The classical motion of a one-dimensional chain of atoms coupled through a specific force function that depends on position shows features very similar to the Wannier-Stark problem of a quantum particle under the combined effects of a periodic lattice potential and a constant electric field. Both problems exhibit localized modes and a ladder of equally-spaced eigenfrequencies, leading to temporal dynamics characterized by periodic oscillations.

Optical rectification of intense, circularly polarized light penetrating a material generates a static magnetic field aligned with the light's direction and proportional to its intensity. Recent experiments have unveiled a substantial, orders-of-magnitude gap between the observed magnetization and theoretical predictions. In this study, we demonstrate that circularly polarized light creates large non-Maxwellian fields that disrupt time-reversal symmetry, effectively mimicking authentic magnetic fields within the material while eluding detection externally. These unconventional fields give rise to Faraday-rotation-like phenomena, which are a high-frequency manifestation of Berry's curvature.

The concept of Wannier-Stark ladders, describing the equally spaced spectrum of a tightly bound particle in a constant electric field, is generalized to account for arbitrary slowly varying potentials. It is shown that an abrupt transition exists that separates Wannier-Stark-like from effective-mass-like behavior when the depth of the perturbation becomes equal to the width of the band of extended states. For potentials bounded from below, the spectrum bifurcates above the critical energy while the wavefunctions detach from the effective-mass region and split into two pieces.

A resolvable quantum many-body Hamiltonian is introduced that mimics the behavior of the autocatalytic chemical reaction A+B⇄2B involving two different molecular species, A and B. The model also describes two nonlinearly coupled modes of an optical cavity. Consistent with the current understanding of the relaxation dynamics of integrable systems in isolation, the wave function following a quantum quench exhibits irreversibility with retention of the memory about its initial conditions. Salient features of the model include a marked similarity with conventional quantum decay and a total B-to-A conversion, with associated classical-like behavior of the wave function, when the initial state does not contain A-type molecules.

We report the observation of photo-induced plasmon-phonon coupled modes in the group IV-VI semiconductor PbTe using Fourier-transform inelastic X-ray scattering at the Linac Coherent Light Source (LCLS). We measure the near-zone-center dispersion of the heavily screened longitudinal optical (LO) phonon branch as extracted from differential changes in x-ray diffuse scattering intensity following above band gap photoexcitation.

Pulses applied to an inhomogeneously broadened set of harmonic oscillators, previously prepared in squeezed states, can lead to a recovery of coherence, manifesting itself as echoes, similar to those exhibited by an ensemble of spins when excited by properly designed electromagnetic pulses. Such echoes, of classical or quantum nature, are expected to arise in the squeezing of linear systems of various sorts and, in particular, light and vibrational modes.

A method involving intensity correlation measurements is described, which allows for the complete removal of Doppler broadening in the emission of electromagnetic radiation from far-away sources that are inaccessible to conventional Doppler-free measurements. The technique, relying on a correction to g(2) of order N-1, probes the separation between neighboring spectral lines and is also applicable to the elimination of broadening due to collisions (N is the number of emitting particles and g(2) is the second-order field correlation function). Possible applications include a determination of cosmological parameters from red shifts of gravitationally-lensed quasars.

Rabi oscillations and Floquet states are likely the most familiar concepts associated with a periodically time-varying Hamiltonian. Here, we present an exactly solvable model of a two-level system coupled to both a continuum and a classical field that varies sinusoidally with time, which sheds light on the relationship between the two problems. For a field of the rotating-wave-approximation form, results show that the dynamics of the two-level system can be mapped exactly onto that for a static field, if one shifts the energy separation between the two levels by an amount equal to ℏω, where ω is the frequency of the field and ℏ is Planck's constant. This correspondence allows one to view Rabi oscillations and Floquet states from the simpler perspective of their time-independent-problem equivalents. The comparison between the rigorous results and those from perturbation theory helps clarify some of the difficulties underlying textbook proofs of Fermi's golden rule, and the discussions on quantum decay and linear response theory.

A brief, tutorial account is given of the differences between the near and far regions of the elec-tromagnetic field emphasizing the source-dependent behavior of the former and the universal properties of the latter. Field patterns of near-field plates, that is, metasurfaces used for sub-wavelength applications, are discussed in some detail. Examples are given of fields that decay away from the plates in an exponential manner, a ubiquitous feature of many interface problems, and metasurfaces for which the decay is not exponential, but algebraic. It is also shown that a properly designed system of two parallel near-field plates can produce fields that exhibit pseudo minima, which are potentially useful for near-field tweezer-like applications.

An awkward question from an amateur science buff makes the author realise they do not fully understand what defines a quantum measuring device.

We used a combination of polarized Raman spectroscopy and spin wave calculations to study magnetic excitations in the strong spin-orbit-coupled bilayer perovskite antiferromagnet Sr_{3}Ir_{2}O_{7}. We observed two broad Raman features at ∼800 and ∼1400  cm^{-1} arising from magnetic excitations. Unconventionally, the ∼800  cm^{-1} feature is fully symmetric (A_{1g}) with respect to the underlying tetragonal (D_{4h}) crystal lattice which, together with its broad line shape, definitively rules out the possibility of a single magnon excitation as its origin. In contrast, the ∼1400  cm^{-1} feature shows up in both the A_{1g} and B_{2g} channels. From spin wave and two-magnon scattering cross-section calculations of a tetragonal bilayer antiferromagnet, we identified the ∼800  cm^{-1} (1400  cm^{-1}) feature as two-magnon excitations with pairs of magnons from the zone-center Γ point (zone-boundary van Hove singularity X point). We further found that this zone-center two-magnon scattering is unique to bilayer perovskite magnets which host an optical branch in addition to the acoustic branch, as compared to their single layer counterparts. This zone-center two-magnon mode is distinct in symmetry from the time-reversal symmetry broken "spin wave gap" and "phase mode" proposed to explain the ∼92  meV (742  cm^{-1}) gap in resonant inelastic x-ray spectroscopy magnetic excitation spectra of Sr_{3}Ir_{2}O_{7}.

We report on the observation of coherent terahertz (THz) emission from the quasi-one-dimensional charge-density wave (CDW) system, blue bronze (K0.3MoO3), upon photo-excitation with ultrashort near-infrared optical pulses. The emission contains a broadband, low-frequency component due to the photo-Dember effect, which is present over the whole temperature range studied (30-300 K), as well as a narrow-band doublet centered at 1.5 THz, which is only observed in the CDW state and results from the generation of coherent transverse-optical phonons polarized perpendicular to the incommensurate CDW b-axis. As K0.3MoO3 is centrosymmetric, the lowest-order generation mechanism which can account for the polarization dependence of the phonon emission involves either a static surface field or quadrupolar terms due to the optical field gradients at the surface. This phonon signature is also present in the ground-state conductivity, and decays in strength with increasing temperature to vanish above T similar to 100 K, i.e. significantly below the CDW transition temperature. The temporal behavior of the phonon emission can be well described by a simple model with two coupled modes, which initially oscillate with opposite polarity.

We have used rotational anisotropic polarized Raman spectroscopy to study the symmetries, the temperature, and the doping dependence of the charge ordered state in metallic (Sr1-xLax)(3)Ir2O7. Despite the fact that the Raman probe size is greater than the charge ordering length, we establish that the charge ordering breaks the fourfold rotational symmetry of the underlying tetragonal crystal lattice into twofold, as well as the translational symmetry, and forms short-range domains with 90 degrees rotated charge order wave vectors, as soon as the charge order sets in below T-CO = similar to 200 K and across the doping-induced insulator metal transition. We observe that this charge order mode frequency remains nearly constant over a wide temperature range and up to the highest doping level. These features above are highly reminiscent of the ubiquitous unidirectional charge order in underdoped high-T-C copper-oxide-based superconductors (cuprates). We further resolve that the charge order damping rate diverges when approaching T-CO from below and increases significantly as increasing the La-doping level, which resembles the behaviors for a disorder-interrupted ordered phase and has not been observed for the charge order in cuprates.

Raman scattering [K. M. F. Shahil et al., Appl. Phys. Lett. 96, 153103 (2010), V. Gnezdilov et al., Phys. Rev. B 84, 195118 (2011) and H. -H. Kung et al., Phys. Rev. B 95, 245406 (2017)], inelastic helium scattering [X. Zhu et al., Phys. Rev. Lett. 107, 186102 (2011)] and photoemission experiments [J. A. Sobota et al., Phys. Rev. Lett. 113, 157401 (2014)] on the topological insulators Bi2Se3 and Bi2Te3 show features in the range similar to 50-160 cm(-1), which have been assigned alternatively to Raman-forbidden, bulk infrared modes arising from symmetry breaking at the surface or to surface phonons, which couple to the topologically protected electronic states. Here, we present temperature-and wavelength-dependent Raman studies showing additional modes we ascribe to surface phonons in both Bi2Se3 and Bi2Te3. Our assignment is supported by density functional theory calculations revealing surface phonons at frequencies close to those of the extra peaks in the Raman data. The theoretical results also indicate that these modes are not a consequence of spin-orbit coupling and, thus, that their occurrence is unrelated to the topological properties of these materials.

It has been recently shown that especially engineered light beams have the remarkable ability to propagate along curved trajectories in vacuum. Current methods for generating accelerating beams use phase modulators and lenses leading to length scales on the order of tens of centimeters or larger. This poses constraints and severely limits their applicability inside materials. Here, we accelerate light inside glass using a metasurface consisting of plasmonic nanoantennas. Highly-bending beams with radii of curvature on the order of a hundred microns were generated, and the imaged intensities agree well with theory. Our approach for generating accelerating beams allows for their integration into on-chip photonic systems.

Synchrotron radiation-namely, electromagnetic radiation produced by charges moving in a curved path-is regularly generated at large-scale facilities where giga-electron volt electrons move along kilometer-long circular paths. We use a metasurface to bend light and demonstrate synchrotron radiation produced by a subpicosecond pulse, which moves along a circular arc of radius 100 micrometers inside a nonlinear crystal. The emitted radiation, in the terahertz frequency range, results from the nonlinear polarization induced by the pulse. The generation of synchrotron radiation from a pulse revolving about a circular trajectory holds promise for the development of on-chip terahertz sources.

We use coherent midinfrared optical pulses to resonantly excite large-amplitude oscillations of the Si-C stretching mode in silicon carbide. When probing the sample with a second pulse, we observe parametric optical gain at all wavelengths throughout the reststrahlen band. This effect reflects the amplification of light by phonon-mediated four-wave mixing and, by extension, of optical-phonon fluctuations. Density functional theory calculations clarify aspects of the microscopic mechanism for this phenomenon. The high-frequency dielectric permittivity and the phonon oscillator strength depend quadratically on the lattice coordinate; they oscillate at twice the frequency of the optical field and provide a parametric drive for the lattice mode. Parametric gain in phononic four-wave mixing is a generic mechanism that can be extended to all polar modes of solids, as a means to control the kinetics of phase transitions, to amplify many-body interactions or to control phonon-polariton waves.

We present a polarization resolved Raman scattering study of surface vibration modes in the topological insulator ${\mathrm{Bi}}_{2}{\mathrm{Se}}_{3}$ single crystal and thick films. Besides the four Raman active bulk phonons, we observed four additional modes with much weaker intensity and slightly lower energy than the bulk counterparts. Using symmetry analysis, we assigned these additional modes to out-of-plane surface phonons. Comparing with first-principle calculations, we conclude that the appearance of these modes is due to $c$-axis lattice distortion and van der Waals gap expansion near the crystal surface. Two of the surface modes at 60 and 173 ${\mathrm{cm}}^{\ensuremath{-}1}$ are associated with Raman active ${A}_{1g}$ bulk phonon modes, the other two at 136 and 158 ${\mathrm{cm}}^{\ensuremath{-}1}$ are associated with infrared active bulk phonons with ${A}_{2u}$ symmetry. The latter become Raman allowed due to reduction of crystalline symmetry from ${D}_{3d}$ in the bulk to ${C}_{3v}$ on the crystal surface. In particular, the 158 ${\mathrm{cm}}^{\ensuremath{-}1}$ surface phonon mode shows a Fano line shape under resonant excitation, suggesting interference in the presence of electron-phonon coupling of the surface excitations.