β detection, and the BRIKEN detector for neutron counting. Using this setup, 4 new T 1/2 have been measured for the first time, and 38 T 1/2 have been remeasured with improved precision in several cases. These new experimental data should help to constrain theoretical models for calculations of T 1/2 . The status of the experimental analysis and preliminary results are provided in this contribution.

The β-delayed neutron-emission probabilities of 28 exotic neutron-rich isotopes of Pm, Sm, Eu, and Gd were measured for the first time at RIKEN Nishina Center using the Advanced Implantation Detector Array (AIDA) and the BRIKEN neutron detector array. The existing β-decay half-life (T 1/2) database was significantly increased toward more neutron-rich isotopes, and uncertainties for previously measured values were decreased. The new data not only constrain the theoretical predictions of half-lives and β-delayed neutron-emission probabilities, but also allow for probing the mechanisms of formation of the high-mass wing of the rare-earth peak located at A ≈ 160 in the r-process abundance distribution through astrophysical reaction network calculations. An uncertainty quantification of the calculated abundance patterns with the new data shows a reduction of the uncertainty in the rare-earth peak region. The newly introduced variance-based sensitivity analysis method offers valuable insight into the influence of important nuclear physics inputs on the calculated abundance patterns. The analysis has identified the half-lives of 168Sm and of several gadolinium isotopes as some of the key variables among the current experimental data to understand the remaining abundance uncertainty at A = 167–172.

A CAEN DT5742 digitizer has been investigated to process the fast signals from the photomultiplier tubes of the time-of-flight detectors for fast ion beams. A test setup consisting of two plastic scintillation detectors and a pulsed laser source provided signals which were recorded by the digitizer and systematically analyzed with different algorithms to derive the amplitude, rise time and arrival time of the detection signal. To obtain the best amplitude and time resolutions, various optimization techniques including peak fitting and signal smoothing, interpolation improvement, and time-walk correction by amplitude and rise time have been performed and compared in detail. We compared the time resolutions obtained by three digital algorithms of leading-edge, zero-crossing constant-fraction (ZC-CFD) and direct constant-fraction discriminations. Finally, we found that the best time-of-flight resolution between two PMTs can be achieved as 12 ps by the method using sample minimum for peak location and using the time-walk-resistant ZC-CFD with 4-point interpolation for timing.

Fast timing detectors are an essential element in the experimental setup for time-of-flight (ToF) mass measurements of unstable nuclei. We have upgraded the scintillator detectors used in experiments at the National Superconducting Cyclotron Laboratory (NSCL) by increasing the number of photomultiplier tubes that read out their light signals to four per detector, and characterized them in a test experiment with 48Ca beam at the NSCL. The new detectors achieved a time resolution (σ) of 7.5 ps. We systematically investigated different factors that affect their timing performance. In addition, we evaluated the ability of positioning the hitting points on the scintillator using the timing information and obtained a resolution (σ) below 1 mm for well-defined beam spots.