Imperfections in X-ray imaging systems can limit their performance, especially in High Energy Density (HED) or Inertial Fusion Energy (IFE)-relevant experiments that are typically single shot, by introducing structured, non-stationary features that overlap with the signal of interest. When the X-ray transmission is reconstructed by typical flat-field normalization, even small shot-to-shot drift of structured features imprints residual patterns onto transmission maps, degrading signal visibility and biasing measurements such as electron density, velocity and feature sizes. We investigate this limitation by modeling the artifacts as a separable feature layer and training a U-Net architecture to estimate and infer them directly from the experimental data. We compare our method against Fourier filtering and more advanced procedures like Dynamic Flat-Field Normalization (DFFN) to evaluate artifact suppression capability and signal preservation in the reconstructed transmission maps. In multiple synthetic injection tests, our Physics-Guided Deep Learning approach is able to obtain an improvement in mean Structural Similarity Index (SSIM) from 0.345 to 0.906 and from 0.0679 to 0.945, while better preserving filament profiles and reducing degradation of the filament signal during artifact suppression. Additionally, we utilize deep ensembles to obtain predictive epistemic uncertainty estimates for the U-Net based reconstruction, to ensure Out Of Distribution (OOD) robustness for this procedure.
We consider a compact isotrajectory-optics scheme for proton radiography. The calculation uses a 30-60 MeV proton interval as a reference example, typical of high-energy short-pulse laser acceleration in the TNSA regime. The idea is to use synchronized time-dependent fields such that, for one selected energy-arrival-time branch, the proton energy changes mainly the arrival time and not the transverse image position. The reference lattice consists of four pulsed electric quadrupoles with horizontal sign pattern + - + -, magnification Mx = My = -3.0 at a detector plane of 2.57 m, a common Fourier plane at zF = 0.962 m, and equal outer and equal inner lens lengths. The ideal closure residual is calculated from second central moments. Fourth central moments are kept separately as a diagnostic of non-Gaussian tails. The quoted residual widths are numerical closure tests of the ideal map, not experimental resolution predictions. Real electrode fields, waveform errors, scattering, detector blur, and space charge define the next level of the problem.
The robust diagnosis of conditions generated in warm dense matter experiments remains a persistent challenge. Here, we describe the measurement of shock-compressed aluminium at 50 GPa with angle-resolved femtosecond x-ray Thomson scattering (XRTS) over a wide range of scattering wave vectors at the European X-Ray Free-Electron Laser. The measured plasmon dispersion and line shape show that the de facto standard approach for analyzing XRTS spectra, using uniform-electron-gas models, systematically overestimates the resonance energy by up to 8 eV. We present an approach using ab initio methods that agrees within the experimental uncertainty and demonstrates how accounting for shock-induced disorder in shock-compressed systems is critical for their understanding, providing evidence that ab initio treatments are required for reliable XRTS inference in warm dense aluminium.
This roadmap presents the state-of-the-art, current challenges and near future developments anticipated in the thriving field of warm dense matter physics. Originating from strongly coupled plasma physics, high pressure physics and high energy density science, the warm dense matter physics community has recently taken a giant leap forward. This is due to spectacular developments in laser technology, diagnostic capabilities, and computer simulation techniques. Only in the last decade has it become possible to perform accurate enough simulations & experiments to truly verify theoretical results as well as to reliably design experiments based on predictions. Consequently, this roadmap discusses recent developments and contemporary challenges that are faced by theoretical methods, and experimental techniques needed to create and diagnose warm dense matter. A large part of this roadmap is dedicated to specific warm dense matter systems and applications in astrophysics, inertial confinement fusion and novel material synthesis.
Microstructured foams are emerging as a promising class of targets, with applications ranging from laser-driven particle acceleration to inertial confinement fusion. To unlock their full potential, a deeper understanding of their properties, especially the changes and behavior of the microstructure under extreme conditions, is required. While recently advancing 3D printed foam targets can be observed by X-ray radiography, the microstructure in chemically produced targets is far below the spatial resolution of conventional radiography. To overcome this limitation, we apply grating-based X-ray dark-field imaging to observe structural changes in foams that are rapidly heated by laser-accelerated proton pulses. The experimental data is compared to synthetic dark-field values obtained from hydrodynamic simulations of a simplified foam model. Both experimental and simulation results demonstrate the viability of utilizing grating-based dark-field imaging for observing microstructural changes in foam targets.
We report on commissioning experiments at the high-energy, high-temperature (HHT) target area at the GSI Helmholtzzentrum für Schwerionenforschung GmbH, Darmstadt, Germany, combining for the first time intense pulses of heavy ions from the SIS18 synchrotron with high-energy laser pulses from the PHELIX laser facility. We demonstrate the use of X-ray diagnostic techniques based on intense laser-driven X-ray sources, which will allow probing of large samples volumetrically heated by the intense heavy-ion beams. A new target chamber as well as optical diagnostics for ion-beam characterization and fast pyrometric temperature measurements complement the experimental capabilities. This platform is designed for experiments at the future Facility for Antiproton and Ion Research in Europe GmbH (FAIR), where unprecedented ion-beam intensities will enable the generation of millimeter-sized samples under high-energy-density conditions.
In this work, we discuss the challenges related to the preliminary investigation of high repetition rate (HRR) experiments in the field of high energy density (HED) physics, and we present the results of preparation experiments done at the Prague Asterix Laser System (PALS) laser facility conducted with the aim of defining the needed developments in target design, real-time diagnostics and data collection needed to meet HRR requirements. Although the PALS laser facility is not an HRR facility, it has served as a valuable test bed for advancing diagnostic techniques and refining target design in preparation for HRR experimental platforms. HRR operation will result in improved statistical errors of the experimental results, in particular for experiments related to equation of state studies in extreme conditions.
The possibility of existence of carbon-rich-planets makes it important to study High Energy States of carbon in order to understand the internal structure of such planets. In this paper, we present two-dimensional hydrodynamic simulations of a low-entropy compression of a carbon sample that is enclosed in a high-Z cylindrical shell that is driven by a high intensity uranium beam. The considered beam parameters are the ones that will be available at the accelerator facility, named, FAIR, at Darmstadt. This study has shown that the carbon sample can be compressed to 2 to 3 times solid density and ultra-high pressures are achieved. The temperature, on the other hand, remains relatively low. These are the typical physical conditions that are expected to exist in the planetary interiors. An experimental study of the thermophysical and transport properties of such samples will significantly improve our knowledge about formation and evolution of different type of planets.
The high-energy/high-intensity laser facility PHELIX of the GSI Helmholtzzentrum für Schwerionenforschung in Darmstadt,Germany,has been in operation since 2008.Here,we review the current system performance,which is the result of continuous development and further improvement.Through its versatile frontend architecture,PHELIX can be operated in both long-and short-pulse modes,corresponding to ns-pulses with up to 1 kJ pulse energy and sub-ps,200 J pulses,respectively.In the short-pulse mode,the excellent temporal contrast and the control over the wavefront make PHELIX an ideal driver for secondary sources of high-energy ions,neutrons,electrons and X-rays.The long-pulse mode is mainly used for plasma heating,which can then be probed by the heavy-ion beam of the linear accelerator of GSI.In addition,PHELIX can now be used to generate X-rays for studying exotic states of matter created by heavy-ion heating using the ion beam of the heavy-ion synchrotron of GSI.
Mosaic crystals, with their high integrated reflectivities, are widely employed in spectrometers used to diagnose high energy density systems. X-ray Thomson scattering (XRTS) has emerged as a powerful diagnostic tool of these systems, providing in principle direct access to important properties such as the temperature via detailed balance. However, the measured XRTS spectrum is broadened by the spectrometer instrument function (IF), and without careful consideration of the IF one risks misdiagnosing system conditions. Here, we consider in detail the IF of 40 and 100 μm mosaic Highly Annealed Pyrolytic Graphite crystals, and how the broadening varies across the spectrometer in an energy range of 6.7–8.6 keV. Notably, we find a strong asymmetry in the shape of the IF toward higher energies. As an example, we consider the effect of the asymmetry in the IF on the temperature inferred via XRTS for simulated 80 eV CH plasmas and find that the temperature can be overestimated if an approximate symmetric IF is used. We, therefore, expect a detailed consideration of the full IF will have an important impact on system properties inferred via XRTS in both forward modeling and model-free approaches.
Multi-wavelength pyrometry is an efficient tool for measuring high temperatures in dynamic experiments. A fast 5-channel pyrometer was built and successfully employed in ion-beam heating experiments at the GSI Centre for Heavy Ion Research (Darmstadt, Germany). Temperatures of metallic samples heated by an intense focused heavy ion beam up to their melting points and beyond were measured with nanosecond time resolution and a spatial resolution of about 200 μm. The modular instrument has demonstrated its high versatility also for temperature measurements of exothermic reactions with millisecond temporal resolution.
Single-shot X-ray phase-contrast imaging is used to take high-resolution images of laser-driven strong shock waves. Employing a two-grating Talbot interferometer, we successfully acquire standard absorption, differential phase-contrast, and dark-field images of the shocked target. Good agreement is demonstrated between experimental data and the results of two-dimensional radiation hydrodynamics simulations of the laser–plasma interaction. The main sources of image noise are identified through a thorough assessment of the interferometer’s performance. The acquired images demonstrate that grating-based phase-contrast imaging is a powerful diagnostic tool for high-energy-density science. In addition, we make a novel attempt at using the dark-field image as a signal modality of Talbot interferometry to identify the microstructure of a foam target.
We present in situ measurements of spectrally resolved X-ray scattering and X-ray diffraction from monocrystalline diamond samples heated with an intense pulse of heavy ions. In this way, we determine the samples’ heating dynamics and their microscopic and macroscopic structural integrity over a timespan of several microseconds. Connecting the ratio of elastic to inelastic scattering with state-of-the-art density functional theory molecular dynamics simulations allows the inference of average temperatures around 1300 K, in agreement with predictions from stopping power calculations. The simultaneous diffraction measurements show no hints of any volumetric graphitization of the material, but do indicate the onset of fracture in the diamond sample. Our experiments pave the way for future studies at the Facility for Antiproton and Ion Research, where a substantially increased intensity of the heavy ion beam will be available.
We present numerical simulations used to interpret laser-driven plasma experiments at the GSI Helmholtz Centre for Heavy Ion Research. The mechanisms by which non-thermal particles are accelerated in astrophysical environments, e.g., the solar wind, supernova remnants, and gamma ray bursts, is a topic of intense study. When shocks are present, the primary acceleration mechanism is believed to be first-order Fermi, which accelerates particles as they cross a shock. Second-order Fermi acceleration can also contribute, utilizing magnetic mirrors for particle energization. Despite this mechanism being less efficient, the ubiquity of magnetized turbulence in the universe necessitates its consideration. Another acceleration mechanism is the lower-hybrid drift instability, arising from gradients of both density and magnetic field, which produce lower-hybrid waves with an electric field that energizes particles as they cross these waves. With the combination of high-powered laser systems and particle accelerators, it is possible to study the mechanisms behind cosmic-ray acceleration in the laboratory. In this work, we combine experimental results and high-fidelity three-dimensional simulations to estimate the efficiency of ion acceleration in a weakly magnetized interaction region. We validate the FLASH magneto-hydrodynamic code with experimental results and use OSIRIS particle-in-cell code to verify the initial formation of the interaction region, showing good agreement between codes and experimental results. We find that the plasma conditions in the experiment are conducive to the lower-hybrid drift instability, yielding an increase in energy Delta E of similar to 264 keV for 242 MeV calcium ions.
On December 5, 2022, an indirect drive fusion implosion on the National Ignition Facility (NIF) achieved a target gain G_{target} of 1.5. This is the first laboratory demonstration of exceeding "scientific breakeven" (or G_{target}>1) where 2.05 MJ of 351 nm laser light produced 3.1 MJ of total fusion yield, a result which significantly exceeds the Lawson criterion for fusion ignition as reported in a previous NIF implosion [H. Abu-Shawareb et al. (Indirect Drive ICF Collaboration), Phys. Rev. Lett. 129, 075001 (2022)PRLTAO0031-900710.1103/PhysRevLett.129.075001]. This achievement is the culmination of more than five decades of research and gives proof that laboratory fusion, based on fundamental physics principles, is possible. This Letter reports on the target, laser, design, and experimental advancements that led to this result.
Laser -driven shock waves in matter propagate with multiple kilometers per second and therefore require sources like a laser -driven backlighter, which emit the X-rays within picoseconds, to be able to capture sharp images. The small spatial extent of shocks in low -density materials pose challenges on the imaging setup. In this work, we present a design process for a single -shot X-ray phase -contrast imaging system geared towards these objects, consisting of a two -grating Talbot interferometer and a digital X-ray detector. This imaging system is optimized with respect to the detectable refraction angle of the X-rays induced by an object, which implies a high phase sensitivity. Therefore, an optimization parameter is defined that considers experimental constraints such as the limited number of photons, the required magnification, the size and spectrum of the X-ray source, and the visibility of the moir & eacute; fringes. In this way, a large parameter space is sampled and a suitable imaging system is chosen. During a campaign at the PHELIX high -power laser facility a static test sample was imaged which is used to benchmark the optimization process and the imaging system under real conditions. The results show good agreement with the predicted performance, which demonstrates the reliability of the presented design process. Likewise, the process can be adapted to other types of laser experiments or X-ray sources and is not limited to the application presented here.
We demonstrate a significantly simplified experimental approach for investigating liquid metallic hydrogen, which is crucial to understand the internal structure and evolution of giant planets. Plastic samples were shock-compressed and then probed by short pulses of X-rays generated by free electron lasers. By comparison with ab initio simulations, we provide indirect evidence for the creation of elemental hydrogen in shock-compressed plastics at -150 GPa and -5, 000 K and thus in a regime where hydrogen is predicted to be metallic. Being the most common form of condensed matter in our solar system, and ostensibly the simplest of all elements, hydrogen is the model case for many theoretical studies and we provide a new possibility to benchmark models for conditions with extreme pressures and temperatures. Moreover, this approach will also allow to probe the chemical behavior of metallic hydrogen in mixture with other elements, which, besides its importance for planetary physics, may open up promising pathways for the synthesis of new materials.
Diamonds are supposedly abundantly present in different objects in the Universe including meteorites, carbon-rich stars as well as carbon-rich extrasolar planets. Moreover, the prediction that in deep layers of Uranus and Neptune, methane may undergo a process of phase separation into diamond and hydrogen, has been experimentally verified. In particular, high power lasers have been used to study this problem. It is therefore important from the point of view of astrophysics and planetary physics, to further study the production processes of diamond in the laboratory. In the present paper, we present numerical simulations of implosion of a solid carbon sample using an intense uranium beam that is to be delivered by the heavy ion synchrotron, SIS100, that is under construction at the Facility for Antiprotons and Ion Research (FAIR), at Darmstadt. These calculations show that using our proposed experimental scheme, one can generate the extreme pressure and temperature conditions, necessary to produce diamonds of mm3 dimensions.
The gravitational pressure in many astrophysical objects exceeds one gigabar (one billion atmospheres)1-3, creating extreme conditions where the distance between nuclei approaches the size of the K shell. This close proximity modifies these tightly bound states and, above a certain pressure, drives them into a delocalized state4. Both processes substantially affect the equation of state and radiation transport and, therefore, the structure and evolution of these objects. Still, our understanding of this transition is far from satisfactory and experimental data are sparse. Here we report on experiments that create and diagnose matter at pressures exceeding three gigabars at the National Ignition Facility5 where 184 laser beams imploded a beryllium shell. Bright X-ray flashes enable precision radiography and X-ray Thomson scattering that reveal both the macroscopic conditions and the microscopic states. The data show clear signs of quantum-degenerate electrons in states reaching 30 times compression, and a temperature of around two million kelvins. At the most extreme conditions, we observe strongly reduced elastic scattering, which mainly originates from K-shell electrons. We attribute this reduction to the onset of delocalization of the remaining K-shell electron. With this interpretation, the ion charge inferred from the scattering data agrees well with ab initio simulations, but it is significantly higher than widely used analytical models predict6.
This work presents first insights into the dynamics of free-surface release clouds from dynamically compressed polystyrene and pyrolytic graphite at pressures up to 200 GPa, where they transform into diamond or lonsdaleite, respectively. These ejecta clouds are released into either vacuum or various types of catcher systems, and are monitored with high-speed recordings (frame rates up to 10 MHz). Molecular dynamics simulations are used to give insights to the rate of diamond preservation throughout the free expansion and the catcher impact process, highlighting the challenges of diamond retrieval. Raman spectroscopy data show graphitic signatures on a catcher plate confirming that the shock-compressed PS is transformed. First electron microscopy analyses of solid catcher plates yield an outstanding number of different spherical-like objects in the size range between ten(s) up to hundreds of nanometres, which are one type of two potential diamond candidates identified. The origin of some objects can unambiguously be assigned, while the history of others remains speculative.