Hybrid photonic quantum computers, combining stationary matter qubits and flying photonic qubits, offer an intrinsically networked and resource-efficient route to large-scale, error-corrected quantum computation. Their core components are cavity-coupled matter qubits that act as light–matter interfaces, enabling: high-efficiency on-demand single-photon generation, stable near-unity photon indistinguishability and spin–multi-photon entanglement. Semiconductor quantum dots in microcavities are a leading platform for realizing such devices. Yet reaching the performance, reproducibility and spin-coherence thresholds for large-scale error correction remains a major challenge requiring industrial fabrication and control. Here we report thousands of monolithic semiconductor quantum-dot devices fabricated using a III–V pilot production-line process compatible with large-scale deployment. Systematic control of source parameters yields state-of-the-art efficiency and supports a path to optical losses below fault-tolerance thresholds. Using field-quadrature state reconstruction as a stringent joint test of efficiency and indistinguishability, we observe near-unity photon quantum purity stable over tens of minutes and a record single-photon Wigner-function negativity. We further demonstrate seven-partite spin–multi-photon entanglement and spin coherence extendable to microsecond timescales in the low-magnetic-field regime. Finally, photons from distant sources are as indistinguishable as photons emitted successively by a single source. These results establish foundry-compatible III–V quantum dots as a scalable platform for hybrid photonic quantum computing.

Light-matter interfaces are pivotal for quantum computation and communication. While typically analyzed using single-mode or open-quantum-system approximations, these models often neglect multi-mode field states and light-matter entanglement, hindering exact protocol modeling. Here, we solve the full Hamiltonian dynamics of a solid-state spin-photon interface for three key protocols: the generation of photon-number superpositions, a controlled photon-photon gate, and the production of photonic cluster states. By deriving exact fidelities, we identify fundamental performance limits. Our results reveal that while realistic imperfections severely limit photon-photon gates, they only slightly affect linear photonic clusters and are nearly harmless for photon-number state superpositions.

Coherent light-matter interfaces controllably modifying the state of a photon upon interaction with a stationary qubit are a key resource for implementing deterministic entangling gates for optical quantum technologies. This requires a one-to-one mapping between the state of the scattered photon and that of the embedded qubit. Here, we present an experimental signature of such a bijection by leveraging the spin-induced Kerr rotation present in a low-noise charged quantum dot-micropillar cavity device. Through time-resolved polarization measurements, we project the electron spin to one of its eigenstates with 95±2% fidelity with a single reflected photon detection, and follow the subsequent spin relaxation through the detection of a second reflected photon. We demonstrate that, after a transient regime governed by the trion radiative lifetime, two orthogonal polarization states can be produced, each associated to a given spin eigenstate. While the current results are limited by a timescale competition between electron spin relaxation and trion radiative lifetime, they could be improved using hole spins displaying increased relaxation times. Our work paves the way towards deterministic logic gates exploiting this one-to-one mapping between a spin and the polarization of a scattered photon.

Polarization-encoded spin-photon interfaces constitute promising candidates for the development of stationary nodes used as photon receivers, for quantum communication and distributed quantum computing. Here we introduce a time-resolved tomography approach which allows observing the dynamics of an electron spin, in a semiconductor quantum dot, mapped onto the dynamics of the polarization state of reflected photons. Through a single tomography experiment, we infer all the relevant spin dynamics timescales, including precession, decoherence and relaxation times. We also demonstrate and quantify the measurement back-action induced, on the embedded spin qubit, by the detection of a single reflected photon. We show that the induced population and coherence of the spin state can be tuned by the chosen polarization basis of the measurement. The control of the photon-induced back-action on the embedded spin qubit constitutes a crucial requirement for the use of spin-photon interfaces as quantum receivers.

Spin noise spectroscopy has become a widespread technique to extract information on spin dynamics in atomic and solid-state systems, in a potentially nonperturbative way. Here we experimentally demonstrate a new approach in spin noise spectroscopy, based on the detection of single photons. Because of the large spin-dependent polarization rotations provided by a deterministically coupled quantum dot-micropillar device, giant spin noise signals induced by a single-hole spin are extracted in the form of photon-photon cross-correlations. Ultimately, such a technique can be extended to an ultrafast regime probing mechanisms down to few tens of picoseconds.

Generating identical photons from remote emitter-based bright single-photon sources is an important step for scaling up optical quantum technologies. Here, we study the Hong-Ou-Mandel interference of photons emitted from remote sources based on semiconductor quantum dots (QDs). We make use of a deterministic fabrication technique to position the QDs in a spectrally resonant micropillar cavity and fine-tune their operation wavelength electrically. In doing so, we can match four pairs of sources between five distinct sources, study them under various excitation schemes, and measure their degree of indistinguishability. We demonstrate remote indistinguishabiltity between 44 ± 1% and 69 ± 1% depending on the pair of sources and excitation conditions, record values for QDs in cavities. The relative contribution of pure dephasing and spectral diffusion is then analyzed, revealing that the remaining distinguishability is mostly due to low-frequency noise.

Self-assembled InGaAs/GaAs quantum dots (QDs) are of particular importance for the deterministic generation of spin-photon entanglement. One promising scheme relies on the Larmor precession of a spin in a transverse magnetic field, which is governed by the in-plane $g$-factors of the electron and valence band heavy-hole. We probe the origin of heavy-hole $g$-factor anisotropy with respect to the in-plane magnetic field direction and uncover how it impacts the entanglement generated between the spin and the photon polarization. First, using polarization-resolved photoluminescence measurements on a single QD, we determine that the impact of valence-band mixing dominates over effects due to a confinement-renormalized cubic Luttinger $q$ parameter. From this, we construct a comprehensive hole $g$-tensor model. We then use this model to simulate the concurrence and fidelity of spin-photon entanglement generation with anisotropic hole $g$-factors, which can be tuned via magnetic field angle and excitation polarization. The results demonstrate that post-growth control of the hole $g$-factor can be used to improve spin-photon cluster state generation.

The frequency or color of photons is an attractive degree of freedom to encode and distribute quantum information over long distances. However, the generation of frequency-encoded photonic qubits has so far relied on probabilistic nonlinear single-photon sources and inefficient gates. Here, we demonstrate the deterministic generation of photonic qubits hyper-encoded in frequency and polarization based on a semiconductor quantum dot in a cavity. We exploit the double dipole structure of a neutral exciton and demonstrate the generation of any quantum superposition in amplitude and phase, controlled by the polarization of the pump laser pulse. The source generates frequency-polarization single-photon qubits at a rate of 4 MHz corresponding to a generation probability at the first lens of 28 +/- 2%, with a photon number purity >98%. The photons show an indistinguishability >91% for each dipole and 88% for a balanced quantum superposition of both. The density matrix of the hyper-encoded photonic state is measured by time-resolved polarization tomography, evidencing a fidelity to the target state of 94 +/- 8% and concurrence of 77 +/- 2%, here limited by frequency overlap in our device. Our approach brings the advantages of quantum dot sources to the field of quantum information processing based on frequency encoding.

Quantum key distribution is a key application of quantum mechanics, shaping the future of privacy and secure communications. Many protocols require single photons, often approximated by strongly attenuated laser pulses. Here, we harness the emission of a quantum dot embedded in a micropillar and explore a hybrid approach where the information is encoded on a mixture of single photons and laser pulses. We derive a phenomenological analysis of the configuration where both sources of light are mixed incoherently to perform the BB84 protocol, showing nearly perfect matching between theory and experiment. This provides a flexible technology compensating limited collected brightnesses of single-photon sources as well as a thorough investigation of single-photon statistics advantage scenarios over Poisson-distributed statistics. Explicitly, our model highlights an efficiency threshold for unconditional advantage of single photons over laser along with insights on the interplay between single-photon purity and collected brightness in the performances of BB84.

Accessing acoustic phonons at high frequencies in nanostructures becomes more and more essential in nanoelectronics, nano- and opto-mechanics and quantum technologies, as phonons can strongly interact with electrons and photons at the nanoscale. In spontaneous Brillouin scattering processes, the scattered photons energy, direction and polarisation are constrained by selection rules for a given input state. These selection rules are usually considered as intrinsic material properties in crystalline solids and the polarisation of the scattered photons depends on the polarisation of the excitation. In this work, we use elliptical optophononic micropillar resonators to control these optical polarisation selection rules. The degeneracy of the optical cavity modes of circular micropillars is lifted due to the elliptical cross-section of the micropillars, leading to two cavity modes orthogonally polarised and split in energy. The optical field polarisation state will depend on both orthogonal cavity modes and their associated polarisation states. Therefore, an incident laser beam linearly polarised along the diagonal axis of the elliptical pillar undergoes a wavelength dependent polarisation rotation. By choosing the polarisation and wavelength of the incident laser, we demonstrate that the polarisation state of the incident and reflected laser and the Brillouin scattering signal are different. In this way, background-free spontaneous Brillouin scattering spectra can be efficiently measured in a cross-polarisation scheme down to 18 GHz. Here, we theoretically and experimentally explore the optimal conditions for the polarisation and wavelength of the incident laser, and the ellipticity of the micropillars, to improve the polarisation-based filtering applied to Brillouin spectroscopy.

Abstract In the framework of optical quantum computing and communications, a major objective consists in building receiving nodes implementing conditional operations on incoming photons, using a single stationary qubit. In particular, the quest for scalable nodes motivated the development of cavity-enhanced spin-photon interfaces with solid-state emitters. An important challenge remains, however, to produce a stable, controllable, spin-dependent photon state, in a deterministic way. Here we use an electrically-contacted pillar-based cavity, embedding a single InGaAs quantum dot, to demonstrate giant polarisation rotations induced on reflected photons by a single electron spin. A complete tomography approach is introduced to extrapolate the output polarisation Stokes vector, conditioned by a specific spin state, in presence of spin and charge fluctuations. We experimentally approach polarisation states conditionally rotated by $$\frac{\pi }{2}$$ π 2 , π, and $$-\frac{\pi }{2}$$ − π 2 in the Poincaré sphere with extrapolated fidelities of (97 ± 1) %, (84 ± 7) %, and (90 ± 8) %, respectively. We find that an enhanced light-matter coupling, together with limited cavity birefringence and reduced spectral fluctuations, allow targeting most conditional rotations in the Poincaré sphere, with a control both in longitude and latitude. Such polarisation control may prove crucial to adapt spin-photon interfaces to various configurations and protocols for quantum information.

Spin-photon interfaces (SPIs) are key devices of quantum technologies, aimed at coherently transferring quantum information between spin qubits and propagating pulses of polarized light. We study the potential of a SPI for quantum non demolition (QND) measurements of a spin state. After being initialized and scattered by the SPI, the state of a light pulse depends on the spin state. It thus plays the role of a pointer state, information being encoded in the light's temporal and polarization degrees of freedom. Building on the fully Hamiltonian resolution of the spin-light dynamics, we show that quantum superpositions of zero and single photon states outperform coherent pulses of light, producing pointer states which are more distinguishable with the same photon budget. The energetic advantage provided by quantum pulses over coherent ones is maintained when information on the spin state is extracted at the classical level by performing projective measurements on the light pulses. The proposed schemes are robust against imperfections in state of the art semi-conducting devices.

Spontaneous Brillouin scattering in bulk crystalline solids is governed by the intrinsic selection rules locking the relative polarization of the excitation laser and the Brillouin signal. In this work, we independently manipulate the polarization of the two by employing polarization-sensitive optical resonances in elliptical micropillars to induce a wavelength-dependent rotation of the polarization states. Consequently, a polarization-based filtering technique allows us to measure acoustic phonons with frequencies difficult to access with standard Brillouin and Raman spectroscopies. This technique can be extended to other polarization-sensitive optical systems, such as plasmonic, photonic, or birefringent nanostructures, and finds applications in optomechanical, optoelectronic, and quantum optics devices.

Spins in semiconductor quantum dots (QDs) are promising local quantum memories to generate polarization-encoded photonic cluster states, as proposed in the pioneering Lindner and Rudolph scheme (2009 Phys. Rev. Lett. 103 113602). However, harnessing the polarization degree of freedom of the optical transitions is hindered by resonant excitation schemes that are widely used to obtain high photon indistinguishability. Here we show that acoustic phonon-assisted excitation, a scheme that preserves high indistinguishability, also allows to fully exploit the polarization selective optical transitions to initialise and measure single spin states. We access the coherence of hole spin systems in a low transverse magnetic field and directly monitor the spin Larmor precession both during the radiative emission process of an excited state or in the QD ground state. We report a spin state detection fidelity of 94.7 +/- 0.2% granted by the optical selection rules and a 25 +/- 5 ns hole spin coherence time, demonstrating the potential of this scheme and system to generate linear cluster states with a dozen of photons.

Photonic graph states, quantum light states where multiple photons are mutually entangled, are key resources for optical quantum technologies. They are notably at the core of error-corrected measurement-based optical quantum computing and all-optical quantum networks. In the discrete variable framework, these applications require high efficiency generation of cluster-states whose nodes are indistinguishable photons. Such photonic cluster states can be generated with heralded single photon sources and probabilistic quantum gates, yet with challenging efficiency and scalability. Spin-photon entanglement has been proposed to deterministically generate linear cluster states. First demonstrations have been obtained with semiconductor spins achieving high photon indistinguishablity, and most recently with atomic systems at high collection efficiency and record length. Here we report on the efficient generation of three partite cluster states made of one semiconductor spin and two indistinguishable photons. We harness a semiconductor quantum dot inserted in an optical cavity for efficient photon collection and electrically controlled for high indistinguishability. We demonstrate two and three particle entanglement with fidelities of 80 % and 63 % respectively, with photon indistinguishability of 88%. The spin-photon and spin-photon-photon entanglement rates exceed by three and two orders of magnitude respectively the previous state of the art. Our system and experimental scheme, a monolithic solid-state device controlled with a resource efficient simple experimental configuration, are very promising for future scalable applications.

Semiconductor quantum dots have emerged as excellent artificial atoms to both generate and manipulate quantum light. When embedded in cavities, they can generate single photons and entangled photons with unparalleled efficiency and high quantum purity. In this talk, I will discuss how such devices can be used to generate strings of many entangled photons. The method, leveraging the spin-selective optical transition in a charged quantum dot, leads to the generation of indistinguishable photons in linear cluster states or GHZ states at high rates, realizing an important milestone for scaling-up optical quantum technologies.

In the framework of optical quantum computing and communications, a major objective consists in building receiving nodes that implement conditional operations on incoming photons, using the interaction with a single stationary qubit. In particular, the quest for scalable nodes motivated the development of cavity-enhanced spin-photon interfaces with solid-state emitters. An important challenge remains, however, to produce a stable, controllable, spin-dependant photon state, in a deterministic way. Here we use a pillar-based high-Q cavity, embedding a singly-charged semiconductor quantum dot, to demonstrate the control of giant polarisation rotations induced by a single electron spin. A complete tomography approach is used to deduce the output polarisation Stokes vector, conditioned by a single spin state. We experimentally demonstrate rotation amplitudes such as $\pm \frac{\pi}{2}$ and $\pi$ in the Poincar\'e sphere, as required for applications based on spin-polarisation mapping and spin-mediated photon-photon gates. In agreement with our modeling, we observe that the environmental noise does not limit the amplitude of the spin-induced rotation, yet slightly degrades the polarisation purity of the output states. We find that the polarisation state of the reflected photons can be manipulated in most of the Poincar\'e sphere, through controlled spin-induced rotations, thanks to moderate cavity birefringence and limited noise. This control allows the operation of spin-photon interfaces in various configurations, including at zero or low magnetic fields, which ensures compatibility with key protocols for photonic cluster state generation.

The excitonic fine structure plays a key role for the quantum light generated by semiconductor quantum dots, both for entangled photon pairs and single photons. Controlling the excitonic fine structure has been demonstrated using electric, magnetic, or strain fields, but not for quantum dots in optical cavities, a key requirement to obtain high source efficiency and near-unity photon indistinguishability. Here, we demonstrate the control of the fine structure splitting for quantum dots embedded in micropillar cavities. We propose and implement a scheme based on remote electrical contacts connected to the pillar cavity through narrow ridges. Numerical simulations show that such a geometry allows for a three-dimensional control of the electrical field. We experimentally demonstrate tuning and reproducible canceling of the fine structure, a crucial step for the reproducibility of quantum light source technology.

Entanglement and spontaneous emission are fundamental quantum phenomena that drive many applications of quantum physics. During the spontaneous emission of light from an excited two-level atom, the atom briefly becomes entangled with the photonic field. Here we show that this natural process can be used to produce photon-number entangled states of light distributed in time. By exciting a quantum dot—an artificial two-level atom—with two sequential π-pulses, we generate a photon-number Bell state. We characterize this state using time-resolved intensity and phase correlation measurements. Furthermore, we theoretically show that applying longer sequences of pulses to a two-level atom can produce a series of multi-temporal mode entangled states with properties intrinsically related to the Fibonacci sequence. Our results on photon-number entanglement can be further exploited to generate new states of quantum light with applications in quantum technologies.

Semiconductor quantum dots in cavities are promising single-photon sources. Here, we present a path to deterministic operation, by harnessing the intrinsic linear dipole in a neutral quantum dot via phonon-assisted excitation. This enables emission of fully polarized single photons, with a measured degree of linear polarization up to 0.994±0.007, and high population inversion-85% as high as resonant excitation. We demonstrate a single-photon source with a polarized first lens brightness of 0.50±0.01, a single-photon purity of 0.954±0.001, and single-photon indistinguishability of 0.909±0.004.